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We analyze the low energy properties of a device with $N+1$ quantum dots in a star configuration. A central quantum dot is tunnel coupled to source and drain electrodes and to $N$ quantum dots. Extending previous results for the $N=2$ case we show th at, in the appropriate parameter regime, the low energy Hamiltonian of the system is a ferromagnetic Kondo model for a $S=(N-1)/2$ impurity spin. For small enough interdot tunnel coupling, however, a two-stage Kondo effect takes place as the temperature is decreased. The spin $1/2$ in the central quantum dot is Kondo screened first and at lower temperatures the antiferromagnetic coupling to the side coupled quantum dots leads to an underscreened $S=N/2$ Kondo effect. We present numerical results for the thermodynamic and spectral properties of the system which show a singular behavior at low temperatures and allow to characterize the different strongly correlated regimes of the device.
Electron Spin Resonance (ESR) measurements performed on the filled skutterudite system Ce1-x$YbxFe4P12 (x< 0.003) unequivocally reveal the coexistence of two Yb3+ resonances, associated with sites of considerably different occupations and temperature behaviors. Detailed analysis of the ESR data suggests a scenario where the fraction of oversized (Fe2P3)4 cages that host Yb ions are filled with a low occupation of on-center Yb3+ sites and a highly occupied T-dependent distribution of off-center Yb3+ sites. Analysis of the 171Yb3+ (I=1/2) isotope hyperfine splittings reveal that these two sites are associated with a low (~ 1 GHz) and a high (> 15 GHz) rattling frequency, respectively. Our findings introduce Yb3+ in Th symmetry systems and uses the Yb3+ ESR as a sensitive microscopic probe to investigate the Yb3+ ions dynamics.
359 - Julian Rincon , D. J. Garcia , 2009
A distributed-memory parallelization strategy for the density matrix renormalization group is proposed for cases where correlation functions are required. This new strategy has substantial improvements with respect to previous works. A scalability an alysis shows an overall serial fraction of 9.4% and an efficiency of around 60% considering up to eight nodes. Sources of possible parallel slowdown are pointed out and solutions to circumvent these issues are brought forward in order to achieve a better performance.
Despite extensive research on the skutterudites for the last decade, their electric crystalline field ground state is still a matter of controversy. We show that Electron Spin Resonance (ESR) measurements can determine the full set of crystal field p arameters (CFPs) for the Th cubic symmetry (Im3) of the Ce$_{1-x}$R$_{x}$Fe$_{4}$P$_{12}$ (R = Dy, Er, Yb, $xlesssim 0.003$) skutterudite compounds. From the analysis of the ESR data the three CFPs, B4c, B6c and B6t were determined for each of these rare-earths at the Ce$^{3+}$ site. The field and temperature dependence of the measured magnetization for the doped crystals are in excellent agreement with the one predicted by the CFPs Bnm derived from ESR.
We report measurements of temperature dependent magnetic susceptibility, resonant x-ray magnetic scattering (XRMS) and heat capacity on single crystals of Tb1-xLaxRhIn5 for nominal concentrations in the range 0.0 < x < 1.0. TbRhIn5 is an antiferromag netic (AFM) compound with TN ~ 46 K, which is the highest TN values along the RRhIn5 series. We explore the suppression of the antiferromagnetic (AFM) state as a function of La-doping considering the effects of La-induced dilution and perturbations to the tetragonal crystalline electrical field (CEF) on the long range magnetic interaction between the Tb$^{3+}$ ions. Additionally, we also discuss the role of disorder. Our results and analysis are compared to the properties of the undoped compound and of other members of the RRhIn5 family and structurally related compounds (R2RhIn8 and RIn3). The XRMS measurements reveal that the commensurate magnetic structure with the magnetic wave-vector (0,1/2,1/2) observed for the undoped compound is robust against doping perturbations in Tb0.6La0.4RhIn5 compound.
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