Moire materials, and in particular twisted bilayer graphene (TBG), exhibit a range of fascinating phenomena, that emerge from the interplay of band topology and interactions. We show that the non-linear second-order photoresponse is an appealing prob
e of this rich interplay. A dominant part of the photoresponse is the shift-current, which is determined by the geometry of the electronic wavefunctions and carrier properties, and thus becomes strongly modified by electron-electron interactions. We analyze its dependence on the twist angle and doping, and investigate the role of interactions. In the absence of interactions, the response of the system is dictated by two energy scales: the mean energy of direct transitions between the hole and electron flat bands, and the gap between flat and dispersive bands. Including electron-electron interactions, both enhance the response at the non-interacting characteristic frequencies as well as produce new resonances. We attribute these changes to the filling-dependent band renormalization in TBG. Our results highlight the connection between non-trivial geometric properties of TBG and its optical response, as well as demonstrate how optical probes can access the role of interactions in moire materials.
Twisted bilayer graphene exhibits a panoply of many-body phenomena that are intimately tied to the appearance of narrow and well isolated electronic bands near magic-angle. The microscopic ingredients that are responsible for the complex experimental
phenomenology include electron-electron (phonon) interactions and non-trivial Bloch wavefunctions associated with the narrow bands. Inspired by recent experiments, we focus here on an interplay of two independent interaction-induced phenomena on superconductivity. We analyze the combined effects of Coulomb interaction driven band-flattening and phonon-mediated attraction due to the exchange of multiple electron-phonon umklapp processes, as a function of filling and twist angle. The former leads to a filling-dependent enhancement of the renormalized density of states, which contributes to a robust increase in the tendency towards pairing in a range of angles near magic-angle. In addition, the minimal spatial extent associated with the Wannier functions develops a non-trivial enhancement as a result of these many-body renormalizations, which can further contribute towards stabilizing the superconducting state over a wider range of fillings and twist-angles.
Flat electronic bands, characteristic of magic-angle twisted bilayer graphene (TBG), host a wealth of correlated phenomena. Early theoretical considerations suggested that, at the magic angle, the Dirac velocity vanishes and the entire width of the m
oire bands becomes extremely narrow. Yet, this scenario contradicts experimental studies that reveal a finite Dirac velocity as well as bandwidths significantly larger than predicted. Here we use spatially resolved spectroscopy in finite and zero magnetic fields to examine the electronic structure of moire bands and their intricate connection to correlated phases. By following the relative shifts of Landau levels in finite fields, we detect filling-dependent band flattening, that unexpectedly starts already at ~1.3 degrees, well above the magic angle and hence nominally in the weakly correlated regime. We further show that, as the twist angle is reduced, the moire bands become maximally flat at progressively lower doping levels. Surprisingly, when the twist angles reach values for which the maximal flattening occurs at approximate filling of $-2$, $+1$,$+2$,$+3$ electrons per moire unit cell, the corresponding zero-field correlated phases start to emerge. Our observations are corroborated by calculations that incorporate an interplay between the Coulomb charging energy and exchange interactions; together these effects produce band flattening and hence a significant density-of-states enhancement that facilitates the observed symmetry-breaking cascade transitions. Besides emerging phases pinned to integer fillings, we also experimentally identify a series of pronounced correlation-driven band deformations and soft gaps in a wider doping range around $pm 2$ filling where superconductivity is expected. Our results highlight the role of interaction-driven band-flattening in forming robust correlated phases in TBG.
Collective plasma excitations in moire flat bands display unique properties reflecting strong electron-electron interactions and unusual carrier dynamics in these systems. Unlike the conventional two-dimensional plasmon modes, dispersing as $sqrt{k}$
at low frequencies and plunging into particle-hole continuum at higher frequencies, the moire plasmons pierce through the flat-band continuum and acquire a strong over-the-band character. Due to the complex structure of the moire superlattice unit cell, the over-the-band plasmons feature several distinct branches connected through zone folding in the superlattice Brillouin zone. Using a toy Hubbard model for the correlated insulating order in a flat band, we predict that these high-frequency modes become strongly dipole-active upon the system undergoing charge ordering, with the low-frequency modes gapped out within the correlated insulator gap. Strong dipole moments and sensitivity to charge order make these modes readily accessible by optical measurements, providing a convenient diagnostic of the correlated states.
We propose a new current-driven mechanism for achieving significant plasmon dispersion nonreciprocity in systems with narrow, strongly hybridized electron bands. The magnitude of the effect is controlled by the strength of electron-electron interacti
ons $alpha$, which leads to its particular prominence in moire materials, characterized by $alpha gg 1$. Moreover, this phenomenon is most evident in the regime where Landau damping is quenched and plasmon lifetime is increased. The synergy of these two effects holds a great promise for novel optoelectronic applications of moire materials.
Identifying the microscopic mechanism for superconductivity in magic-angle twisted bilayer graphene (MATBG) is an outstanding open problem. While MATBG exhibits a rich phase-diagram, driven partly by the strong interactions relative to the electronic
bandwidth, its single-particle properties are unique and likely play an important role in some of the phenomenological complexity. Some of the salient features include an electronic bandwidth smaller than the characteristic phonon bandwidth and a non-trivial structure of the underlying Bloch wavefunctions. We perform a theoretical study of the cooperative effects due to phonons and plasmons on pairing in order to disentangle the distinct role played by these modes on superconductivity. We consider a variant of MATBG with an enlarged number of fermion flavors, $N gg 1$, where the study of pairing instabilities reduces to the conventional (weak-coupling) Eliashberg framework. In particular, we show that certain umklapp processes involving mini-optical phonon modes, which arise physically as a result of the folding of the original acoustic branch of graphene due to the moire superlattice structure, contribute significantly towards enhancing pairing. We also investigate the role played by the dynamics of the screened Coulomb interaction on pairing, which leads to an enhancement in a narrow window of fillings, and study the effect of external screening due to a metallic gate on superconductivity. At strong coupling the dynamical pairing interaction leaves a spectral mark in the single particle tunneling density of states. We thus predict such features will appear at specific frequencies of the umklapp phonons corresponding to the sound velocity of graphene times an integer multiple of the Brillouin zone size.
Surface plasmons in 2-dimensional electron systems with narrow Bloch bands feature an interesting regime in which Landau damping (dissipation via electron-hole pair excitation) is completely quenched. This surprising behavior is made possible by stro
ng coupling in narrow-band systems characterized by large values of the fine structure constant $alpha=e^2/hbar kappa v_{rm F}$. Dissipation quenching occurs when dispersing plasmon modes rise above the particle-hole continuum, extending into the forbidden energy gap that is free from particle-hole excitations. The effect is predicted to be prominent in moire graphene, where at magic twist-angle values, flat bands feature $alphagg1$. The extinction of Landau damping enhances spatial optical coherence. Speckle-like interference, arising in the presence of disorder scattering, can serve as a telltale signature of undamped plasmons directly accessible in near-field imaging experiments.
In Dirac materials linear band dispersion blocks momentum-conserving interband transitions, creating a bottleneck for electron-hole pair production and carrier multiplication in the photoexcitation cascade. Here we show that the decays are unblocked
and the bottleneck is relieved by subtle many-body effects involving multiple off-shell e-h pairs. The decays result from a collective behavior due to emission of many soft pairs. We discuss characteristic signatures of the off-shell pathways, in particular the sharp angular distribution of secondary carriers, resembling relativistic jets in high-energy physics. The jets can be directly probed using solid-state equivalent of particle detectors. Collinear scattering enhances carrier multiplication, allowing for emission of as many as ${sim}10$ secondary carriers per single absorbed photon.
Interactions between charge carriers in graphene lead to logarithmic renormalization of observables mimicking the behavior known in (3+1)-dimensional quantum electrodynamics (QED). Here we analyze soft electron-hole (e-h) excitations generated as a r
esult of fast charge dynamics, a direct analog of the signature QED effect - multiple soft photons produced by the QED vacuum shakeup. We show that such excitations are generated in photon absorption, when a photogenerated high-energy e-h pair cascades down in energy and gives rise to multiple soft e-h excitations. This fundamental process is manifested in a double-log divergence in the emission rate of soft pairs and a characteristic power-law divergence in their energy spectrum of the form $frac{1}{omega}ln left(frac{omega}{Delta}right) $. Strong carrier-carrier interactions make pair production a prominent pathway in the photoexcitation cascade.
Quantum Measure Theory (QMT) is an approach to quantum mechanics, based on the path integral, in which quantum theory is conceived of as a generalised stochastic process. One of the postulates of QMT is that events with zero quantum measure do not oc
cur, however this is not sufficient to give a full picture of the quantum world. Determining the other postulates is a work in progress and this paper investigates a proposal called the Multiplicative Scheme for QMT in which the physical world corresponds, essentially, to a set of histories from the path integral. This scheme is applied to Sorkins $n$-site hopper, a discrete, unitary model of a single particle on a ring of $n$ sites, motivated by free Schrodinger propagation. It is shown that the multiplicative schemes global features lead to the conclusion that no non-trivial, time-finite event can occur.
