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Quasiparticle properties in the superconducting state are masked by the superfluid and are not directly accessible to infrared spectroscopy. We show how one can use a Kramers--Kronig transformation to separate the quasiparticle from superfluid respon se and extract intrinsic quasiparticle properties in the superconducting state. We also address the issue of a narrow quasiparticle peak observed in microwave measurements, and demonstrate how it can be combined with infrared measurements to obtain unified picture of electrodynamic properties of cuprate superconductors.
The optical conductivity of quasicrystals is characterized by two features not seen in ordinary metallic systems. There is an absence of the Drude peak and the interband conductivity rises linearly from a very low value up to normal metallic levels o ver a wide range of frequencies. The absence of a Drude peak has been attributed to a pseudogap at the Fermi surface but a detailed explanation of the linear behavior has not been found. Here we show that the linear conductivity, which seems to be universal in all Al based icosahedral quasicrystal families, as well as their periodic approximants, follows from a simple model that assumes that the entire Fermi surface is gapped except at a finite set of Dirac points. There is no evidence of a semiconducting gap in any of the materials suggesting that the Dirac spectrum is massless, protected by topology leading to a Weyl semimetal. This model gives rise to a linear conductivity with only one parameter, the Fermi velocity. This picture suggests that decagonal quasicrystals should, like graphene, have a frequency independent conductivity, without a Drude peak. This is in accord with the experimental data as well.
Universal scaling relations are of tremendous importance in science, as they reveal fundamental laws of nature. Several such scaling relations have recently been proposed for superconductors; however, they are not really universal in the sense that s ome important families of superconductors appear to fail the scaling relations, or obey the scaling with different scaling pre-factors. In particular, a large group of materials called organic (or molecular) superconductors are a notable example. Here, we show that such apparent violations are largely due to the fact that the required experimental parameters were collected on different samples, with different experimental techniques. When experimental data is taken on the same sample, using a single experimental technique, organic superconductors, as well as all other studied superconductors, do in fact follow universal scaling relations.
We analyze optical spectroscopy data of the electron-doped superconductor (Pr$_{2-x}$Ce$_x$)CuO$_4$ (PCCO) to investigate the coupling of the charge carriers to bosonic modes. The method of analysis is the inversion of the optical scattering rate $ta u^{-1}_{rm op}(omega,T)$ at different temperatures $T$ by means of maximum entropy technique combined with Eliashberg theory. We find that in the superconducting state the charge carriers couple to two dominant modes one at $sim 10 $meV and a second one at $sim 45 $meV. The low energy mode shows a strong temperature dependence and disappears at or slightly above the critical temperature $T_c$. The high energy mode exists above $T_c$ and moves towards higher energies with increasing temperatures. It also becomes less prominent at temperatures $> 100 $K above which it evolves into a typical spin-fluctuation background. In contrast to the hole-doped High-$T_c$ superconductors PCCO proves to be a superconductor close to the dirty limit.
We have extended the range of the high-pressure optical spectroscopy to the far-infrared region keeping the accuracy of ambient-pressure experiments. The newly-developed method offers a powerful tool for the study of pressure-induced phase transition s and electronic-structural changes in correlated electron systems. The novel-type optical pressure cell, equipped with large free-aperture diamond window, allows the measurement of optical reflectivity down to $omegaapprox20-30$ cm$^{-1}$ for hydrostatic pressures up to $papprox26$ kbar. The efficiency of the technique is demonstrated by the investigation of the 2-dimensional charge-density-wave 1$T$-TaS$_2$ whose electronic structure shows high sensitivity to external pressure. The room-temperature semi-metallic phase of 1$T$-TaS$_2$ is effectively extended by application of pressure and stabilized as the ground state above $p=14$ kbar. The corresponding fully incoherent low-energy optical conductivity is almost temperature independent below T=300 K. For intermediate pressures, the onset of the low-temperature insulating phase is reflected by the sudden drop of the reflectivity and by the emergence of sharp phonon resonances.
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