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106 - T. Shang , Wesen Wei , C. Baines 2018
The noncentrosymmetric superconductor Mo$_3$Rh$_2$N, with $T_c = 4.6$ K, adopts a $beta$-Mn-type structure (space group $P$4$_1$32), similar to that of Mo$_3$Al$_2$C. Its bulk superconductivity was characterized by magnetization and heat-capacity mea surements, while its microscopic electronic properties were investigated by means of muon-spin rotation and relaxation ($mu$SR). The low-temperature superfluid density, measured via transverse-field (TF)-$mu$SR, evidences a fully-gapped superconducting state with $Delta_0 = 1.73 k_mathrm{B}T_c$, very close to 1.76 $k_mathrm{B}T_c$ - the BCS gap value for the weak coupling case, and a magnetic penetration depth $lambda_0 = 586$ nm. The absence of spontaneous magnetic fields below the onset of superconductivity, as determined by zero-field (ZF)-$mu$SR measurements, hints at a preserved time-reversal symmetry in the superconducting state. Both TF-and ZF-$mu$SR results evidence a spin-singlet pairing in Mo$_3$Rh$_2$N.
335 - T. Shang , G. M. Pang , C. Baines 2018
The noncentrosymmetric superconductor Re$_{24}$Ti$_{5}$, a time-reversal symmetry (TRS) breaking candidate with $T_c = 6$,K, was studied by means of muon-spin rotation/relaxation ($mu$SR) and tunnel-diode oscillator (TDO) techniques. At a macroscopic level, its bulk superconductivity was investigated via electrical resistivity, magnetic susceptibility, and heat capacity measurements. The low-temperature penetration depth, superfluid density and electronic heat capacity all evidence an $s$-wave coupling with an enhanced superconducting gap. The spontaneous magnetic fields revealed by zero-field $mu$SR below $T_c$ indicate a time-reversal symmetry breaking and thus the unconventional nature of superconductivity in Re$_{24}$Ti$_{5}$. The concomitant occurrence of TRS breaking also in the isostructural Re$_6$(Zr,Hf) compounds, hints at its common origin in this superconducting family and that an enhanced spin-orbital coupling does not affect pairing symmetry.
110 - A. Ribak , I. Silber , C. Baines 2017
1T-TaS$_2$ is a layered transition metal dichalgeonide with a very rich phase diagram. At T=180K it undergoes a metal to Mott insulator transition. Mott insulators usually display anti-ferromagnetic ordering in the insulating phase but 1T-TaS$_2$ was never shown to order magnetically. In this letter we show that 1T-TaS$_2$ has a large paramagnetic contribution to the magnetic susceptibility but it does not show any sign of magnetic ordering or freezing down to 20mK, as probed by $mu$SR, possibly indicating a quantum spin liquid ground state. Although 1T-TaS$_2$ exhibits a strong resistive behavior both in and out-of plane at low temperatures we find a linear term in the heat capacity suggesting the existence of a Fermi-surface, which has an anomalously strong magnetic field dependence.
102 - J. Xu , C. Balz , C. Baines 2016
We present a muon spin relaxation study on the Ising pyrochlore Nd$_2$Zr$_2$O$_7$ which develops an all-in-all-out magnetic order below 0.4~K. At 20~mK far below the ordering transition temperature, the zero-field muon spin relaxation spectra show no static features and can be well described by a dynamical Gaussian-broadened Gaussian Kubo-Toyabe function indicating strong fluctuations of the ordered state. The spectra of the paramagnetic state (below 4.2~K) reveal anomalously slow paramagnetic spin dynamics and show only small difference with the spectra of the ordered state. We find that the fluctuation rate decreases with decreasing temperature and becomes nearly temperature independent below the transition temperature indicating persistent slow spin dynamics in the ground state. The field distribution width shows a small but sudden increase at the transition temperature and then becomes almost constant. The spectra in applied longitudinal fields are well fitted by the conventional dynamical Gaussian Kubo-Toyabe function, which further supports the dynamical nature of the ground state. The fluctuation rate shows a peak as a function of external field which is associated with a field-induced spin-flip transition. The strong dynamics in the ordered state are attributed to the transverse coupling of the Ising spins introduced by the multipole interactions.
A study of the temperature and field dependence of the penetration depth lambda of the superconductor RbFe_2As_2 (T_c=2.52 K) was carried out by means of muon-spin rotation measurements. In addition to the zero temperature value of the penetration de pth lambda(0)=267(5) nm, a determination of the upper critical field B_c2(0)=2.6(2) T was obtained. The temperature dependence of the superconducting carrier concentration is discussed within the framework of a multi-gap scenario. Compared to the other 122 systems which exhibit much higher Fermi level, a strong reduction of the large gap BCS ratio 2Delta/k_B T_c is observed. This is interpreted as a consequence of the absence of interband processes. Indications of possible pair-breaking effect are also discussed.
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