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We report low-energy inelastic neutron scattering data of the paramagnetic (PM) to hidden-order (HO) phase transition at $T_0=17.5,{rm K}$ in URu$_2$Si$_2$. While confirming previous results for the HO and PM phases, our data reveal a pronounced wave vector dependence of low-energy excitations across the phase transition. To analyze the energy scans we employ a damped harmonic oscillator model containing a fit parameter $1/Gamma$ which is expected to diverge at a second-order phase transition. Counter to expectations the excitations at $vec{Q}_1=(1.44,0,0)$ show an abrupt step-like suppression of $1/Gamma$ below $T_0$, whereas excitations at $vec{Q}_0=(1,0,0)$, associated with large-moment antiferromagnetism (LMAF) under pressure, show an enhancement and a pronounced peak of $1/Gamma$ at $T_0$. Therefore, at the critical HO temperature $T_0$, LMAF fluctuations become nearly critical as well. This is the behavior expected of a super-vector order parameter with nearly degenerate components for the HO and LMAF leading to nearly isotropic fluctuations in the combined order-parameter space.
Spin manipulation using electric currents is one of the most promising directions in the field of spintronics. We used neutron scattering to observe the influence of an electric current on the magnetic structure in a bulk material. In the skyrmion la ttice of MnSi, where the spins form a lattice of magnetic vortices similar to the vortex lattice in type II superconductors, we observe the rotation of the diffraction pattern in response to currents which are over five orders of magnitude smaller than those typically applied in experimental studies on current-driven magnetization dynamics in nanostructures. We attribute our observations to an extremely efficient coupling of inhomogeneous spin currents to topologically stable knots in spin structures.
Recent small angle neutron scattering suggests, that the spin structure in the A-phase of MnSi is a so-called triple-$Q$ state, i.e., a superposition of three helices under 120 degrees. Model calculations suggest that this structure in fact is a latt ice of so-called skyrmions, i.e., a lattice of topologically stable knots in the spin structure. We report a distinct additional contribution to the Hall effect in the temperature and magnetic field range of the proposed skyrmion lattice, where such a contribution is neither seen nor expected for a normal helical state. Our Hall effect measurements constitute a direct observation of a topologically quantized Berry phase that identifies the spin structure seen in neutron scattering as the proposed skyrmion lattice.
We have studied the pressure dependence of the magnetization of single crystalline CeSi_1.81. At ambient pressure ferromagnetism develops below T_C = 9.5 Below ~ 5 K an additional shoulder in low-field hysteresis loops and a metamagnetic crossover ar ound 4 T suggest the appearance of an additional magnetic modulation to the ferromagnetic state. The suppression of the magnetic order in CeSi_1.81 as function of temperature at ambient pressure and as function of pressure at low temperature are in remarkable qualitative agreement. The continuous suppression of the ordered moment at p ~ 13.1 kbar suggests the existence of a ferromagnetic quantum critical point in this material.
Supplementary information for our manuscript, entitled Spontaneous Skyrmion Ground States of Magnetic Metals, cond-mat/0603103, is presented. The physical nature of the gradient terms of our generalized micromagnetic model for ferromagnets with softe ned longitudinal fluctuations is explained. The relationship of our micromagnetic model with the spin fluctuation theory of itinerant-electron magnets is discussed. Experimental estimates of the parameter eta, which accounts for an effective reduced longitudinal stiffness, are presented for real materials from published polarized neutron scattering experiments on EuS, Ni and MnSi. The available experimental data clearly show that eta is significantly reduced for the latter two systems. It is suggested that particle-hole excitations are at the root of this longitudinal softness in itinerant-electron ferromagnets. The current status of the experimental evidence supporting spontaneous, amorphous skyrmion textures in MnSi and other materials is reviewed. Finally, we also address the general potential of skyrmion textures in chiral magnets for other fields of physics.
Since the 1950s Heisenberg and others have attempted to explain the appearance of countable particles in quantum field theory in terms of stable localized field configurations. As an exception Skyrmes model succeeded to describe nuclear particles as localized states, so-called skyrmions, within a non-linear field theory. Skyrmions are a characteristic of non-linear continuum models ranging from microscopic to cosmological scales. Skyrmionic states have been found under non-equilibrium conditions, or when stabilised by external fields or the proliferation of topological defects. Examples are Turing patterns in classical liquids, spin textures in quantum Hall magnets, or the blue phases in liquid crystals, respectively. However, it is believed that skyrmions cannot form spontaneous ground states like ferromagnetic or antiferromagnetic order in magnetic materials. Here, we show theoretically that this assumption is wrong and that skyrmion textures may form spontaneously in condensed matter systems with chiral interactions without the assistance of external fields or the proliferation of defects. We show this within a phenomenological continuum model, that is based on a few material-specific parameters that may be determined from experiment. As a new condition not considered before, we allow for softened amplitude variations of the magnetisation - a key property of, for instance, metallic magnets. Our model implies that spontaneous skyrmion lattice ground states may exist quite generally in a large number of materials, notably at surfaces and in thin films as well as in bulk compounds, where a lack of space inversion symmetry leads to chiral interactions.
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