Frequency encoding of quantum information together with fiber and integrated photonic technologies can significantly reduce the complexity and resource requirements for realizing all-photonic quantum networks. The key challenge for such frequency dom
ain processing of single photons is to realize coherent and selective interactions between quantum optical fields of different frequencies over a range of bandwidths. Here, we report frequency-domain Hong-Ou-Mandel interference with spectrally distinct photons generated from a chip-based microresonator. We use four-wave mixing to implement an active frequency beam-splitter and achieve interference visibilities of $0.95 pm 0.02$. Our work establishes four-wave mixing as a tool for selective high-fidelity two-photon operations in the frequency domain which, combined with integrated single-photon sources, provides a building block for frequency-multiplexed photonic quantum networks.
Second-order optical processes lead to a host of applications in classical and quantum optics. With the enhancement of parametric interactions that arise due to light confinement, on-chip implementations promise very-large-scale photonic integration.
But as yet there is no route to a device that acts at the single photon level. Here we exploit the $chi^{(3)}$ nonlinear response of a Si$_{3}$N$_{4}$ microring resonator to induce a large effective $chi^{(2)}$. Effective second-order upconversion (ESUP) of a seed to an idler can be achieved with 74,000 %/W efficiency, indicating that single photon nonlinearity is within reach of current technology. Moreover, we show a nonlinear coupling rate of seed and idler larger than the energy dissipation rate in the resonator, indicating a strong coupling regime. Consequently we observe a Rabi-like splitting, for which we provide a detailed theoretical description. This yields new insight into the dynamics of ultrastrong effective nonlinear interactions in microresonators, and access to novel phenomena and applications in classical and quantum nonlinear optics.
Single-photon sources based on optical parametric processes have been used extensively for quantum information applications due to their flexibility, room-temperature operation and potential for photonic integration. However, the intrinsically probab
ilistic nature of these sources is a major limitation for realizing large-scale quantum networks. Active feedforward switching of photons from multiple probabilistic sources is a promising approach that can be used to build a deterministic source. However, previous implementations of this approach that utilize spatial and/or temporal multiplexing suffer from rapidly increasing switching losses when scaled to a large number of modes. Here, we break this limitation via frequency multiplexing in which the switching losses remain fixed irrespective of the number of modes. We use the third-order nonlinear process of Bragg scattering four-wave mixing as an efficient ultra-low noise frequency switch and demonstrate multiplexing of three frequency modes. We achieve a record generation rate of $4.6times10^4$ multiplexed photons per second with an ultra-low $g^{2}(0)$ = 0.07, indicating high single-photon purity. Our scalable, all-fiber multiplexing system has a total loss of just 1.3 dB independent of the number of multiplexed modes, such that the 4.8 dB enhancement from multiplexing three frequency modes markedly overcomes switching loss. Our approach offers a highly promising path to creating a deterministic photon source that can be integrated on a chip-based platform.
