Domain wall conductivity in semiconducting hexagonal ferroelectric TbMnO$_3$ thin films

Although enhanced conductivity at ferroelectric domain boundaries has been found in BiFeO$_3$ films, Pb(Zr,Ti)O$_3$ films, and hexagonal rare-earth manganite single crystals, the mechanism of the domain wall conductivity is still under debate. Using conductive atomic force microscopy, we observe enhanced conductance at the electrically-neutral domain walls in semiconducting hexagonal ferroelectric TbMnO$_3$ thin films where the structure and polarization direction are strongly constrained along the c-axis. This result indicates that domain wall conductivity in ferroelectric rare-earth manganites is not limited to charged domain walls. We show that the observed conductivity in the TbMnO$_3$ films is governed by a single conduction mechanism, namely, the back-to-back Schottky diodes model tuned by the segregation of defects.

A detailed X-ray investigation of PSR J2021+4026 and $gamma$-Cygni supernova remnant

We have investigated the field around the radio-quiet $gamma$-ray pulsar, PSR J2021+4026, with a ~140 ks XMM-Newton observation and a ~56 ks archival Chandra data. Through analyzing the pulsed spectrum, we show that the X-ray pulsation is purely thermal in nature which suggests the pulsation is originated from a hot polar cap with $Tsim3times10^{6}$ K on the surface of a rotating neutron star. On the other hand, the power-law component that dominates the pulsar emission in the hard band is originated from off-pulse phases, which possibly comes from a pulsar wind nebula. In re-analyzing the Chandra data, we have confirmed the presence of bow-shock nebula which extends from the pulsar to west by ~10 arcsec. The orientation of this nebular feature suggests that the pulsar is probably moving eastward which is consistent with the speculated proper motion by extrapolating from the nominal geometrical center of the supernova remnant (SNR) G78.2+2.1 to the current pulsar position. For G78.2+2.1, our deep XMM-Newton observation also enables a study of the central region and part of the southeastern region with superior photon statistics. The column absorption derived for the SNR is comparable with that for PSR J2021+4026, which supports their association. The remnant emission in both examined regions are in an non-equilibrium ionization state. Also, the elapsed time of both regions after shock-heating is apparently shorter than the Sedov age of G78.2+2.1. This might suggest the reverse shock has reached the center not long ago. Apart from PSR J2021+4026 and G78.2+2.1, we have also serendipitously detected an X-ray flash-like event XMM J202154.7+402855 from this XMM-Newton observation.

X-ray properties of G308.3-1.4 and its central compact object

We present a short Chandra observation that confirms a previous unidentified extended X-ray source, G308.3-1.4, as a new supernova remnant (SNR) in the Milky Way. Apart from identifying its SNR nature, a bright X-ray point source has also been discovered at the geometrical center. Its X-ray spectral properties are similar to those of a particular class of neutron star known as central compact objects (CCOs). On the other hand, the optical properties of this counterpart suggests it to be a late-type star. Together with the interesting ~ 1.4 hours X-ray periodicity found by Chandra, this system can possibly provide the first direct evidence of a compact binary survived in a supernova explosion.

Atomic layer engineering of perovskite oxides for chemically sharp heterointerfaces

Advances in synthesis techniques and materials understanding have given rise to oxide heterostructures with intriguing physical phenomena that cannot be found in their constituents. In these structures, precise control of interface quality, including oxygen stoichiometry, is critical for unambiguous tailoring of the interfacial properties, with deposition of the first monolayer being the most important step in shaping a well-defined functional interface. Here, we studied interface formation and strain evolution during the initial growth of LaAlO3 on SrTiO3 by pulsed laser deposition, in search of a means for controlling the atomic-sharpness of the interfaces. Our experimental results show that growth of LaAlO3 at a high oxygen pressure dramatically enhances interface abruptness. As a consequence, the critical thickness for strain relaxation was increased, facilitating coherent epitaxy of perovskite oxides. This provides a clear understanding of the role of oxygen pressure during the interface formation, and enables the synthesis of oxide heterostructures with chemically-sharper interfaces.

Detection of X-ray periodicity from a new eclipsing polar candidate XGPS-I J183251-100106

We report the results from a detailed analysis of an archival XMM-Newton observation of the X-ray source XGPS-I J183251-100106, which has been suggested as a promising magnetic cataclysmic variable candidate based on its optical properties. A single periodic signal of 1.5 hrs is detected from all EPIC cameras on board XMM-Newton. The phase-averaged X-ray spectrum can be well-modeled with a thermal bremsstrahlung of a temperature kT~50 keV. Both X-ray spectral and temporal behavior of this system suggest it as a eclipsing cataclysmic variable of AM Herculis (or polar) type.

Identification campaign of supernova remnant candidates in the Milky Way - I: Chandra observation of G308.3-1.4

ROSAT all-sky survey (RASS) data have provided another window to search for supernova remnants (SNRs). In reexamining this data archive, a list of unidentified extended X-ray objects have been suggested as promising SNR candidate. However, most of these targets have not yet been fully explored by the state-of-art X-ray observatories. For selecting a pilot target for a long-term identification campaign, we have observed the brightest candidate, G308.3-1.4, with Chandra X-ray observatory. An incomplete shell-like X-ray structure which well-correlated with the radio shell emission at 843 MHz has been revealed. The X-ray spectrum suggests the presence of a shock-heated plasma. All these evidences confirm G308.3-1.4 as a SNR. The brightest X-ray point source detected in this field-of-view is also the one locates closest to the geometrical center of G308.3-1.4, which has a soft spectrum. The intriguing temporal variability and the identification of optical/infrared counterpart rule out the possibility of an isolated neutron star. On the other hand, the spectral energy distribution from Ks band to R band suggests a late-type star. Together with a putative periodicity of sim1.4 hrs, the interesting excesses in V, B bands and H-alpha suggest this source as a promising candidate of a compact binary survived in a supernova explosion (SN).

Two-Dimensional Confinement of 3d1 Electrons in LaTiO3/LaAlO3 Multilayers

We report spectroscopic ellipsometry measurements of the anisotropy of the interband transitions parallel and perpendicular to the planes of (LaTiO3)n(LaAlO3)5 multilayers with n = 1-3. These provide direct information about the electronic structure of the two-dimensional (2D) 3d^1 state of the Ti ions. In combination with LDA+U calculations, we suggest that 2D confinement in the TiO2 slabs lifts the degeneracy of the t_{2g} states leaving only the planar d_xy orbitals occupied. We outline that these multilayers can serve as a model system for the study of the t_{2g} 2D Hubbard model.

Multiple conducting carriers generated in LaAlO3/SrTiO3 heterostructures

We have found that there is more than one type of conducting carriers generated in LaAlO3/SrTiO3 heterostructures by comparing the sheet carrier density and mobility from optical transmission spectroscopy with those from dc-transport measurements. When multiple types of carriers exist, optical characterization dominantly reflects the contribution from the high-density carriers whereas dc-transport measurements may exaggerate the contribution of the high-mobility carriers even though they are present at low-density. Since the low-temperature mobilities determined by dc-transport in the LaAlO3/SrTiO3 heterostructures are much higher than those extracted by optical method, we attribute the origin of high-mobility transport to the low-density conducting carriers.

Strain-coupled ferroelectric polarization in BaTiO3-CaTiO3 superlattices

We report on growth and ferroelectric (FE) properties of superlattices (SLs) composed of the FE BaTiO3 and the paraelectric (PE) CaTiO3. Previous theories have predicted that the polarization in (BaTiO3)n/(CaTiO3)n SLs increases as the sublayer thickness (n) increases when the same strain state is maintained. However, our BaTiO3/CaTiO3 SLs show a varying lattice-strain state and systematic reduction in polarization with increasing n while coherently-strained SLs with n=1, 2 show a FE polarization of ca. 8.5 uC/cm^2. We suggest that the strain coupling plays more important role in FE properties than the electrostatic interlayer coupling based on constant dielectric permittivities.

Optical spectroscopic investigation on the coupling of electronic and magnetic structure in multiferroic hexagonal RMnO3 (R = Gd, Tb, Dy, and Ho) thin films

We investigated the effects of temperature and magnetic field on the electronic structure of hexagonal RMnO3 (R = Gd, Tb, Dy, and Ho) thin films using optical spectroscopy. As the magnetic ordering of the system was disturbed, a systematic change in the electronic structure was commonly identified in this series. The optical absorption peak near 1.7 eV showed an unexpectedly large shift of more than 150 meV from 300 K to 15 K, accompanied by an anomaly of the shift at the Neel temperature. The magnetic field dependent measurement clearly revealed a sizable shift of the corresponding peak when a high magnetic field was applied. Our findings indicated strong coupling between the magnetic ordering and the electronic structure in the multiferroic hexagonal RMnO3 compounds.