Ultracold molecular gases are promising as an avenue to rich many-body physics, quantum chemistry, quantum information, and precision measurements. This richness, which flows from the complex internal structure of molecules, makes the creation of ult
racold molecular gases using traditional methods (laser plus evaporative cooling) a challenge, in particular due to the spontaneous decay of molecules into dark states. We propose a way to circumvent this key bottleneck using an all-optical method for decelerating molecules using stimulated absorption and emission with a single ultrafast laser. We further describe single-photon cooling of the decelerating molecules that exploits their high dark state pumping rates, turning the principal obstacle to molecular laser cooling into an advantage. Cooling and deceleration may be applied simultaneously and continuously to load molecules into a trap. We discuss implementation details including multi-level numerical simulations of strontium monohydride (SrH). These techniques are applicable to a large number of molecular species and atoms with the only requirement being an electric dipole transition that can be accessed with an ultrafast laser.
We present the results of theoretical and experimental studies of dispersively coupled (or membrane in the middle) optomechanical systems. We calculate the linear optical properties of a high finesse cavity containing a thin dielectric membrane. We f
ocus on the cavitys transmission, reflection, and finesse as a function of the membranes position along the cavity axis and as a function of its optical loss. We compare these calculations with measurements and find excellent agreement in cavities with empty-cavity finesses in the range 10^4 to 10^5. The imaginary part of the membranes index of refraction is found to be approximately 10^(-4). We calculate the laser cooling performance of this system, with a particular focus on the less-intuitive regime in which photons tunnel through the membrane on a time scale comparable to the membranes period of oscillation. Lastly, we present calculations of quantum non-demolition measurements of the membranes phonon number in the low signal-to-noise regime where the phonon lifetime is comparable to the QND readout time.
We have measured the optical and mechanical loss of commercial silicon nitride membranes. We find that 50 nm-thick, 1 mm^2 membranes have mechanical Q > 10^6 at 293 K, and Q > 10^7 at 300 mK, well above what has been observed in devices with comparab
le dimensions. The near-IR optical loss at 293 K is less than 2E-4. This combination of properties make these membranes attractive candidates for studying quantum effects in optomechanical systems.
Macroscopic mechanical objects and electromagnetic degrees of freedom couple to each other via radiation pressure. Optomechanical systems with sufficiently strong coupling are predicted to exhibit quantum effects and are a topic of considerable inter
est. Devices reaching this regime would offer new types of control of the quantum state of both light and matter and would provide a new arena in which to explore the boundary between quantum and classical physics. Experiments to date have achieved sufficient optomechanical coupling to laser-cool mechanical devices but have not yet reached the quantum regime. The outstanding technical challenge in this field is integrating sensitive micromechanical elements (which must be small, light, and flexible) into high finesse cavities (which are typically much more rigid and massive) without compromising the mechanical or optical properties of either. A second, and more fundamental, challenge is to read out the mechanical elements quantum state: displacement measurements (no matter how sensitive) cannot determine the energy eigenstate of an oscillator, and measurements which couple to quantities other than displacement have been difficult to realize. Here we present a novel optomechanical system which seems to resolve both these challenges. We demonstrate a cavity which is detuned by the motion of a thin dielectric membrane placed between two macroscopic, rigid, high-finesse mirrors. This approach segregates optical and mechanical functionality to physically distinct structures and avoids compromising either. It also allows for direct measurement of the square of the membranes displacement, and thus in principle the membranes energy eigenstate. We estimate it should be practical to use this scheme to observe quantum jumps of a mechanical system.
