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Frustrated magnets can exhibit many novel forms of order when exposed to high magnetic fields, however, much less is known about materials where frustration occurs in the presence of itinerant electrons. Here we report thermodynamic and transport mea surements on micron-sized single crystals of the triangular-lattice metallic antiferromagnet 2H-AgNiO2, in magnetic fields of up to 90 T and temperatures down to 0.35 K. We observe a cascade of magnetic phase transitions at 13.5 20, 28 and 39T in fields applied along the easy axis, and we combine magnetic torque, specific heat and transport data to construct the field-temperature phase diagram. The results are discussed in the context of a frustrated easy-axis Heisenberg model for the localized moments where intermediate applied magnetic fields are predicted to stabilize a magnetic supersolid phase. Deviations in the measured phase diagram from this model predictions are attributed to the role played by the itinerant electrons.
In the quasi-one-dimensional cuprate PrBa$_2$Cu$_4$O$_8$, the Pr cations order antiferromagnetically at 17 K in zero field. Through a combination of magnetic susceptibility, torque magnetometry, specific heat and interchain transport measurements, th e anisotropic temperature-magnetic field phase diagram associated with this ordering has been mapped out. A low-temperature spin-flop transition in the Pr sub-lattice is found to occur at the same magnetic field strength and orientation as a dimensional crossover in the ground state of the metallic CuO chains. This coincidence suggests that the spin reorientation is driven by a change in the anisotropic Rudermann-Kittel-Kasuya-Yosida (RKKY) interaction induced by a corresponding change in effective dimensionality of the conduction electrons.
We report the electronic and magnetic behaviour of the frustrated triangular metallic antiferromagnet 2H-AgNiO2 in high magnetic fields (54 T) using thermodynamic and transport measurements. Here localized d electrons are arranged on an antiferromagn etic triangular lattice nested inside a honeycomb lattice with itinerant d electrons. When the magnetic field is along the easy axis we observe a cascade of field-induced transitions, attributed to the competition between easy-axis anisotropy, geometrical frustration and coupling of the localized and itinerant system. The quantum oscillations data suggest that the Fermi surface is reconstructed by the magnetic order but in high fields magnetic breakdown orbits are possible. The itinerant electrons are extremely sensitive to scattering by spin fluctuations and a significant mass enhancement (~ 3) is found.
We review recent experimental measurements of the Fermi surface of the iron-pnictide superconductor LaFePO using quantum oscillation techniques. These studies show that the Fermi surface topology is close to that predicted by first principles density functional theory calculations, consisting of quasi-two-dimensional electron-like and hole-like sheets. The total volume of the two hole sheets is almost equal to that of the two electron sheets, and the hole and electron Fermi surface sheets are close to a nesting condition. No evidence for the predicted three dimensional pocket arising from the Fe $d_{z^2}$ band is found. Measurements of the effective mass suggest a renormalisation of around two, close to the value for the overall band renormalisation found in recent angle resolved photoemission measurements.
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