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Register a new userChemical modelling of dust-gas chemistry within AGB outflows -- II. Effect of the dust-grain size distribution
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AGB stars are, together with supernovae, the main contributors of stellar dust to the interstellar medium (ISM). Dust grains formed by AGB stars are thought to be large. However, as dust nucleation and growth within their outflows are still not understood, the dust-grain size distribution (GSD) is unknown. This is an important uncertainty regarding our knowledge of the chemical and physical history of interstellar dust, as AGB dust forms $sim$ 70% of the starting point of its evolution. We expand on our chemical kinetics model, which uniquely includes a comprehensive dust-gas chemistry. The GSD is now allowed to deviate from the commonly assumed canonical Mathis et al. (1977) distribution. We find that the specific GSD can significantly influence the dust-gas chemistry within the outflow. Our results show that the level of depletion of gas-phase species depends on the average grain surface area of the GSD. Gas-phase abundance profiles and their possible depletions can be retrieved from observations of molecular emission lines when using a range of transitions. Due to degeneracies within the prescription of GSD, specific parameters cannot be retrieved, only (a lower limit to) the average grain surface area. Nonetheless, this can discriminate between dust composed of predominantly large or small grains. We show that when combined with other observables such as the spectral energy distribution and polarised light, depletion levels from molecular gas-phase abundance profiles can constrain the elusive GSD of the dust delivered to the ISM by AGB outflows.
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Chemical modelling of AGB outflows is typically focused on either non-thermodynamic equilibrium chemistry in the inner region or photon-driven chemistry in the outer region. We include, for the first time, a comprehensive dust-gas chemistry in our AGB outflow chemical kinetics model, including both dust-gas interactions and grain-surface chemistry. The dust is assumed to have formed in the inner region, and follows an interstellar-like dust-size distribution. Using radiative transfer modelling, we obtain dust temperature profiles for different dust types in an O-rich and a C-rich outflow. We calculate a grid of models, sampling different outflow densities, drift velocities between the dust and gas, and dust types. Dust-gas chemistry can significantly affect the gas-phase composition, depleting parent and daughter species and increasing the abundance of certain daughter species via grain-surface formation followed by desorption/sputtering. Its influence depends on four factors: outflow density, dust temperature, initial composition, and drift velocity. The largest effects are for higher density outflows with cold dust and O-rich parent species, as these species generally have a larger binding energy. At drift velocities larger than $sim 10$ km s$^{-1}$, ice mantles undergo sputtering; however, they are not fully destroyed. Models with dust-gas chemistry can better reproduce the observed depletion of species in O-rich outflows. When including colder dust in the C-rich outflows and adjusting the binding energy of CS, the depletion in C-rich outflows is also better reproduced. To best interpret high-resolution molecular line observations from AGB outflows, dust-gas interactions are needed in chemical kinetics models.
To explain the properties of dust in the interstellar medium (ISM), the presence of a refractory organic mantle is necessary. The outflows of AGB stars are among the main contributors of stellar dust to the ISM. We present the first study of the refractory organic contribution of AGB stars to the ISM. Based on laboratory experiments, we included a new reaction in our extended chemical kinetics model: the photoprocessing of volatile complex ices into inert refractory organic material. The refractory organic feedback of AGB outflows to the ISM is estimated using observationally motivated parent species and grids of models of C-rich and O-rich outflows. Refractory organic material is mainly inherited from the gas phase through accretion onto the dust and subsequent photoprocessing. Grain-surface chemistry, initiated by photodissociation of ices, produces only a minor part and takes place in a sub-monolayer regime in almost all outflows. The formation of refractory organic material increases with outflow density and depends on the initial gas-phase composition. While O-rich dust is negligibly covered by refractory organics, C-rich dust has an average coverage of $3-9%$, but can be as high as $8-22%$. Although C-rich dust does not enter the ISM bare, its average coverage is too low to influence its evolution in the ISM or significantly contribute to the coverage of interstellar dust. This study opens up questions on the coverage of other dust-producing environments. It highlights the need for an improved understanding of dust formation and for models specific to density structures within the outflow.
It has recently been shown that turbulence in the interstellar medium (ISM) can significantly accelerate the growth of dust grains by accretion of molecules, but the turbulent gas-density distribution also plays a crucial role in shaping the grain-size distribution. The growth velocity, i.e., the rate of change of the mean grain radius, is proportional to the local gas density if the growth species (molecules) are well-mixed in the gas. As a consequence, grain growth happens at vastly different rates in different locations, since the gas-density distribution of the ISM shows a considerable variance. Here, it is shown that grain-size distribution (GSD) rapidly becomes a reflection of the gas-density distribution, irrespective of the shape of the initial GSD. This result is obtained by modelling ISM turbulence as a Markov process, which in the special case of an Ornstein-Uhlenbeck process leads to a lognormal gas-density distribution, consistent with numerical simulations of isothermal compressible turbulence. This yields an approximately lognormal GSD; the sizes of dust grains in cold ISM clouds may thus not follow the commonly adopted power-law GSD with index -3.5, but corroborates the use of a log-nomral GSD for large grains, suggested by several studies. It is also concluded that the very wide range of gas densities obtained in the high Mach-number turbulence of molecular clouds must allow formation of a tail of very large grains reaching radii of several microns.
We present a detailed analysis of the radial distribution of dust properties in the SINGS sample, performed on a set of UV, IR and HI surface brightness profiles, combined with published molecular gas profiles and metallicity gradients. The internal extinction, derived from the TIR-to-FUV luminosity ratio, decreases with radius, and is larger in Sb-Sbc galaxies. The TIR-to-FUV ratio correlates with the UV spectral slope beta, following a sequence shifted to redder UV colors with respect to that of starbursts. The star formation history (SFH) is identified as the main driver of this departure. We have also derived radial profiles of the total dust mass surface density, the fraction of the dust mass contributed by PAHs, the fraction of the dust mass heated by very intense starlight and the intensity of the radiation field heating the grains. The dust profiles are exponential, their radial scale-length being constant from Sb to Sd galaxies (only ~10% larger than the stellar scale-length). Many S0/a-Sab galaxies have central depressions in their dust radial distributions. The PAH abundance increases with metallicity for 12+log(O/H)<9, and at larger metallicities the trend flattens and even reverses, with the SFH being a plausible underlying driver for this behavior. The dust-to-gas ratio is also well correlated with metallicity and therefore decreases with galactocentric radius.
We study the evolution of extremely metal-poor AGB stars, with metallicities down to [Fe/H]=-5, to understand the main evolutionary properties, the efficiency of the processes able to alter their surface chemical composition and to determine the gas and dust yields. We calculate two sets of evolutionary sequences of stars in the 1-7.5Msun mass range, evolved from the pre-main sequence to the end of the AGB phase. To explore the extremely metal-poor chemistries we adopted the metallicities Z=3x10^{-5} and Z=3x10^{-7} which correspond, respectively to [Fe/H]=-3 and [Fe/H]=-5. The results from stellar evolution modelling are used to calculate the yields of the individual chemical species. We also modelled dust formation in the wind, to determine the dust produced by these objects. The evolution of AGB stars in the extremely metal-poor domain explored here proves tremendously sensitive to the initial mass of the star. M<2Msun stars experience several third dredge-up events, which favour the gradual surface enrichment of C12 and the formation of significant quantities of carbonaceous dust, of the order of 0.01Msun. The C13 and nitrogen yiel are found to be significantly smaller than in previous explorations of low-mass, metal-poor AGB stars, owing to the weaker proton ingestion episodes experienced during the initial AGB phases. M>5Msun stars experience hot bottom burning and their surface chemistry reflects the equilibria of a very advanced proton-capture nucleosynthesis; little dust production takes place in their wind. Intermediate mass stars experience both third dredge-up and hot bottom burning: they prove efficient producers of nitrogen, which is formed by proton captures on C12 nuclei of primary origin dredged-up from the internal regions.
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