Ambient magnetic field, if trapped in the penetration depth, leads to the residual resistance and therefore sets the limit for the achievable quality factors in superconducting niobium resonators for particle accelerators. Here we show that a complete expulsion of the magnetic flux can be performed and leads to: 1) record quality factors $Q > 2times10^{11}$ up to accelerating gradient of 22 MV/m; 2) $Qsim3times10^{10}$ at 2 K and 16 MV/m in up to 190 mG magnetic fields. This is achieved by large thermal gradients at the normal/superconducting phase front during the cooldown. Our findings open up a way to ultra-high quality factors at low temperatures and show an alternative to the sophisticated magnetic shielding implemented in modern superconducting accelerators.
In this paper we present the discovery of a new surface treatment applied to superconducting radio frequency (SRF) niobium cavities, leading to unprecedented accelerating fields of 49 MV/m in TESLA-shaped cavities, in continuous wave (CW); the corresponding peak magnetic fields are the highest ever measured in CW, about 210 mT. For TESLA-shape cavities the maximum quench field ever achieved was ~45 MV/m - reached very rarely- with most typical values being below 40 MV/m. These values are reached for niobium surfaces treated with electropolishing followed by the so called mild bake, a 120C vacuum bake (for 48 hours for fine grain and 24 hours for large grain surfaces). We discover that the addition during the mild bake of a step at 75C for few hours, before the 120C, increases systematically the quench fields up to unprecedented values of 49 MV/m. The significance of the result lays not only in the relative improvement, but in the proof that niobium surfaces can sustain and exceed CW radio frequency magnetic fields much larger than Hc1, pointing to an extrinsic nature of the current field limitations, and therefore to the potential to reach accelerating fields well beyond the current state of the art.
We report the finding of new surface treatments that permit to manipulate the niobium resonator nitrogen content in the first few nanometers in a controlled way, and the resonator fundamental Mattis-Bardeen surface resistance and residual resistance accordingly. In particular, we find surface infusion conditions that systematically a) increase the quality factor of these 1.3 GHz superconducting radio frequency (SRF) bulk niobium resonators, up to very high gradients; b) increase the achievable accelerating gradient of the cavity compared to its own baseline with state-of-the-art surface processing. Cavities subject to the new surface process have larger than two times the state of the art Q at 2K for accelerating fields > 35 MV/m. Moreover, very high accelerating gradients ~ 45 MV/m are repeatedly reached, which correspond to peak magnetic surface fields of 190 mT, among the highest measured for bulk niobium cavities. These findings open the opportunity to tailor the surface impurity content distribution to maximize performance in Q and gradients, and have therefore very important implications on future performance and cost of SRF based accelerators. They also help deepen the understanding of the physics of the RF niobium cavity surface.
A systematic study is presented on the superconductivity (sc) parameters of the ultrapure niobium used for the fabrication of the nine-cell 1.3 GHz cavities for the linear collider project TESLA. Cylindrical Nb samples have been subjected to the same surface treatments that are applied to the TESLA cavities: buffered chemical polishing (BCP), electrolytic polishing (EP), low-temperature bakeout (LTB). The magnetization curves and the complex magnetic susceptibility have been measured over a wide range of temperatures and dc magnetic fields, and also for di erent frequencies of the applied ac magnetic field. The bulk superconductivity parameters such as the critical temperature Tc = 9.26 K and the upper critical field Bc2(0) = 410 mT are found to be in good agreement with previous data. Evidence for surface superconductivity at fields above Bc2 is found in all samples. The critical surface field exceeds the Ginzburg-Landau field Bc3 = 1.695Bc2 by about 10% in BCP-treated samples and increases even further if EP or LTB are applied. From the field dependence of the susceptibility and a power-law analysis of the complex ac conductivity and resistivity the existence of two different phases of surface superconductivity can be established which resemble the Meissner and Abrikosov phases in the bulk: (1) coherent surface superconductivity, allowing sc shielding currents flowing around the entire cylindrical sample, for external fields B in the range between Bc2 and Bcohc3, and (2) incoherent surface superconductivity with disconnected sc domains between Bcohc3 and Bc3. The coherent critical surface field separating the two phases is found to be Bcoh c3 = 0.81Bc3 for all samples. The exponents in the power law analysis are different for BCP and EP samples, pointing to different surface topologies.
The vacuum arc is a well-known technique to produce coating with enhanced adhesion and film density. Many cathodic arc deposition systems are actually in use in industry and research. They all work under (high) vacuum conditions in which water vapor pressure is an important source of film contamination, especially in the pulsed arc mode of operation. Here we present a Cathodic Arc system working under Ultra High Vacuum conditions (UHVCA). UHVCA has been used to produce ultra-pure niobium films with excellent structural and electrical properties at a deposition temperature lower than 100oC. The UHVCA technique therefore opens new perspectives for all applications requiring ultra-pure films or, as in the case of Plasma Immersion Ion Implantation, ultra-pure plasmas.
Even when cooled through its transition temperature in the presence of an external magnetic field, a superconductor can expel nearly all external magnetic flux. This Letter presents an experimental study to identify the parameters that most strongly influence flux trapping in high purity niobium during cooldown. This is critical to the operation of superconducting radiofrequency cavities, in which trapped flux degrades the quality factor and therefore cryogenic efficiency. Flux expulsion was measured on a large survey of 1.3 GHz cavities prepared in various ways. It is shown that both spatial thermal gradient and high temperature treatment are critical to expelling external magnetic fields, while surface treatment has minimal effect. For the first time, it is shown that a cavity can be converted from poor expulsion behavior to strong expulsion behavior after furnace treatment, resulting in a substantial improvement in quality factor. Future plans are described to build on this result in order to optimize treatment for future cavities.
A. Romanenko
,A. Grassellino
,A. C. Crawford
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(2014)
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"Ultra-high quality factors in superconducting niobium cavities in ambient magnetic fields up to 190 mG"
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Alexander Romanenko
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