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Register a new userAn electrical probe for mechanical vibrations in suspended carbon nanotubes
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The transport properties of a suspended carbon nanotube probed by means of a STM tip are investigated. A microscopic theory of the coupling between electrons and mechanical vibrations is developed. It predicts a position-dependent coupling constant, sizeable only in the region where the vibron is located. This fact has profound consequences on the transport properties, which allow to extract information on the location and size of the vibrating portions of the nanotube.
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We have generated and detected the radial-breathing mode of coherent lattice vibrations in single-walled carbon nanotubes using ultrashort laser pulses. Because the band gap is a function of diameter, these diameter oscillations cause ultrafast band gap oscillations, modulating interband excitonic resonances at the phonon frequencies (3-9 THz). Excitation spectra show a large number of pronounced peaks, mapping out chirality distributions in great detail.
The electronic Raman scattering (ERS) features of single-walled carbon nanotubes (SWNTs) can reveal a wealth of information about their electronic structures, but have previously been thought to appear exclusively in metallic (M-) but not in semiconducting (S-) SWNTs. We report the experimental observation of the ERS features with an accuracy of 1 meV in suspended S-SWNTs, the processes of which are accomplished via the available high-energy electron-hole pairs. The ERS features can facilitate further systematic studies on the properties of SWNT, both metallic and semiconducting, with defined chirality.
We present a simple technique which uses a self-aligned oxide etch to suspend individual single-wall carbon nanotubes between metallic electrodes. This enables one to compare the properties of a particular nanotube before and after suspension, as well as to study transport in suspended tubes. As an example of the utility of the technique, we study quantum dots in suspended tubes, finding that their capacitances are reduced owing to the removal of the dielectric substrate.
We propose a framework for inducing strong optomechanical effects in a suspended carbon nanotube based on deformation potential exciton-phonon coupling. The excitons are confined using an inhomogeneous axial electric field which generates optically active quantum dots with a level spacing in the milli-electronvolt range and a characteristic size in the 10-nanometer range. A transverse field induces a tunable parametric coupling between the quantum dot and the flexural modes of the nanotube mediated by electron-phonon interactions. We derive the corresponding excitonic deformation potentials and show that this interaction enables efficient optical ground-state cooling of the fundamental mode and could allow us to realise the strong and ultra-strong coupling regimes of the Jaynes-Cummings and Rabi models.
Transport in suspended metallic single wall carbon nanotubes in the presence of strong electron-electron interaction is investigated. We consider a tube of finite length and discuss the effects of the coupling of the electrons to the deformation potential associated to the acoustic stretching and breathing modes. Treating the interacting electrons within the framework of the Luttinger liquid model, the low-energy spectrum of the coupled electron-phonon system is evaluated. The discreteness of the spectrum is reflected in the differential conductance which, as a function of the applied bias voltage, exhibits three distinct families of peaks. The height of the phonon-assisted peaks is very sensitive to the parameters. The phonon peaks are best observed when the system is close to the Wentzel-Bardeen singularity.
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