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Register a new userCoexistence of, and Competition between, Superconductivity and Charge-Stripe Order in La(1.6-x)Nd(0.4)Sr(x)CuO(4)
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Previously we have presented evidence for stripe order of holes and spins in La(1.6-x)Nd(0.4)Sr(x)CuO(4) with x=0.12. Here we show, via neutron diffraction measurements of magnetic scattering, that similar order occurs in crystals with x=0.15 and 0.20. Zero-field-cooled magnetization measurements show that all 3 compositions are also superconducting, with the superconducting transition temperature increasing as the low-temperature staggered magnetization decreases.
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We demonstrate that the integrated intensity of Cu-63 nuclear quadrupole resonance (NQR) in La(1.6-x)Nd(0.4)Sr(x)CuO(4) decreases dramatically below the charge-stripe ordering temperature T(charge). Comparison with neutron and X-ray scattering indica
tes that the wipeout fraction F(T) (i.e. the missing fraction of the integrated intensity of the NQR signal) represents the charge-stripe order parameter. The systematic study reveals bulk charge-stripe order throughout the superconducting region 0.07 <= x <= 0.25. As a function of the reduced temperature t = T/T(charge), the temperature dependence of F(t) is sharpest for the hole concentration x=1/8, indicating that x=1/8 is the optimum concentration for stripe formation.
The dynamics of the charge-order domains has been investigated in La$_{1.48}$Nd$_{0.4}$Sr$_{0.12}$CuO$_{4}$, a prototypical stripe-ordered cuprate, using pulsed current injection. We first identify the regime in which nonthermal effects dominate over simple Joule heating, and then demonstrate that, for small enough perturbation, pulsed current injection allows access to nonthermally-induced resistive metastable states. The results are consistent with pinning of the fluctuating charge order, with fluctuations being most pronounced at the charge-order onset temperature. The nonequilibrium effects are revealed only when the transition is approached from the charge-ordered phase. Our experiment establishes pulsed current injection as a viable and effective method for probing the charge-order dynamics in various other materials.
We report an angle-resolved photoemission study of the charge stripe ordered La$_{1.6-x}$Nd$_{0.4}$Sr$_x$CuO$_4$ system. A comparative and quantitative line shape analysis is presented as the system evolves from the overdoped regime into the charge ordered phase. On the overdoped side ($x=0.20$), a normal state anti-nodal spectral gap opens upon cooling below ~ 80 K. In this process spectral weight is preserved but redistributed to larger energies. A correlation between this spectral gap and electron scattering is found. A different lineshape is observed in the antinodal region of charge ordered Nd-LSCO $x=1/8$. Significant low-energy spectral weight appears to be lost. These observations are discussed in terms of spectral weight redistribution and gapping %of spectral weight originating from charge stripe ordering.
We demonstrate that one can measure the charge-stripe order parameter in the hole-doped CuO(2) planes of La(1.875)Ba(0.125)CuO(4), La(1.48)Nd(0.4)Sr(0.12)CuO(4) and La(1.68)Eu(0.2)Sr(0.12)CuO(4) utilizing the wipeout effects of Cu-63 NQR. Application of the same approach to La(2-x)Sr(x)CuO(4) reveals the presence of similar stripe order for the entire underdoped superconducting regime 1/16 < x < 1/8.
We report the observation of a bulk charge modulation in La$_{1.88}$Sr$_{0.12}$CuO$_4$ (LSCO) with a characteristic in-plane wave-vector of (0.236, $pm delta$), with $delta$=0.011 r.l.u. The transverse shift of the ordering wave-vector indicates the presence of rotated charge-stripe ordering, demonstrating that the charge ordering is not pinned to the Cu-O bond direction. On cooling through the superconducting transition, we find an abrupt change in the growth of the charge correlations and a suppression of the charge order parameter indicating competition between the two orderings. Orthorhombic LSCO thus helps bridge the apparent disparities between the behavior previously observed in the tetragonal 214 cuprates and the orthorhombic yttrium and bismuth-based cuprates and thus lends strong support to the idea that there is a common motif to charge order in all cuprate families.
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