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Register a new userFourier transform spectroscopy of d-wave quasiparticles in the presence of atomic scale pairing disorder
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The local density of states power spectrum of optimally doped Bi$_2$Sr$_2$CaCu$_2$O$_{8+x}$ (BSCCO) has been interpreted in terms of quasiparticle interference peaks corresponding to an octet of scattering wave vectors connecting k-points where the density of states is maximal. Until now, theoretical treatments have not been able to reproduce the experimentally observed weights and widths of these octet peaks; in particular, the predominance of the dispersing q$_1$ peak parallel to the Cu-O bond directions has remained a mystery. In addition, such theories predict background features which are not observed experimentally. Here, we show that most of the discrepancies can be resolved when a realistic model for the out-of-plane disorder in BSCCO is used. Weak extended potential scatterers, which are assumed to represent cation disorder, suppress large-momentum features and broaden the low-energy q$_7$-peaks, whereas scattering at order parameter variations, possibly caused by a dopant-modulated pair interaction around interstitial oxygens, strongly enhances the dispersing q$_1$-peaks.
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The recent discovery of superconductivity in NaSn$_2$As$_2$ with a van der Waals layered structure raises immediate questions on its pairing mechanism and underlying electronic structure. Here, we present measurements of the temperature-dependent magnetic penetration depth $lambda(T)$ in single crystals of NaSn$_2$As$_2$ down to $sim40$ mK. We find a very long penetration depth $lambda (0) = 960$ nm, which is strongly enhanced from the estimate of first-principles calculations. This enhancement comes from a short mean free path $ell approx 1.7$ nm, indicating atomic scale disorder possibly associated with the valence-skipping states of Sn. The temperature dependence of superfluid density is fully consistent with the conventional fully gapped s-wave state in the dirty limit. These results suggest that NaSn$_2$As$_2$ is an ideal material to study quantum phase fluctuations in strongly disordered superconductors with its controllable dimensionality.
Rapid proliferation of hyperspectral imaging in scanning probe microscopies creates unique opportunities to systematically capture and categorize higher dimensional datasets, toward new insights into electronic, mechanical and chemical properties of materials with nano- and atomic-scale resolution. Here we demonstrate similarity learning for tunneling spectroscopy acquired on superconducting material (FeSe) with sparse density of imperfections (Fe vacancies). Popular methods for unsupervised learning and discrete representation of the data in terms of clusters of characteristic behaviors were found to produce inconsistencies with respect to capturing the location and tunneling characteristics of the vacancy sites. To this end, we applied a more general, non-linear similarity learning. This approach was found to outperform several widely used methods for dimensionality reduction and produce a clear differentiation of the type of tunneling spectra. In particular, significant spectral weight transfer likely associated with the electronic reconstruction by the vacancy sites, is systematically captured, as is the spatial extent of the vacancy region. Given that a great variety of electronic materials will exhibit similarly smooth variation of the spectral responses due to random or engineered inhomogeneities in their structure, we believe our approach will be useful for systematic analysis of hyperspectral imaging with minimal prior knowledge, as well as prospective comparison of experimental measurements to theoretical calculations with explicit consideration of disorder.
We discuss a scenario for interface-induced superconductivity involving pairing by dipolar excitations proximate to a two-dimensional electron system controlled by a transverse electric field. If the interface consists of transition metal oxide materials, the repulsive on-site Coulomb interaction is typically strong and a superconducting state is formed via exchange of non-local dipolar excitations in the d-wave channel. Perspectives to enhance the superconducting transition temperature are discussed.
In the theoretical analyses of impurity effects in superconductors the assumption is usually made that all quantities, except for the Green functions, are slowly varying functions of energy. When this so-called Fermi Surface Restricted Approximation is combined with the assumption that impurities can be represented by delta-function potentials of arbitrary strength, many reasonable looking results can be obtained. The agreement with experiments is not entirely satisfactory and one reason for this might be the assumption that the impurity potential has zero range. The generalization to finite range potentials appears to be straightforward, independent of the strength of the potential. However, the selfenergy resulting from scattering off finite range impurities of infinite strength such as hard spheres, diverges in this approximation at frequencies much larger than the gap amplitude! To track down the source of this unacceptable result we consider the normal state. The elementary results for scattering off a hard sphere, including the result that even an infinitely strong delta-function potential does not lead to scattering at all in systems of two and more dimensions, are recovered only when the energy dependencies of all quantities involved are properly taken into account. To obtain resonant scattering, believed to be important for the creation of mid-gap states, the range of the potential is almost as important as its strength.
Extensive research into high temperature superconducting cuprates is now focused upon identifying the relationship between the classic pseudogap phenomenon$^{1,2}$ and the more recently investigated density wave state$^{3-13}$. This state always exhibits wave vector $Q$ parallel to the planar Cu-O-Cu bonds$^{4-13}$ along with a predominantly $d$-symmetry form factor$^{14-17}$ (dFF-DW). Finding its microscopic mechanism has now become a key objective$^{18-30}$ of this field. To accomplish this, one must identify the momentum-space ($k$-space) states contributing to the dFF-DW spectral weight, determine their particle-hole phase relationship about the Fermi energy, establish whether they exhibit a characteristic energy gap, and understand the evolution of all these phenomena throughout the phase diagram. Here we use energy-resolved sublattice visualization$^{14}$ of electronic structure and show that the characteristic energy of the dFF-DW modulations is actually the pseudogap energy $Delta_{1}$. Moreover, we demonstrate that the dFF-DW modulations at $E=-Delta_{1}$ (filled states) occur with relative phase $pi$ compared to those at $E=Delta_{1}$ (empty states). Finally, we show that the dFF-DW $Q$ corresponds directly to scattering between the hot frontier regions of $k$-space beyond which Bogoliubov quasiparticles cease to exist$^{31,32,33}$. These data demonstrate that the dFF-DW state is consistent with particle-hole interactions focused at the pseudogap energy scale and between the four pairs of hot frontier regions in $k$-space where the pseudogap opens.
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