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Register a new userVery high upper critical fields in MgB2 produced by selective tuning of impurity scattering
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We report a significant enhancement of the upper critical field $H_{c2}$ of different $MgB_2$ samples alloyed with nonmagnetic impurities. By studying films and bulk polycrystals with different resistivities $rho$, we show a clear trend of $H_{c2}$ increase as $rho$ increases. One particular high resistivity film had zero-temperature $H_{c2}(0)$ well above the $H_{c2}$ values of competing non-cuprate superconductors such as $Nb_3Sn$ and Nb-Ti. Our high-field transport measurements give record values $H_{c2}^perp (0) approx 34T$ and $H_{c2}|(0) approx 49 T$ for high resistivity films and $H_{c2}(0)approx 29 T$ for untextured bulk polycrystals. The highest $H_{c2}$ film also exhibits a significant upward curvature of $H_{c2}(T)$, and temperature dependence of the anisotropy parameter $gamma(T) = H_{c2}|/ H_{c2}^perp$ opposite to that of single crystals: $gamma(T)$ decreases as the temperature decreases, from $gamma(T_c) approx 2$ to $gamma(0) approx 1.5$. This remarkable $H_{c2}$ enhancement and its anomalous temperature dependence are a consequence of the two-gap superconductivity in $MgB_2$, which offers special opportunities for further $H_{c2}$ increase by tuning of the impurity scattering by selective alloying on Mg and B sites. Our experimental results can be explained by a theory of two-gap superconductivity in the dirty limit. The very high values of $H_{c2}(T)$ observed suggest that $MgB_2$ can be made into a versatile, competitive high-field superconductor.
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Critical fields of four MgB2 thin films with a normal state resistivity ranging from 5 to 50 mWcm and Tc from 29.5 to 38.8 K were measured up to 28 T. Hc2(T) curves present a linear behavior towards low temperatures. Very high critical field values have been found, up to 24 T along the c-axis and 57 T in the basal plane not depending on the normal state resistivity values. In this paper, critical fields will be analyzed taking into account the multiband nature of MgB2; we will show that resistivity and upper critical fields can be ascribed to different scattering mechanisms.
In this paper, we analyze the upper critical field of four MgB2 thin films, with different resistivity (between 5 to 50 mWcm) and critical temperature (between 29.5 to 38.8 K), measured up to 28 Tesla. In the perpendicular direction the critical fields vary from 13 to 24 T and we can estimate 42-57 T range in other direction. We observe linear temperature dependence even at low temperatures without saturation, in contrast to BCS theory. Considering the multiband nature of the superconductivity in MgB2, we conclude that two different scattering mechanisms influence separately resistivity and critical field. In this framework, resistivity values have been calculated from Hc2(T) curves and compared with the measured ones.
Nanoscale defects in superconductors play a dominant role in enhancing superconducting properties through electron scattering, modulation of coherence length, and correlation with quantized magnetic flux. For iron-based superconductors (IBSCs) that are expected to be employed in high-field magnetic applications, a fundamental question is whether such defects develop an upper critical field (Hc2) similar to that of conventional BCS-type superconductors. Herein, we report the first demonstration of a significantly improved Hc2 in a 122-phase IBSC by introducing defects through high-energy milling. Co-doped Ba122 polycrystalline bulk samples (Ba(Fe,Co)2As2) were prepared by sintering powder which was partially mechanically alloyed through high-energy milling. A remarkable increase in full-width at half maximum of X-ray powder diffraction peaks, anomalous shrinkage in the a-axis, and elongation in the c-axis were observed. When lattice defects are introduced into the grains, semiconductor behavior of the electric resistivity at low temperature (T < 100 K), slight decrease in transition temperature (Tc), upturn of Hc2(T) near Tc, and a large increase in Hc2(T) slope were observed. The slope of Hc2(T) increased approximately by 50%, i.e., from 4 to 6 T/K, and exceeded that of single crystals and thin films. Defect engineering through high-energy milling is expected to facilitate new methods for the designing and tuning of Hc2 in 122-phase IBSCs.
Here we report the comparison of the upper critical fields of different superconductors being calculated by two different theories i.e., Werthamer Helfand Hohenburg (WHH) and Ginzberg Landau (GL). All the samples are synthesized through previously known solid state reaction route. Phase purity is determined from the Rietveld refinement of powder X-Ray diffraction (XRD) data. High field (up to 14Tesla) magneto transport r{ho}(T)H of different superconductors is studied to estimate their upper critical field (Hc2). The present inter comparison covers from Cuprates (YBa2Cu3O7) - Borides (MgB2) - Fe pnictides (NdFeAsO0.8F0.2) and chalcogenides (FeSe0.5Te0.5) to robust Nb2PdS5. The upper critical fields [Hc2(T)] at zero temperature are calculated by extrapolating the data using GL and WHH equations.
We present the resistively-determined upper critical field H^{rho}_{c2}(T) and the irreversibility lines H^{rho}_{irr}(T) of various high-T_c cuprates, deduced from measurements in 61-T pulsed magnetic fields applied parallel to the c-axis. The SHAPE of both H^{rho}_{c2}(T) and H^{rho}_{irr}(T) depends monotonically on the anisotropy of the material and none of the samples show saturation of H^{rho}(T) at low temperatures. The anomalous positive curvature, d^2 H^{rho}/dT^2 > 0, is the strongest in materials with the largest normal-state anisotropy, regardless of whether anisotropy is varied by changing the carrier concentration or by comparing a variety of optimally-doped compounds.
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