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Register a new userSeparation quality of a geometric ratchet
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We consider an experimentally relevant model of a geometric ratchet in which particles undergo drift and diffusive motion in a two-dimensional periodic array of obstacles, and which is used for the continuous separation of particles subject to different forces. The macroscopic drift velocity and diffusion tensor are calculated by a Monte-Carlo simulation and by a master-equation approach, using the correponding microscopic quantities and the shape of the obstacles as input. We define a measure of separation quality and investigate its dependence on the applied force and the shape of the obstacles.
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Liquid-liquid phase separation of liquids exhibiting interconversion between alternative states has been proposed as an underlying mechanism for fluid polyamorphism, and may be of relevance to protein function and intracellular organization. However, molecular-level insight into the interplay between competing forces that can drive or restrict phase separation in interconverting fluids remains elusive. Here, we utilize an off-lattice model of enantiomers with tunable chiral interconversion and interaction properties to elucidate the physics underlying the stabilization and tunability of phase separation in fluids with interconverting states. We show that introducing an imbalance in the intermolecular forces between two enantiomers results in nonequilibrium, arrested phase separation into microdomains. We also find that in the equilibrium case, when all interaction forces are conservative, the growth of the phase domain is restricted only by system size. In this case, we observe phase amplification, in which one of the two alternative phases grows at the expense of the other. These findings provide novel insights on how the interplay between dynamics and thermodynamics defines the equilibrium and steady-state morphologies of phase transitions in fluids with interconverting molecular or supramolecular states.
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As a result of nonequilibrium forces, purely repulsive self-propelled particles undergo macrophase separation between a dense and a dilute phase. We present a thorough study of the ordering kinetics of such motility-induced phase separation (MIPS) in active Brownian particles in two dimensions, and we show that it is generically accompanied by microphase separation. The growth of the dense phase follows a law akin to the one of liquid-gas phase separation. However, it is made of a mosaic of hexatic microdomains whose size does not coarsen indefinitely, leaving behind a network of extended topological defects from which microscopic dilute bubbles arise. The characteristic length of these finite-size structures increases with activity, independently of the choice of initial conditions.
We investigate experimentally a two-dimensional rocking ratchet for cold atoms, realized by using a driven three-beam dissipative optical lattice. AC forces are applied in perpendicular directions by phase-modulating two of the lattice beams. As predicted by the general theory [S. Denisov et al., Phys. Rev. Lett. 100, 224102 (2008)], we observe a rectification phenomenon unique to high-dimensional rocking ratchets, as determined by two single-harmonic drivings applied in orthogonal directions. Also, by applying two bi-harmonic forces in perpendicular directions, we demonstrate the possibility of generating a current in an arbitrary direction within the optical lattice plane.
Motivated by recent work [D. Cubero et al., Phys. Rev. E 82, 041116 (2010)], we examine the mechanisms which determine current reversals in rocking ratchets as observed by varying the frequency of the drive. We found that a class of these current reversals in the frequency domain are precisely determined by dissipation-induced symmetry breaking. Our experimental and theoretical work thus extends and generalizes the previously identified relationship between dynamical and symmetry-breaking mechanisms in the generation of current reversals.
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