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Register a new userGenerating optical supercontinuum and frequency comb in tenuous plasmas
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There are several mechanisms by which the frequency spectrum of a laser broadens when it propagates at near-relativistic-intensity in tenuous plasma. Focusing on one dimensional effects, we identify two strong optical nonlinearities, namely, four-wave mixing (FWM) and forward Raman scattering (FRS), for creating octave-wide spectra. FWM dominates the interaction when the laser pulse is short and intense; Its combination with phase modulation produces a symmetrically broadened supercontinuum. FRS dominates when the laser pulse is long and relatively weak; It broadens the laser spectrum mainly towards lower frequencies and produces a frequency comb. The creation of the supercontinuum and frequency combs only frequency modulates, but does not compress, the laser pulse.
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Laser frequency can be upconverted in a plasma undergoing ionization. For finite ionization rates, the laser pulse energy is partitioned into a pair of counter-propagating waves and static transverse currents. The wave amplitudes are determined by the ionization rates and the input pulse duration. The strongest output waves can be obtained when the plasma is fully ionized in a time that is shorter than the pulse duration. The static transverse current can induce a static magnetic field with instant ionization, but it dissipates as heat if the ionization time is longer than a few laser periods. This picture comports with experimental data, providing a description of both laser frequency upconverters as well as other laser-plasma interaction with evolving plasma densities.
We have built a frequency chain which enables to measure the absolute frequency of a laser emitting in the 28-31 THz frequency range and stabilized onto a molecular absorption line. The set-up uses an optical frequency comb and an ultrastable 1.55 $mu$m frequency reference signal, transferred from LNE-SYRTE to LPL through an optical link. We are now progressing towards the stabilization of the mid-IR laser via the frequency comb and the extension of this technique to quantum cascade lasers. Such a development is very challenging for ultrahigh resolution molecular spectroscopy and fundamental tests of physics with molecules.
Full phase control of THz emitting quantum cascade laser (QCL) combs has recently been demonstrated, opening new perspectives for even the most demanding applications. In this framework, simplifying the set-ups for control of these devices will help to accelerate their spreading in many fields. We report a new way to control the emission frequencies of a THz QCL comb by small optical frequency tuning (SOFT), using a very simple experimental setup, exploiting the incoherent emission of an ordinary white light emitting diode. The slightly perturbative regime accessible in these condition allows tweaking the complex refractive index of the semiconductor without destabilizing the broadband laser gain. The SOFT actuator is characterized and compared to another actuator, the QCL driving current. The suitability of this additional degree of freedom for frequency and phase stabilization of a THz QCL comb is shown and perspectives are discussed.
Optical frequency combs (OFCs), consisting of a set of phase locked equally spaced laser frequency lines, have enabled a great leap in precision spectroscopy and metrology since seminal works of Hansch et al. . Nowadays, OFCs are cornerstones of a wealth of further applications ranging from chemistry and biology to astrophysics and including molecular fingerprinting and LIDARs among others. Driven passive optical resonators constitute the ideal platform for OFCs generation in terms of compactness and low energy footprint. We propose here a new technique for generation of OFCs with tuneable repetition rate in externally driven optical resonators based on the gain-through-filtering process, a simple and elegant method, due to an asymmetric spectral filtering on one side of the pump wave. We demonstrate a proof-of-concept experimental result in a fibre resonator, pioneering a new technique that does not require specific engineering of the resonator dispersion to generate frequency agile OFCs.
We study the properties of a soliton crystal, an bound state of several optical pulses that propagate with a fixed temporal separation through the optical fibres of the proposed approach for generation of optical frequency combs (OFC) for astronomical spectrograph calibration. This approach - also being suitable for subpicosecond pulse generation for other applications - consists of a conventional single-mode fibre and a suitably pumped Erbium-doped fibre. Two continuous-wave lasers are used as light source. The soliton crystal arises out of the initial deeply modulated laser field at low input powers; for higher input powers, it dissolves into free solitons. We study the soliton crystal build-up in the first fibre stage with respect to different fibre parameters (group-velocity dispersion, nonlinearity, and optical losses) and to the light source characteristics (laser frequency separation and intensity difference). We show that the soliton crystal can be described by two quantities, its fundamental frequency and the laser power-threshold at which the crystal dissolves into free solitons. The soliton crystal exhibits features of a linear and nonlinear optical pattern at the same time and is insensitive to the initial laser power fluctuations. We perform our studies using the numerical technique called Soliton Radiation Beat Analysis.
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