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Controlling and Phase-Locking a THz Quantum Cascade Laser Frequency Comb by Small Optical Frequency Tuning

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 Added by Luigi Consolino
 Publication date 2020
  fields Physics
and research's language is English




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Full phase control of THz emitting quantum cascade laser (QCL) combs has recently been demonstrated, opening new perspectives for even the most demanding applications. In this framework, simplifying the set-ups for control of these devices will help to accelerate their spreading in many fields. We report a new way to control the emission frequencies of a THz QCL comb by small optical frequency tuning (SOFT), using a very simple experimental setup, exploiting the incoherent emission of an ordinary white light emitting diode. The slightly perturbative regime accessible in these condition allows tweaking the complex refractive index of the semiconductor without destabilizing the broadband laser gain. The SOFT actuator is characterized and compared to another actuator, the QCL driving current. The suitability of this additional degree of freedom for frequency and phase stabilization of a THz QCL comb is shown and perspectives are discussed.



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Optical frequency comb synthesizers (FCs) [1] are laser sources covering a broad spectral range with a number of discrete, equally spaced and highly coherent frequency components, fully controlled through only two parameters: the frequency separation between adjacent modes and the carrier offset frequency. Providing a phase-coherent link between the optical and the microwave/radio-frequency regions [2], FCs have become groundbreaking tools for precision measurements[3,4]. Despite these inherent advantages, developing miniaturized comb sources across the whole infrared (IR), with an independent and simultaneous control of the two comb degrees of freedom at a metrological level, has not been possible, so far. Recently, promising results have been obtained with compact sources, namely diode-laser-pumped microresonators [5,6] and quantum cascade lasers (QCL-combs) [7,8]. While both these sources rely on four-wave mixing (FWM) to generate comb frequency patterns, QCL-combs benefit from a mm-scale miniaturized footprint, combined with an ad-hoc tailoring of the spectral emission in the 3-250 {mu}m range, by quantum engineering [9]. Here, we demonstrate full stabilization and control of the two key parameters of a QCL-comb against the primary frequency standard. Our technique, here applied to a far-IR emitter and open ended to other spectral windows, enables Hz-level narrowing of the individual comb modes, and metrological-grade tuning of their individual frequencies, which are simultaneously measured with an accuracy of 2x10^-12, limited by the frequency reference used. These fully-controlled, frequency-scalable, ultra-compact comb emitters promise to pervade an increasing number of mid- and far-IR applications, including quantum technologies, due to the quantum nature of the gain media [10].
117 - Hanzhong Wu , Jun Ke , Panpan Wang 2021
In this work, we describe an updated version of single arm locking, and the noise amplification due to the nulls can be flexibly restricted with the help of optical frequency comb. We show that, the laser phase noise can be divided by a specific factor with optical frequency comb as the bridge. The analytical results indicate that, the peaks in the science band have been greatly reduced. The performance of the noise suppression shows that the total noise after arm locking can well satisfy the requirement of time delay interferometry, even with the free-running laser source. We also estimate the frequency pulling characteristics of the updated single arm locking, and the results suggest that the pulling rate can be tolerated, without the risk of mode hopping. Arm locking will be a valuable solution for the noise reduction in the space-borne GW detectors. We demonstrate that, with the precise control of the returned laser phase noise, the noise amplification in the science band can be efficiently suppressed based on the updated single arm locking. Not only our method allows the suppression of the peaks, the high gain, low pulling rate, it can also serve for full year, without the potential risk of locking failure due to the arm length mismatch. We finally discuss the unified demonstration of the updated single arm locking, where both the local and the returned laser phase noises can be tuned to generate the expected arm-locking sensor actually. Our work could provide a powerful method for the arm locking in the future space-borne GW detectors.
We present homogeneous quantum cascade lasers (QCLs) emitting around 3 THz which display bandwidths up to 950 GHz with a single stable beatnote. Devices are spontaneously operating in a harmonic comb state, and when in a dense mode regime they can be injection locked at the cavity roundtrip frequency with very small RF powers down to -55 dBm. When operated in the electrically unstable region of negative differential resistance, the device displays ultra-broadband operation exceeding 1.83 THz ($Delta f/f=50%$) with high phase noise, exhibiting self-sustained, periodic voltage oscillations. The low CW threshold (115 A$cdot$ cm$^{-2}$) and broadband comb operation ($Delta f/f=25%$) make these sources extremely appealing for on-chip frequency comb applications.
We report on an ultralow noise optical frequency transfer from a remotely located Sr optical lattice clock laser to a Ti:Sapphire optical frequency comb through telecom-wavelength optical fiber networks. The inherent narrow linewidth of the Ti:Sapphire optical frequency comb eliminates the need for a local reference high-finesse cavity. The relative fractional frequency instability of the optical frequency comb with respect to the remote optical reference was $6.7(1) times 10^{-18}$ at 1 s and $1.05(3) times 10^{-19}$ at 1,000 s including a 2.9 km-long fiber network. This ensured the optical frequency comb had the same precision as the optical standard. Our result paves the way for ultrahigh-precision spectroscopy and conversion of the highly precise optical frequency to radio frequencies in a simpler setup.
Dual-comb sources with equally spaced and low phase noise frequency lines are of great importance for high resolution spectroscopy and metrology. In the terahertz frequency range, electrically pumped semiconductor quantum cascade lasers (QCLs) are suitable candidates for frequency comb and dual-comb operation. For a single laser frequency comb, the repetition rate can be locked using a microwave injection locking and the carrier frequency can be locked to a highly stable source. However, for the locking of two laser combs, four frequencies (two repetition rates and two carrier offset frequencies) should be simultaneously locked; If one only refers to the dual-comb signal, two relative frequencies, i.e., the offset frequency and repetition frequency of one laser against those of the other laser, should be locked. Although the locking techniques that have been successfully used for a single laser comb can be, in principle, applied to a dual-comb laser source, the complete locking considerably complicates the implementation of such a system. Here, we propose a method to stabilize a terahertz QCL dual-comb source by phase locking one of the dual-comb lines to a radio frequency (RF) synthesizer. This technique forces one of the lasers to follow the tone of the other one (keeping the sum of the carrier offset frequency difference and repetition frequency difference between the two laser combs as a constant) by exploiting a laser self-detection that avoids the use of an external detector. Through the demonstration of this locking technique, we demonstrate that the dual-comb can generate periodic pulses over a 2 us time scale, showing that the terahertz QCL comb without a control of the repetition rate can produce pulsed-type waveforms.
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