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Register a new userFluctuating Cooper pairs in FeSe at temperatures exceeding double Tc
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Temperature dependencies of excess conductivity, Sigma, have been studied in detail for three FeSe_{0.94} textured polycrystalline samples prepared by partial melting and solid state reaction. It was revealed that both Sigma and its temperature dependence are extremely sensitive to the method of sample preparation. Then, it was shown that in the range from the superconducting transition temperature Tc ~ 9 K up to the characteristic temperature T_01 ~ 19 K, Sigma(T) obeys the classical fluctuation theories of Aslamazov-Larkin (AL) and Hikami-Larkin (Maki-Thompson (MT) term) pointing to the existence of fluctuating Cooper pairs in FeSe at temperatures exceeding double Tc. Like in cuprates, AL-MT crossover at T_0 < T_{01} is observed, which means the appearance of 3D-2D dimensional transition at this temperature. This allows us to determine the coherence length along the c-axis, Xi_c(0) ~ 3 A, and a set of additional samples parameters, including the phase relaxation time, Tau_{Phi}, of fluctuating Cooper pairs, within a simple two-dimensional free-carrier picture. It was shown that Tau_{Phi} in FeSe coincides with that found for YBa2Cu3O7 suggesting that the nature of superconducting fluctuations is very similar for these high-temperature superconductors of different types.
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Superconductivity arises from two distinct quantum phenomena: electron pairing and long-range phase coherence. In conventional superconductors, the two quantum phenomena generally take place simultaneously, while the electron pairing occurs at higher temperature than the long-range phase coherence in the underdoped high-Tc cuprate superconductors. Recently, whether electron pairing is also prior to long-range phase coherence in single-layer FeSe film on SrTiO3 substrate is under debate. Here, by measuring Knight shift and nuclear spin-lattice relaxation rate, we unambiguously reveal a pseudogap behavior below Tp ~ 60 K in two layered FeSe-based superconductors with quasi-two-dimension. In the pseudogap regime, a weak diamagnetic signal and a remarkable Nernst effect are also observed, which indicate that the observed pseudogap behavior is related to superconducting fluctuations. These works confirm that strong phase fluctuation is an important character in the two-dimensional iron-based superconductors as widely observed in high-Tc cuprate superconductors.
A theory of the fluctuation-induced Nernst effect is developed for arbitrary magnetic fields and temperatures beyond the upper critical field line in a two-dimensional superconductor. First, we derive a simple phenomenological formula for the Nernst coefficient, which naturally explains the giant Nernst signal due to fluctuating Cooper pairs. The latter is shown to be large even far from the transition and may exceed by orders of magnitude the Fermi liquid terms. We also present a complete microscopic calculation (which includes quantum fluctuations) of the Nernst coefficient and give its asymptotic dependencies in various regions on the phase diagram. It is argued that the magnitude and the behavior of the Nernst signal observed experimentally in disordered superconducting films can be well-understood on the basis of the superconducting fluctuation theory.
Long-range order is destroyed in a superconductor warmed above its critical temperature (Tc). However, amplitude fluctuations of the superconducting order parameter survive and lead to a number of well established phenomena such as paraconductivity : an excess of charge conductivity due to the presence of short-lived Cooper pairs in the normal state. According to an untested theory, these pairs generate a transverse thermoelectric (Nernst) signal. In amorphous superconducting films, the lifetime of Cooper pairs exceeds the elastic lifetime of quasi-particles in a wide temperature range above Tc; consequently, the Cooper pairs Nernst signal dominate the response of the normal electrons well above Tc. In two dimensions, the magnitude of the expected signal depends only on universal constants and the superconducting coherence length, so the theory can be unambiguously tested. Here, we report on the observation of a Nernst signal in such a superconductor traced deep into the normal state. Since the amplitude of this signal is in excellent agreement with the theoretical prediction, the result provides the first unambiguous case for a Nernst effect produced by short-lived Cooper pairs.
We study the time evolution of a system of fermions with pairing interactions at a finite temperature. The dynamics is triggered by an abrupt increase of the BCS coupling constant. We show that if initially the fermions are in a normal phase, the amplitude of the BCS order parameter averaged over the Boltzman distribution of initial states exhibits damped oscillations with a relatively short decay time. The latter is determined by the temperature, the single-particle level spacing, and the ground state value of the BCS gap for the new coupling. In contrast, the decay is essentially absent when the system was in a superfluid phase before the coupling increase.
Recent scanning tunnelling microscopy experiments in NbN thin disordered superconducting films found an emergent inhomogeneity at the scale of tens of nanometers. This inhomogeneity is mirrored by an apparent dimensional crossover in the paraconductivity measured in transport above the superconducting critical temperature $T_c$. This behavior was interpreted in terms of an anomalous diffusion of fluctuating Cooper pairs, that display a {em quasi-confinement} (i.e., a slowing down of their diffusive dynamics) on length scales shorter than the inhomogeneity identified by tunnelling experiments. Here we assume this anomalous diffusive behavior of fluctuating Cooper pairs and calculate the effect of these fluctuations on the electron density of states above $T_c$. We find that the density of states is substantially suppressed up to temperatures well above $T_c$. This behavior, which is closely reminiscent of a pseudogap, only arises from the anomalous diffusion of fluctuating Cooper pairs in the absence of stable preformed pairs, setting the stage for an intermediate behavior between the two common paradigms in the superconducting-insulator transition, namely the localisation of Cooper pairs (the so-called bosonic scenario) and the breaking of Cooper pairs into unpaired electrons due to strong disorder (the so-called fermionic scenario).
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