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Register a new userPerformance Study of Charcoal-based Radon Reduction Systems for Ultraclean Rare Event Detectors
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The continuous emanation of radon due to trace amounts of uranium and thorium in detector materials introduces radon to the active detection volume of low-background rare event search detectors. $^{222}$Rn produces a particularly problematic background in the physics region of interest by the ``naked beta decay of its $^{214}$Pb daughter nucleus. While charcoal-based adsorption traps are expected to be effective for radon reduction in auxiliary circulation loops that service the warm components of current {ton-scale} detectors at slow flow rates $(0.5-2;SLPM)$, radon reduction in the entire circulation loop at high flow rates $mathcal{O}({100s;SLPM})$ is necessary to reach high sensitivity in future generation experiments. In this article we explore radon dynamics with a charcoal-based radon reduction system in the main circulation loop of time projection chamber detectors. We find that even for perfect radon traps, circulation speeds of $2,000;SLPM$ are needed to reduce radon concentration in a 10,ton detector by 90%. This is faster by a factor of four than the highest circulation speeds currently achieved in dark matter detectors. We further find that the effectiveness of vacuum swing adsorption systems, which have been employed very successfully at reducing atmospheric radon levels in clean-rooms, is limited by the intrinsic radon activity of the charcoal adsorbent in ultra-low radon environments. Adsorbents with significantly lower intrinsic radon activity than in currently available activated charcoals would be necessary to build effective vacuum swing adsorption systems operated at room temperature for rare event search experiments. If such VSA systems are cooled to about $190,K$, this requirement relaxes drastically.
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The noble elements, argon and xenon, are frequently employed as the target and event detector for weakly interacting particles such as neutrinos and Dark Matter. For such rare processes, background radiation must be carefully minimized. Radon provides one of the most significant contaminants since it is an inevitable product of trace amounts of natural uranium. To design a purification system for reducing such contamination, the adsorption characteristics of radon in nitrogen, argon, and xenon carrier gases on various types of charcoals with different adsorbing properties and intrinsic radioactive purities have been studied in the temperature range of 190-295 K at flow rates of 0.5 and 2 standard liters per minute. Essential performance parameters for the various charcoals include the average breakthrough times ($tau$), dynamic adsorption coefficients (k$_a$) and the number of theoretical stages (n). It is shown that the k$_a$-values for radon in nitrogen, argon, and xenon increase as the temperature of the charcoal traps decreases, and that they are significantly larger in nitrogen and argon than in xenon gas due to adsorption saturation effects. It is found that, unlike in xenon, the dynamic adsorption coefficients for radon in nitrogen and argon strictly obey the Arrhenius law. The experimental results strongly indicate that nitric acid etched Saratech is the best candidate among all used charcoal brands. It allows reducing total radon concentration in the LZ liquid Xe detector to meet the ultimate goal in the search for Dark Matter.
Type 5A molecular sieves (MS) have been demonstrated to remove radon from SF$_6$ gas. This is important for ultra-sensitive SF$_6$ gas-based directional dark matter and related rare-event physics experiments, as radon can provide a source of unwanted background events. Unfortunately, commercially available sieves intrinsically emanate radon at levels not suitable for ultra-sensitive physics experiments. A method to produce a low radioactive MS has been developed in Nihon University (NU). In this work, we explore the feasibility of the NU-developed 5A type MS for use in such experiments. A comparison with a commercially available Sigma-Aldrich 5A type MS was made. The comparison was done by calculating a parameter indicating the amount of radon intrinsically emanated by the MS per unit radon captured from SF$_6$ gas. The measurements were made using a specially adapted DURRIDGE RAD7 radon detector. The NU-developed 5A MS emanated radon up to 61$pm$9$%$ less per radon captured (2.1$pm$0.1)$times 10^{-3}$, compared to the commercial Sigma-Aldrich MS (5.4$pm$0.4)$times 10^{-3}$, making it a better candidate for use in a radon filtration setup for future ultra-sensitive SF$_6$ gas based experiments.
We present the design and characterization of a large-area Cryogenic PhotoDetector (CPD) designed for active particle identification in rare event searches, such as neutrinoless double beta decay and dark matter experiments. The detector consists of a $45.6$ $mathrm{cm}^2$ surface area by 1-mm-thick $10.6$ $mathrm{g}$ Si wafer. It is instrumented with a distributed network of Quasiparticle-trap-assisted Electrothermal feedback Transition-edge sensors (QETs) with superconducting critical temperature $T_c=41.5$ $mathrm{mK}$ to measure athermal phonons released from interactions with photons. The detector is characterized and calibrated with a collimated $^{55}$Fe X-ray source incident on the center of the detector. The noise equivalent power is measured to be $1times 10^{-17}$ $mathrm{W}/sqrt{mathrm{Hz}}$ in a bandwidth of $2.7$ $mathrm{kHz}$. The baseline energy resolution is measured to be $sigma_E = 3.86 pm 0.04$ $(mathrm{stat.})^{+0.23}_{-0.00}$ $(mathrm{syst.})$ $mathrm{eV}$ (RMS). The detector also has an expected timing resolution of $sigma_t = 2.3$ $mumathrm{s}$ for $5$ $sigma_E$ events.
Simulations of photon propagation in scintillation detectors were performed with the aim to find the optimal scintillator geometry, surface treatment, and shape of external reflector in order to achieve maximum light collection efficiency for detector configurations that avoid direct optical coupling, a situation that is commonly found in cryogenic scintillating bolometers in experimental searches for double beta decay and dark matter. To evaluate the light collection efficiency of various geometrical configurations we used the ZEMAX ray-tracing software. It was found that scintillators in the shape of a triangular prism with an external mirror shaped as truncated cone gives the highest light collection efficiency. The results of the simulations were confirmed by carrying out measurements of the light collection efficiencies of CaWO4 crystal scintillators. A comparison of simulated and measured values of light output shows good agreement
The rare event search experiments using germanium detectors are performed in the underground laboratories to prevent cosmic rays. However, the cosmogenic activation of the cupreous detector components on the ground will generate long half-life radioisotopes and contribute continually to the expected background level. We present a study on the cosmogenic activation of copper after 504 days of exposure at an altitude of 2469.4 m outside the China Jinping Underground Laboratory (CJPL). The specific activities of the cosmogenic nuclides produced in the copper bricks were measured using a low background germanium gamma-ray spectrometer at CJPL. The production rates at sea level, in units of nuclei/kg/day, are 18.6 pm 2.0 for Mn-54, 9.9 pm 1.3 for Co-56, 48.3 pm 5.5 for Co-57, 51.8 pm 2.5 for Co-58 and 39.7 pm 5.7 for Co-60, respectively. Given the expected exposure history of the germanium detectors, a Monte Carlo simulation is conducted to assess the cosmogenic background contributions of the detectors cupreous components.
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