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Register a new userTest of low radioactive molecular sieves for radon filtration in SF6 gas-based rare-event physics experiments
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Robert Renz Marcelo Gregorio
Publication date
2020
fields
Physics
and research's language is
English
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Type 5A molecular sieves (MS) have been demonstrated to remove radon from SF$_6$ gas. This is important for ultra-sensitive SF$_6$ gas-based directional dark matter and related rare-event physics experiments, as radon can provide a source of unwanted background events. Unfortunately, commercially available sieves intrinsically emanate radon at levels not suitable for ultra-sensitive physics experiments. A method to produce a low radioactive MS has been developed in Nihon University (NU). In this work, we explore the feasibility of the NU-developed 5A type MS for use in such experiments. A comparison with a commercially available Sigma-Aldrich 5A type MS was made. The comparison was done by calculating a parameter indicating the amount of radon intrinsically emanated by the MS per unit radon captured from SF$_6$ gas. The measurements were made using a specially adapted DURRIDGE RAD7 radon detector. The NU-developed 5A MS emanated radon up to 61$pm$9$%$ less per radon captured (2.1$pm$0.1)$times 10^{-3}$, compared to the commercial Sigma-Aldrich MS (5.4$pm$0.4)$times 10^{-3}$, making it a better candidate for use in a radon filtration setup for future ultra-sensitive SF$_6$ gas based experiments.
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This study develops low radioactive molecular sieves (MS) for ultra-low background particle physics experiment. The manufactured MS is of type 4A. $^{226}$Ra and $^{232}$Th have concentrations of about 57 and 198 mBq/kg, respectively, measured by applying high-purity germanium (HPGe) measurement. The reduction of the radioactivity from the commercial one is about 99 and 97 percent for $^{226}$Ra and $^{232}$Th, respectively. Furthermore, the radon emanation rate from MS filter is about 2.1 mBq, which is measured by utilizing pin-photo type radon detector. This developed MS is expected to remove the impurity from the noble gas, in which low radioactivity is needed such as dark matter search experiment.
The noble elements, argon and xenon, are frequently employed as the target and event detector for weakly interacting particles such as neutrinos and Dark Matter. For such rare processes, background radiation must be carefully minimized. Radon provides one of the most significant contaminants since it is an inevitable product of trace amounts of natural uranium. To design a purification system for reducing such contamination, the adsorption characteristics of radon in nitrogen, argon, and xenon carrier gases on various types of charcoals with different adsorbing properties and intrinsic radioactive purities have been studied in the temperature range of 190-295 K at flow rates of 0.5 and 2 standard liters per minute. Essential performance parameters for the various charcoals include the average breakthrough times ($tau$), dynamic adsorption coefficients (k$_a$) and the number of theoretical stages (n). It is shown that the k$_a$-values for radon in nitrogen, argon, and xenon increase as the temperature of the charcoal traps decreases, and that they are significantly larger in nitrogen and argon than in xenon gas due to adsorption saturation effects. It is found that, unlike in xenon, the dynamic adsorption coefficients for radon in nitrogen and argon strictly obey the Arrhenius law. The experimental results strongly indicate that nitric acid etched Saratech is the best candidate among all used charcoal brands. It allows reducing total radon concentration in the LZ liquid Xe detector to meet the ultimate goal in the search for Dark Matter.
The continuous emanation of radon due to trace amounts of uranium and thorium in detector materials introduces radon to the active detection volume of low-background rare event search detectors. $^{222}$Rn produces a particularly problematic background in the physics region of interest by the ``naked beta decay of its $^{214}$Pb daughter nucleus. While charcoal-based adsorption traps are expected to be effective for radon reduction in auxiliary circulation loops that service the warm components of current {ton-scale} detectors at slow flow rates $(0.5-2;SLPM)$, radon reduction in the entire circulation loop at high flow rates $mathcal{O}({100s;SLPM})$ is necessary to reach high sensitivity in future generation experiments. In this article we explore radon dynamics with a charcoal-based radon reduction system in the main circulation loop of time projection chamber detectors. We find that even for perfect radon traps, circulation speeds of $2,000;SLPM$ are needed to reduce radon concentration in a 10,ton detector by 90%. This is faster by a factor of four than the highest circulation speeds currently achieved in dark matter detectors. We further find that the effectiveness of vacuum swing adsorption systems, which have been employed very successfully at reducing atmospheric radon levels in clean-rooms, is limited by the intrinsic radon activity of the charcoal adsorbent in ultra-low radon environments. Adsorbents with significantly lower intrinsic radon activity than in currently available activated charcoals would be necessary to build effective vacuum swing adsorption systems operated at room temperature for rare event search experiments. If such VSA systems are cooled to about $190,K$, this requirement relaxes drastically.
The rare event search experiments using germanium detectors are performed in the underground laboratories to prevent cosmic rays. However, the cosmogenic activation of the cupreous detector components on the ground will generate long half-life radioisotopes and contribute continually to the expected background level. We present a study on the cosmogenic activation of copper after 504 days of exposure at an altitude of 2469.4 m outside the China Jinping Underground Laboratory (CJPL). The specific activities of the cosmogenic nuclides produced in the copper bricks were measured using a low background germanium gamma-ray spectrometer at CJPL. The production rates at sea level, in units of nuclei/kg/day, are 18.6 pm 2.0 for Mn-54, 9.9 pm 1.3 for Co-56, 48.3 pm 5.5 for Co-57, 51.8 pm 2.5 for Co-58 and 39.7 pm 5.7 for Co-60, respectively. Given the expected exposure history of the germanium detectors, a Monte Carlo simulation is conducted to assess the cosmogenic background contributions of the detectors cupreous components.
Charge trapping degrades the energy resolution of germanium (Ge) detectors, which require to have increased experimental sensitivity in searching for dark matter and neutrinoless double-beta decay. We investigate the charge trapping processes utilizing nine planar detectors fabricated from USD-grown crystals with well-known net impurity levels. The charge collection efficiency as a function of charge trapping length is derived from the Shockley-Ramo theorem. Furthermore, we develop a model that correlates the energy resolution with the charge collection efficiency. This model is then applied to the experimental data. As a result, charge collection efficiency and charge trapping length are determined accordingly. Utilizing the Lax model (further developed by CDMS collaborators), the absolute impurity levels are determined for nine detectors. The knowledge of these parameters when combined with other traits such as the Fano factor serve as a reliable indicator of the intrinsic nature of charge trapping within the crystals. We demonstrate that electron trapping is more severe than hole trapping in a p-type detector and the charge collection efficiency depends on the absolute impurity level of the Ge crystal when an adequate bias voltage is applied to the detector. Negligible charge trapping is found when the absolute impurity level is less than 1.0$times$10$^{11}/$cm$^{3}$ for collecting electrons and 2.0$times$10$^{11}/$cm$^{3}$ for collecting holes.
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