No Arabic abstract
Computable Information Density (CID), the ratio of the length of a losslessly compressed data file to that of the uncompressed file, is a measure of order and correlation in both equilibrium and nonequilibrium systems. Here we show that correlation lengths can be obtained by decimation - thinning a configuration by sampling data at increasing intervals and recalculating the CID. When the sampling interval is larger than the systems correlation length, the data becomes incompressible. The correlation length and its critical exponents are thus accessible with no a-priori knowledge of an order parameter or even the nature of the ordering. The correlation length measured in this way agrees well with that computed from the decay of two-point correlation functions $g_{2}(r)$ when they exist. But the CID reveals the correlation length and its scaling even when $g_{2}(r)$ has no structure, as we demonstrate by cloaking the data with a Rudin-Shapiro sequence.
We obtain analytic expressions for the time correlation functions of a liquid of spherical particles, exact in the limit of high dimensions $d$. The derivation is long but straightforward: a dynamic virial expansion for which only the first two terms survive, followed by a change to generalized spherical coordinates in the dynamic variables leading to saddle-point evaluation of integrals for large $d$. The problem is thus mapped onto a one-dimensional diffusion in a perturbed harmonic potential with colored noise. At high density, an ergodicity-breaking glass transition is found. In this regime, our results agree with thermodynamics, consistently with the general Random First Order Transition scenario. The glass transition density is higher than the best known lower bound for hard sphere packings in large $d$. Because our calculation is, if not rigorous, elementary, an improvement in the bound for sphere packings in large dimensions is at hand.
We numerically study the relaxation dynamics of several glass-forming models to their inherent structures, following quenches from equilibrium configurations sampled across a wide range of temperatures. In a mean-field Mari-Kurchan model, we find that relaxation changes from a power-law to an exponential decay below a well-defined temperature, consistent with recent findings in mean-field $p$-spin models. By contrast, for finite-dimensional systems, the relaxation is always algebraic, with a non-trivial universal exponent at high temperatures crossing over to a harmonic value at low temperatures. We demonstrate that this apparent evolution is controlled by a temperature-dependent population of localised excitations. Our work unifies several recent lines of studies aiming at a detailed characterization of the complex potential energy landscape of glass-formers.
The existence of a constant density of two-level systems (TLS) was proposed as the basis of some intriguing universal aspects of glasses at ultra-low temperatures. Here we ask whether their existence is necessary for explaining the universal density of states quasi-localized modes (QLM) in glasses at ultra-low temperatures. A careful examination of the QLM that exist in a generic atomistic model of a glass former reveals at least two types of them, each exhibiting a different density of states, one depending on the frequency as $omega^3$ and the other as $omega^4$. The properties of the glassy energy landscape that is responsible for the two types of modes is examined here, explaining the analytic feature responsible for the creations of (at least) two families of QLMs. Although adjacent wells certainly exist in the complex energy landscape of glasses, doubt is cast on the relevance of TLS for the universal density of QLMs.
As shown by early studies on mean-field models of the glass transition, the geometrical features of the energy landscape provide fundamental information on the dynamical transition at the Mode-Coupling temperature $T_d$. We show that active particles can serve as a useful tool for gaining insight into the topological crossover in model glass-formers. In such systems the landmark of the minima-to-saddle transition in the potential energy landscape, taking place in the proximity of $T_d$, is the critical slowing down of dynamics. Nevertheless, the critical slowing down is a bottleneck for numerical simulations and the possibility to take advantage of the new smart algorithms capable to thermalize down in the glass phase is attractive. Our proposal is to consider configurations equilibrated below the threshold and study their dynamics in the presence of a small amount of self-propulsion. As exemplified here from the study of the p-spin model, the presence of self-propulsion gives rise to critical off-equilibrium equal-time correlations at the minima-to-saddles crossover, correlations which are not hindered by the sluggish glassy dynamics.
We review generalized Fluctuation-Dissipation Relations which are valid under general conditions even in ``non-standard systems, e.g. out of equilibrium and/or without a Hamiltonian structure. The response functions can be expressed in terms of suitable correlation functions computed in the unperperturbed dynamics. In these relations, typically one has nontrivial contributions due to the form of the stationary probability distribution; such terms take into account the interaction among the relevant degrees of freedom in the system. We illustrate the general formalism with some examples in non-standard cases, including driven granular media, systems with a multiscale structure, active matter and systems showing anomalous diffusion.