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Register a new userFast reconstruction of atomic-scale STEM-EELS images from sparse sampling
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This paper discusses the reconstruction of partially sampled spectrum-images to accelerate the acquisition in scanning transmission electron microscopy (STEM). The problem of image reconstruction has been widely considered in the literature for many imaging modalities, but only a few attempts handled 3D data such as spectral images acquired by STEM electron energy loss spectroscopy (EELS). Besides, among the methods proposed in the microscopy literature, some are fast but inaccurate while others provide accurate reconstruction but at the price of a high computation burden. Thus none of the proposed reconstruction methods fulfills our expectations in terms of accuracy and computation complexity. In this paper, we propose a fast and accurate reconstruction method suited for atomic-scale EELS. This method is compared to popular solutions such as beta process factor analysis (BPFA) which is used for the first time on STEM-EELS images. Experiments based on real as synthetic data will be conducted.
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Electron microscopy has shown to be a very powerful tool to map the chemical nature of samples at various scales down to atomic resolution. However, many samples can not be analyzed with an acceptable signal-to-noise ratio because of the radiation damage induced by the electron beam. This is particularly crucial for electron energy loss spectroscopy (EELS) which acquires spectral-spatial data and requires high beam intensity. Since scanning transmission electron microscopes (STEM) are able to acquire data cubes by scanning the electron probe over the sample and recording a spectrum for each spatial position, it is possible to design the scan pattern and to sample only specific pixels. As a consequence, partial acquisition schemes are now conceivable, provided a reconstruction of the full data cube is conducted as a post-processing step. This paper proposes two reconstruction algorithms for multi-band images acquired by STEM-EELS which exploits the spectral structure and the spatial smoothness of the image. The performance of the proposed schemes is illustrated thanks to experiments conducted on a realistic phantom dataset as well as real EELS spectrum-images.
Atomically resolved electron energy-loss spectroscopy experiments are commonplace in modern aberrationcorrected transmission electron microscopes. Energy resolution has also been increasing steadily with the continuous improvement of electron monochromators. Electronic excitations however are known to be delocalised due to the long range interaction of the charged accelerated electrons with the electrons in a sample. This has made several scientists question the value of combined high spatial and energy resolution for mapping interband transitions and possibly phonon excitation in crystals. In this paper we demonstrate experimentally that atomic resolution information is indeed available at very low energy losses around 100 meV expressed as a modulation of the broadening of the zero loss peak. Careful data analysis allows us to get a glimpse of what are likely phonon excitations with both an energy loss and gain part. These experiments confirm recent theoretical predictions on the strong localisation of phonon excitations as opposed to electronic excitations and show that a combination of atomic resolution and recent developments in increased energy resolution will offer great benefit for mapping phonon modes in real space.
Porous media are ubiquitous in both nature and engineering applications, thus their modelling and understanding is of vital importance. In contrast to direct acquisition of three-dimensional (3D) images of such medium, obtaining its sub-region (s) like two-dimensional (2D) images or several small areas could be much feasible. Therefore, reconstructing whole images from the limited information is a primary technique in such cases. Specially, in practice the given data cannot generally be determined by users and may be incomplete or partially informed, thus making existing reconstruction methods inaccurate or even ineffective. To overcome this shortcoming, in this study we proposed a deep learning-based framework for reconstructing full image from its much smaller sub-area(s). Particularly, conditional generative adversarial network (CGAN) is utilized to learn the mapping between input (partial image) and output (full image). To preserve the reconstruction accuracy, two simple but effective objective functions are proposed and then coupled with the other two functions to jointly constrain the training procedure. Due to the inherent essence of this ill-posed problem, a Gaussian noise is introduced for producing reconstruction diversity, thus allowing for providing multiple candidate outputs. Extensively tested on a variety of porous materials and demonstrated by both visual inspection and quantitative comparison, the method is shown to be accurate, stable yet fast ($sim0.08s$ for a $128 times 128$ image reconstruction). We highlight that the proposed approach can be readily extended, such as incorporating any user-define conditional data and an arbitrary number of object functions into reconstruction, and being coupled with other reconstruction methods.
Capturing visual image with a hyperspectral camera has been successfully applied to many areas due to its narrow-band imaging technology. Hyperspectral reconstruction from RGB images denotes a reverse process of hyperspectral imaging by discovering an inverse response function. Current works mainly map RGB images directly to corresponding spectrum but do not consider context information explicitly. Moreover, the use of encoder-decoder pair in current algorithms leads to loss of information. To address these problems, we propose a 4-level Hierarchical Regression Network (HRNet) with PixelShuffle layer as inter-level interaction. Furthermore, we adopt a residual dense block to remove artifacts of real world RGB images and a residual global block to build attention mechanism for enlarging perceptive field. We evaluate proposed HRNet with other architectures and techniques by participating in NTIRE 2020 Challenge on Spectral Reconstruction from RGB Images. The HRNet is the winning method of track 2 - real world images and ranks 3rd on track 1 - clean images. Please visit the project web page https://github.com/zhaoyuzhi/Hierarchical-Regression-Network-for-Spectral-Reconstruction-from-RGB-Images to try our codes and pre-trained models.
Inorganic lead halide perovskites are promising candidates for optoelectronic applications, due to their bandgap tunability, high photoluminescence quantum yield, and narrow emission line widths. In particular, they offer the possibility to vary the bandgap as a function of the halide composition and dimension/shape of the crystals at the nanoscale. Here we present an aberration-corrected scanning transmission microscopy (STEM) study of extended nanosheets of CsPbBr3 directly demonstrating their orthorhombic crystal structure and their lateral termination with Cs-Br planes. The bandgaps from individual nanosheets are measured by monochromated electron energy loss spectroscopy (EELS). We find an increase of the bandgap starting at thicknesses below 10 nm, confirming the less dramatic effect of 1D confinement in nanosheets compared to the 3D confinement observed in quantum dots, as predicted by density functional theory calculations and optical spectroscopy data from ensemble measurements.
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