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Multiscale dynamics at the antiferromagnetic-ferromagnetic phase transition in FeRh

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 Added by Guanqiao Li
 Publication date 2020
  fields Physics
and research's language is English




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Using a double-pump pulse approach and laser-induced THz emission as an ultrafast amperemeter and magnetometer, we show that a femtosecond laser pulse generates ferromagnetic nuclei in a FeRh/Pt bilayer, i.e. these nuclei acquire a net magnetization and a susceptibility to a magnetic field, but only 20 ps after the initial laser excitation. We argue that this latency is intrinsic to the first-order phase transitions from antiferromagnetic to ferromagnetic states and must be present even in the case when the sign of the exchange interaction changes instantaneously.



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The antiferromagnetic (AFM) to ferromagnetic (FM) first order phase transition of an epitaxial FeRh thin-film has been studied with x-ray magnetic circular dichroism using photoemission electron microscopy. The FM phase is magnetized in-plane due to shape anisotropy, but the magnetocrystalline anisotropy is negligible and there is no preferred in-plane magnetization direction. When heating through the AFM to FM phase transition the nucleation of the FM phase occurs at many independent nucleation sites with random domain orientation. The domains subsequently align to form the final FM domain structure. We observe no pinning of the FM domain structure.
The antiferromagnetic to ferromagnetic phase transition in B2-ordered FeRh is imaged in laterally confined nanopatterned islands using photoemission electron microscopy with x-ray magnetic circular dichroism contrast. The resulting magnetic images directly detail the progression in the shape and size of the FM phase domains during heating and cooling through the transition. In 5 um square islands this domain development during heating is shown to proceed in three distinct modes: nucleation, growth, and merging, each with subsequently greater energy costs. In 0.5 um islands, which are smaller than the typical final domain size, the growth mode is stunted and the transition temperature was found to be reduced by 20 K. The modification to the transition temperature is found by high resolution scanning transmission electron microscopy to be due to a 100 nm chemically disordered edge grain present as a result of ion implantation damage during the patterning. FeRh has unique possibilities for magnetic memory applications; the inevitable changes to its magnetic properties due to subtractive nanofabrication will need to be addressed in future work in order to progress from sheet films to suitable patterned devices.
We use textit{ab-initio} calculations to investigate spin-orbit torques (SOTs) in FeRh(001) deposited on W(100). Since FeRh undergoes a ferromagnetic-antiferromagnetic phase transition close to room temperature, we consider both phases of FeRh. In the antiferromagnetic case we find that the effective magnetic field of the even torque is staggered and therefore ideal to induce magnetization dynamics or to switch the antiferromagnet (AFM). At the antiferromagnetic resonance the inverse SOT induces a current density, which can be determined from the SOT. In the ferromagnetic case our calculations predict both even and odd components of the SOT, which can also be used to describe the ac and dc currents induced at the ferromagnetic resonance. For comparison we compute the SOTs in the c($2times 2$) AFM state of Fe/W(001).
204 - Z. X. Feng , H. Yan , Z. Q. Liu 2018
Using an electric field instead of an electric current (or a magnetic field) to tailor the electronic properties of magnetic materials is promising for realizing ultralow energy-consuming memory devices because of the suppression of Joule heating, especially when the devices are scaled to the nanoscale. In the review, we summarize recent results on the giant magnetization and resistivity modulation in a metamagnetic intermetallic alloy - FeRh, which is achieved by electric-field-controlled magnetic phase transitions in multiferroic heterostructures. Furthermore, the approach is extended to topological antiferromagnetic spintronics, which is currently receiving attention in the magnetic society, and the antiferromagnetic order parameter has been able to switch back and forth by a small electric field. In the end, we envision the possibility of manipulating exotic physical phenomena in the emerging topological antiferromagnetic spintronics field via the electric-field approach.
Spin-wave resonance measurements were performed in the mixed magnetic phase regime of a Pd-doped FeRh epilayer that appears as the first-order ferromagnetic-antiferromagnetic phase transition takes place. It is seen that the measured value of the exchange stiffness is suppressed throughout the measurement range when compared to the expected value of the fully ferromagnetic regime, extracted via the independent means of a measurement of the Curie point, for only slight changes in the ferromagnetic volume fraction. This behavior is attributed to the influence of the antiferromagnetic phase: inspired by previous experiments that show ferromagnetism to be most persistent at the surfaces and interfaces of FeRh thin films, we modelled the antiferromagnetic phase as forming a thin layer in the middle of the epilayer through which the two ferromagnetic layers are coupled up to a certain critical thickness. The development of this exchange stiffness is then consistent with that expected from the development of an exchange coupling across the magnetic phase boundary, as a consequence of a thickness dependent phase transition taking place in the antiferromagnetic regions and is supported by complimentary computer simulations of atomistic spin-dynamics. The development of the Gilbert damping parameter extracted from the ferromagnetic resonance investigations is consistent with this picture.
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