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Register a new userBand-Gap-Dependent Electronic Compressibility of Carbon Nanotubes in the Wigner Crystal Regime
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Electronic compressibility, the second derivative of ground state energy with respect to total electron number, is a measurable quantity that reveals the interaction strength of a system and can be used to characterize the orderly crystalline lattice of electrons known as the Wigner crystal. Here, we measure the electronic compressibility of individual suspended ultraclean carbon nanotubes in the low-density Wigner crystal regime. Using low-temperature quantum transport measurements, we determine the compressibility as a function of carrier number in nanotubes with varying band gaps. We observe two qualitatively different trends in compressibility versus carrier number, both of which can be explained using a theoretical model of a Wigner crystal that accounts for both the band gap and the confining potential experienced by charge carriers. We extract the interaction strength as a function of carrier number for individual nanotubes and show that the compressibility can be used to distinguish between strongly and weakly interacting regimes.
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Electron-electron interactions strongly affect the behavior of low-dimensional systems. In one dimension (1D), arbitrarily weak interactions qualitatively alter the ground state producing a Luttinger liquid (LL) which has now been observed in a number of experimental systems. Interactions are even more important at low carrier density, and in the limit when the long-ranged Coulomb potential is the dominant energy scale, the electron liquid is expected to become a periodically ordered solid known as the Wigner crystal. In 1D, the Wigner crystal has been predicted to exhibit novel spin and magnetic properties not present in an ordinary LL. However, despite recent progress in coupled quantum wires, unambiguous experimental demonstration of this state has not been possible due to the role of disorder. Here, we demonstrate using low-temperature single-electron transport spectroscopy that a hole gas in low-disorder carbon nanotubes with a band gap is a realization of the 1D Wigner crystal. Our observation can lead to unprecedented control over the behavior of the spatially separated system of carriers, and could be used to realize solid state quantum computing with long coherence times.
Recent NMR experiments by Singer et al. [Singer et al. Phys. Rev. Lett. 95, 236403 (2005).] showed a deviation from Fermi-liquid behavior in carbon nanotubes with an energy gap evident at low temperatures. Here, a comprehensive theory for the magnetic field and temperature dependent NMR 13C spin-lattice relaxation is given in the framework of the Tomonaga-Luttinger liquid. The low temperature properties are governed by a gapped relaxation due to a spin gap (~ 30K), which crosses over smoothly to the Luttinger liquid behaviour with increasing temperature.
We present a detailed theoretical analysis of the Wigner crystal states in confined semiconducting carbon nanotubes. We show by robust scaling arguments as well as by detailed semi-microscopic calculations that the effective exchange interaction has an SU(4) symmetry, and can reach values even as large as $Jsim 100 {rm ,K}$ in weakly screened, small diameter nanotubes, close to the Wigner crystal - electron liquid crossover. Modeling the nanotube carefully and analyzing the magnetic structure of the inhomogeneous electron crystal, we recover the experimentally observed phase boundaries of Deshpande and Bockrath [V. V. Deshpande and M. Bockrath, Nature Physics $mathbf 4$, 314 (2008)]. Spin-orbit coupling only slightly modifies these phase boundaries, but breaks the spin symmetry down to SU(2)$times$SU(2), and in Wigner molecules it gives rise to interesting excitation spectra, reflecting the underlying SU(4) as well as the residual SU(2)$times$SU(2) symmetries.
Conventional wisdom had long held that a composite particle behaves just like an ordinary Newtonian particle. In this paper, we derive the effective dynamics of a type-I Wigner crystal of composite particles directly from its microscopic wave function. It indicates that the composite particles are subjected to a Berry curvature in the momentum space as well as an emergent dissipationless viscosity. Therefore, contrary to the general belief, composite particles follow the more general Sundaram-Niu dynamics instead of the ordinary Newtonian one. We show that the presence of the Berry curvature is an inevitable feature for a dynamics consistent with the dipole picture of composite particles and Kohns theorem. Based on the dynamics, we determine the dispersions of magneto-phonon excitations numerically. We find an emergent magneto-roton mode which signifies the composite-particle nature of the Wigner crystal. It occurs at frequencies much lower than the magnetic cyclotron frequency and has a vanishing oscillator strength in the long wavelength limit.
Carbon nanotubes (CNTs) are a promising material for high-performance electronics beyond silicon. But unlike silicon, the nature of the transport band gap in CNTs is not fully understood. The transport gap in CNTs is predicted to be strongly driven by electron-electron (e-e) interactions and correlations, even at room temperature. Here, we use dielectric liquids to screen e-e interactions in individual suspended ultra-clean CNTs. Using multiple techniques, the transport gap is measured as dielectric screening is increased. Changing the dielectric environment from air to isopropanol, we observe a 25% reduction in the transport gap of semiconducting CNTs, and a 32% reduction in the band gap of narrow-gap CNTs. Additional measurements are reported in dielectric oils. Our results elucidate the nature of the transport gap in CNTs, and show that dielectric environment offers a mechanism for significant control over the transport band gap.
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