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Register a new userThe One-Dimensional Wigner Crystal in Carbon Nanotubes
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Electron-electron interactions strongly affect the behavior of low-dimensional systems. In one dimension (1D), arbitrarily weak interactions qualitatively alter the ground state producing a Luttinger liquid (LL) which has now been observed in a number of experimental systems. Interactions are even more important at low carrier density, and in the limit when the long-ranged Coulomb potential is the dominant energy scale, the electron liquid is expected to become a periodically ordered solid known as the Wigner crystal. In 1D, the Wigner crystal has been predicted to exhibit novel spin and magnetic properties not present in an ordinary LL. However, despite recent progress in coupled quantum wires, unambiguous experimental demonstration of this state has not been possible due to the role of disorder. Here, we demonstrate using low-temperature single-electron transport spectroscopy that a hole gas in low-disorder carbon nanotubes with a band gap is a realization of the 1D Wigner crystal. Our observation can lead to unprecedented control over the behavior of the spatially separated system of carriers, and could be used to realize solid state quantum computing with long coherence times.
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In one-dimensional quantum systems with strong long-range repulsion particles arrange in a quasi-periodic chain, the Wigner crystal. We demonstrate that besides the familiar phonons, such one-dimensional Wigner crystal supports an additional mode of elementary excitations, which can be identified with solitons in the classical limit. We compute the corresponding excitation spectrum and argue that the solitons have a parametrically small decay rate at low energies. We discuss implications of our results for the behavior of the dynamic structure factor.
Electronic compressibility, the second derivative of ground state energy with respect to total electron number, is a measurable quantity that reveals the interaction strength of a system and can be used to characterize the orderly crystalline lattice of electrons known as the Wigner crystal. Here, we measure the electronic compressibility of individual suspended ultraclean carbon nanotubes in the low-density Wigner crystal regime. Using low-temperature quantum transport measurements, we determine the compressibility as a function of carrier number in nanotubes with varying band gaps. We observe two qualitatively different trends in compressibility versus carrier number, both of which can be explained using a theoretical model of a Wigner crystal that accounts for both the band gap and the confining potential experienced by charge carriers. We extract the interaction strength as a function of carrier number for individual nanotubes and show that the compressibility can be used to distinguish between strongly and weakly interacting regimes.
The spatial Fourier spectrum of the electron density distribution in a finite 1D system and the distribution function of electrons over single-particle states are studied in detail to show that there are two universal features in their behavior, which characterize the electron ordering and the deformation of Wigner crystal by boundaries. The distribution function has a $delta$-like singularity at the Fermi momentum $k_F$. The Fourier spectrum of the density has a step-like form at the wavevector $2k_F$, with the harmonics being absent or vanishing above this threshold. These features are found by calculations using exact diagonalization method. They are shown to be caused by Wigner ordering of electrons, affected by the boundaries. However the common Luttinger liquid model with open boundaries fails to capture these features, because it overestimates the deformation of the Wigner crystal. An improvement of the Luttinger liquid model is proposed which allows one to describe the above features correctly. It is based on the corrected form of the density operator conserving the particle number.
We consider a system of one-dimensional spinless particles interacting via long-range repulsion. In the limit of strong interactions the system is a Wigner crystal, with excitations analogous to phonons in solids. In a harmonic crystal the phonons do not interact, and the system never reaches thermal equilibrium. We account for the anharmonism of the Wigner crystal and find the rate at which it approaches equilibrium. The full equilibration of the system requires umklapp scattering of phonons, resulting in exponential suppression of the equilibration rate at low temperatures.
We present a detailed theoretical analysis of the Wigner crystal states in confined semiconducting carbon nanotubes. We show by robust scaling arguments as well as by detailed semi-microscopic calculations that the effective exchange interaction has an SU(4) symmetry, and can reach values even as large as $Jsim 100 {rm ,K}$ in weakly screened, small diameter nanotubes, close to the Wigner crystal - electron liquid crossover. Modeling the nanotube carefully and analyzing the magnetic structure of the inhomogeneous electron crystal, we recover the experimentally observed phase boundaries of Deshpande and Bockrath [V. V. Deshpande and M. Bockrath, Nature Physics $mathbf 4$, 314 (2008)]. Spin-orbit coupling only slightly modifies these phase boundaries, but breaks the spin symmetry down to SU(2)$times$SU(2), and in Wigner molecules it gives rise to interesting excitation spectra, reflecting the underlying SU(4) as well as the residual SU(2)$times$SU(2) symmetries.
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