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For most chiralities, semiconducting nanotubes display topologically protected end states of multiple degeneracies. We demonstrate using density matrix renormalization group based quantum chemistry tools that the presence of Coulomb interactions induces the formation of robust end spins. These are the close analogues of ferromagnetic edge states emerging in graphene nanoribbons. The interaction between the two ends is sensitive to the length of the nanotube, its dielectric constant, as well as the size of the end spins: for $S=1/2$ end spins their interaction is antiferromagnetic, while for $S>1/2$ it changes from antiferromagnetic to ferromagnetic as the nanotube length increases. The interaction between end spins can be controlled by changing the dielectric constant of the environment, thereby providing a possible platform for two-spin quantum manipulations.
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Edge states exhibit the nontrivial topology of energy band in the bulk. As localized states at boundaries, many-particle edge states may obey a special symmetry that is broken in the bulk. When local particle-particle interaction is induced, they may support a particular property. We consider an anisotropic two-dimensional Su-Schrieffer-Heeger Hubbard model and examine the appearance of $eta$-pairing edge states. In the absence of Hubbard interaction, the energy band is characterized by topologically invariant polarization in association with edge states. In the presence of on-site Hubbard interaction, $eta$-pairing edge states with an off-diagonal long-range order appear in the nontrivial topological phase, resulting in the condensation of pairs at the boundary. In addition, as Hamiltonian eigenstates, the edge states contain one paired component and one unpaired component. Neither affects the other; they act as two-fluid states. From numerical simulations of many-particle scattering processes, a clear manifestation and experimental detection scheme of topologically protected two-fluid edge states are provided.
We study spin-orbit coupling in metallic carbon nanotubes (CNTs) within the many-body Tomonaga-Luttinger liquid (TLL) framework. For a well defined sub-class of metallic CNTs, that contains both achiral zig-zag as well as a sub-set of chiral tubes, an effective low energy field theory description is derived. We aim to describe system at finite dopings, but close to the charge neutrality point (commensurability). A new regime is identified where spin-orbit coupling leads to an inverted hierarchy of mini-gaps of bosonic modes. We then add a proximity coupling to a superconducting (SC) substrate and show that the only order parameter that is supported within the novel, spin-orbit induced phase is a topologically trivial s-SC.
Recent NMR experiments by Singer et al. [Singer et al. Phys. Rev. Lett. 95, 236403 (2005).] showed a deviation from Fermi-liquid behavior in carbon nanotubes with an energy gap evident at low temperatures. Here, a comprehensive theory for the magnetic field and temperature dependent NMR 13C spin-lattice relaxation is given in the framework of the Tomonaga-Luttinger liquid. The low temperature properties are governed by a gapped relaxation due to a spin gap (~ 30K), which crosses over smoothly to the Luttinger liquid behaviour with increasing temperature.
Electron-electron interactions strongly affect the behavior of low-dimensional systems. In one dimension (1D), arbitrarily weak interactions qualitatively alter the ground state producing a Luttinger liquid (LL) which has now been observed in a number of experimental systems. Interactions are even more important at low carrier density, and in the limit when the long-ranged Coulomb potential is the dominant energy scale, the electron liquid is expected to become a periodically ordered solid known as the Wigner crystal. In 1D, the Wigner crystal has been predicted to exhibit novel spin and magnetic properties not present in an ordinary LL. However, despite recent progress in coupled quantum wires, unambiguous experimental demonstration of this state has not been possible due to the role of disorder. Here, we demonstrate using low-temperature single-electron transport spectroscopy that a hole gas in low-disorder carbon nanotubes with a band gap is a realization of the 1D Wigner crystal. Our observation can lead to unprecedented control over the behavior of the spatially separated system of carriers, and could be used to realize solid state quantum computing with long coherence times.
The low-energy theory for multi-wall carbon nanotubes including the long-ranged Coulomb interactions, internal screening effects, and single-electron hopping between graphite shells is derived and analyzed by bosonization methods. Characteristic Luttinger liquid power laws are found for the tunneling density of states, with exponents approaching their Fermi liquid value only very slowly as the number of conducting shells increases. With minor modifications, the same conclusions apply to transport in ropes of single-wall nanotubes.
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