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Register a new userLuttinger liquid behavior in multi-wall carbon nanotubes
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R. Egger
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The low-energy theory for multi-wall carbon nanotubes including the long-ranged Coulomb interactions, internal screening effects, and single-electron hopping between graphite shells is derived and analyzed by bosonization methods. Characteristic Luttinger liquid power laws are found for the tunneling density of states, with exponents approaching their Fermi liquid value only very slowly as the number of conducting shells increases. With minor modifications, the same conclusions apply to transport in ropes of single-wall nanotubes.
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Transport properties of metallic single-wall nanotubes are examined based on the Luttinger liquid theory. Focusing on a nanotube transistor setup, the linear conductance is computed from the Kubo formula using perturbation theory in the lead-tube tunnel conductances. For sufficiently long nanotubes and high temperature, phonon backscattering should lead to an anomalous temperature dependence of the resistivity.
An interacting one-dimensional (1D) electron system is predicted to behave very differently than its higher-dimensional counterparts. Coulomb interactions strongly modify the properties away from those of a Fermi liquid, resulting in a Luttinger liquid (LL) characterized by a power-law vanishing of the density of states at the Fermi level. Experiments on one-dimensional semiconductor wires and fractional quantum Hall conductors have been interpreted using this picture, but questions remain about the connection between theory and experiment. Recently, single-walled carbon nanotubes (SWNTs) have emerged as a new type of 1D conductor that may exhibit LL behavior. Here we present measurements of the conductance of individual ropes of such SWNTs as a function of temperature and voltage. Power law behavior as a function of temperature or bias voltage is observed: G~ T^a and dI/dV ~ V^a. Both the power-law functional forms and the inferred exponents are in good agreement with theoretical predictions for tunneling into a LL.
Recent NMR experiments by Singer et al. [Singer et al. Phys. Rev. Lett. 95, 236403 (2005).] showed a deviation from Fermi-liquid behavior in carbon nanotubes with an energy gap evident at low temperatures. Here, a comprehensive theory for the magnetic field and temperature dependent NMR 13C spin-lattice relaxation is given in the framework of the Tomonaga-Luttinger liquid. The low temperature properties are governed by a gapped relaxation due to a spin gap (~ 30K), which crosses over smoothly to the Luttinger liquid behaviour with increasing temperature.
A novel method for detecting Luttinger-liquid behavior is proposed. The idea is to measure the tunneling conductance between a quantum wire and a parallel two-dimensional electron system as a function of both the potential difference between them, $V$, and an in-plane magnetic field, $B$. We show that the two-parameter dependence on $B$ and $V$ allows for a determination of the characteristic dependence on wave vector $q$ and frequency $omega$ of the {it spectral function}, $A_{rm LL}(q,omega)$, of the quantum wire. In particular, the separation of spin and charge in the Luttinger liquid should manifest itself as singularities in the $I$-$V$-characteristic. The experimental feasibility of the proposal is discussed.
A comprehensive theory of electron spin resonance (ESR) for a Luttinger liquid (LL) state of correlated metals is presented. The ESR measurables such as the signal intensity and the line-width are calculated in the framework of Luttinger liquid theory with broken spin rotational symmetry as a function of magnetic field and temperature. We obtain a significant temperature dependent homogeneous line-broadening which is related to the spin symmetry breaking and the electron-electron interaction. The result crosses over smoothly to the ESR of itinerant electrons in the non-interacting limit. These findings explain the absence of the long-sought ESR signal of itinerant electrons in single-wall carbon nanotubes when considering realistic experimental conditions.
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