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Register a new userEmergence of material momentum in optical media
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Understanding the momentum of light when propagating through optical media is not only fundamental for studies as varied as classical electrodynamics and polaritonics in condensed matter physics, but also for important applications such as optical-force manipulations and photovoltaics. From a microscopic perspective, an optical medium is in fact a complex system that can split the light momentum into the electromagnetic field, as well as the material electrons and the ionic lattice. Here, we disentangle the partition of momentum associated with light propagation in optical media, and develop a quantum theory to explicitly calculate its distribution. The material momentum here revealed, which is distributed among electrons and ionic lattice, leads to the prediction of unexpected phenomena. In particular, the electron momentum manifests through an intrinsic DC current, and strikingly, we find that under certain conditions this current can be along the photonic wave vector, implying an optical pulling effect on the electrons. Likewise, an optical pulling effect on the lattice can also be observed, such as in graphene during plasmon propagation. We also predict the emergence of boundary electric dipoles associated with light transmission through finite media, offering a microscopic explanation of optical pressure on material boundaries.
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Spin and orbital angular momentum of light plays a central role in quantum nanophotonics as well as topological electrodynamics. Here, we show that the thermal radiation from finite-sized bodies comprising of nonreciprocal magneto-optical materials can exert a spin torque even in global thermal equilibrium. Moving beyond the paradigm of near-field heat transfer, we calculate near-field radiative angular momentum transfer between finite-sized nonreciprocal objects by combining Rytovs fluctuational electrodynamics with the theory of optical angular momentum. We prove that a single magneto-optical cubic particle in non-equilibrium with its surroundings experiences a torque in the presence of an applied magnetic field (T-symmetry breaking). Furthermore, even in global thermal equilibrium, two particles with misaligned gyrotropic axes experience equal magnitude torques with opposite signs which tend to align their gyrotropic axes parallel to each other. Our results are universally applicable to semiconductors like InSb (magneto-plasmas) as well as Weyl semi-metals which exhibit the anomalous Hall effect (gyrotropy) at infrared frequencies. Our work paves the way towards near-field angular momentum transfer mediated by thermal fluctuations for nanoscale devices.
The coupling of laser light to matter can exert sub-cycle coherent control over material properties, with optically induced currents and magnetism shown to be controllable on ultrafast femtosecond time scales. Here, by employing laser light consisting of both linear and circular pulses, we show that charge of specified spin and crystal momentum can be created with precision throughout the first Brillouin zone. Our hybrid pulses induce in a controlled way both adiabatic intraband motion as well as vertical interband excitation between valence and conduction bands, and require only a gapped spin split valley structure for their implementation. This scenario is commonly found in the 2d semi-conductors, and we demonstrate our approach with monolayer WSe$_2$. We thus establish a route from laser light to local control over excitations in reciprocal space, opening the way to the preparation of momenta specified excited states at ultrafast time scales.
We analyze the laws of conservation of momentum and angular momentum in classical electrodynamics of material media with bound charges, and explore the possibility to describe the properties of such media via a discrete set of point-like charges of zero size (as imposed by special relativity), and via continuous charge/current distributions. This way we put a question: do we have to recognize the infinite fields at the location of elementary charges as the essential physical requirement, or such infinite fields can be ignored via introduction of continuous charge distribution? In order to answer this question, we consider the interaction of a homogeneously charged insulating plate with a compact magnetic dipole, moving along the plate. We arrive at the apparent violation of the angular momentum conservation law and show that this law is re-covered, when the electric field at the location of each elementary charge of the plate is taken infinite. This result signifies that the description of electromagnetic properties of material media via the continuous charge and current distributions is not a universal approximation, and at the fundamental level, we have to deal with a system of elementary discrete charges of zero size, at least in the analysis of laws of conservation of momentum and angular momentum.
We demonstrate the quantized transfer of photon energy and transverse momentum to a high-coherence electron beam. In an ultrafast transmission electron microscope, a three-dimensional phase modulation of the electron wavefunction is induced by transmitting the beam through a laser-illuminated thin graphite sheet. This all-optical free-electron phase space control results in high-purity superpositions of linear momentum states, providing an elementary component for optically programmable electron phase plates and beam splitters.
Very recent experiments have discovered that localized light in strongly absorbing media displays intriguing diffusive phenomena. Here we develop a first-principles theory of light propagation in open media with arbitrary absorption strength and sample length. We show analytically that photons in localized open absorbing media exhibit unusual Brownian motion. Specifically, wave transport follows the diffusion equation with the diffusion coefficient exhibiting spatial resolution. Most strikingly, despite that the system is controlled by two parameters -- the ratio of the localization (absorption) length to the sample length -- the spatially resolved diffusion coefficient displays novel single parameter scaling: it depends on the space via the returning probability. Our analytic predictions for this diffusion coefficient are confirmed by numerical simulations. In the strong absorption limit they agree well with the experimental results.
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