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Register a new userHigh-purity free-electron momentum states prepared by three-dimensional optical phase modulation
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We demonstrate the quantized transfer of photon energy and transverse momentum to a high-coherence electron beam. In an ultrafast transmission electron microscope, a three-dimensional phase modulation of the electron wavefunction is induced by transmitting the beam through a laser-illuminated thin graphite sheet. This all-optical free-electron phase space control results in high-purity superpositions of linear momentum states, providing an elementary component for optically programmable electron phase plates and beam splitters.
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Levitated nanodiamonds containing nitrogen vacancy centres in high vacuum are a potential test bed for numerous phenomena in fundamental physics. However, experiments so far have been limited to low vacuum due to heating arising from optical absorption of the trapping laser. We show that milling pure diamond creates nanodiamonds that do not heat up as the optical intensity is raised above 700 GW/m$^2$ below 5 mbar of pressure. This advance now means that the level of attainable vacuum for nanodiamonds in optical dipole traps is no longer temperature limited.
High-dimensional entangled states are promising candidates for increasing the security and encoding capacity of quantum systems. While it is possible to witness and set bounds for the entanglement, precisely quantifying the dimensionality and purity in a fast and accurate manner remains an open challenge. Here, we report an approach that simultaneously returns the dimensionality and purity of high-dimensional entangled states by simple projective measurements. We show that the outcome of a conditional measurement returns a visibility that scales monotonically with entanglement dimensionality and purity, allowing for quantitative measurements for general photonic quantum systems. We illustrate our method using transverse spatial modes of photons that carry orbital angular momentum and verify high-dimensional entanglement over a wide range of state purities. Our approach advances the high-dimensional tool box for characterising quantum states by providing a simple and direct dimensionality and purity measure, even for mixed entangled states.
Nonlinear metasurfaces that dynamically manipulate the phase of a passing light beam are of interest for a wide range of applications. The controlled operation of such devices requires accurate measurements of the optical transmission phase in both the linear and nonlinear regime, an experimentally challenging task. In this paper we show that this phase information can be extracted directly from simple transmission measurements, using a Hilbert transform approach, removing the need for complicated, interferometric experimental set-ups, and enabling direct measurements of the phase in conditions not suitable for other traditional approaches, such Z-scan measurements.
Van der Waals heterostructures have been lately intensively studied because they offer a large variety of properties that can be controlled by selecting 2D materials and their sequence in the stack. The exact arrangement of the layers as well as the exact arrangement of the atoms within the layers, both are important for the properties of the resulting device. Recently it has been demonstrated that convergent beam electron diffraction (CBED) allows quantitative three-dimensional mapping of atomic positions in three-dimensional materials from a single CBED pattern. In this study we investigate CBED in more detail by simulating and performing various CBED regimes, with convergent and divergent wavefronts, on a somewhat simplified system: a 2D monolayer crystal. In CBED, each CBED spot is in fact an in-line hologram of the sample, where in-line holography is known to exhibit high intensity contrast in detection of weak phase objects that are not detectable in conventional in-focus imaging mode. Adsorbates exhibit strong intensity contrast in zero and higher order CBED spots, whereas lattice deformation such as strain or rippling cause noticeable intensity contrast only in the first and higher order CBED spots. The individual CBED spots can be reconstructed as typical in-line holograms, and the resolution of 2.13 A can be in principle achieved in the reconstructions. We provide simulated and experimental examples of CBED of a 2D monolayer crystal. The simulations show that individual CBED spots can be treated as in-line holograms and sample distributions such as adsorbates, can be reconstructed. Individual atoms can be reconstructed from a single CBED pattern provided the later exhibits high-order CBED spots. Examples of reconstructions obtained from experimental CBED patterns, at a resolution of 2.7 A, are shown.
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