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Register a new userObservation of two-level critical state in the superconducting FeTe thin films
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FeTe, a non-superconducting parent compound in the iron-chalcogenide family, becomes superconducting after annealing in oxygen. Under the presence of magnetism, spin-orbit coupling, inhomogeneity and lattice distortion, the nature of its superconductivity is not well understood. Here, we combined mutual inductance technique with magneto transport to study the magnetization and superconductivity of FeTe thin films. We found that the films with the highest Tc showed non-saturating superfluid density and a strong magnetic hysteresis distinct from that in a homogeneous superconductor. Such hysteresis can be well explained by a two-level critical state model and suggested the importance of granularity to superconductivity in this compound.
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The Hall effect is investigated in thin-film samples of iron-chalcogenide superconductors in detail. The Hall coefficient (RH) of FeTe and Fe(Se1-xTex) exhibits a similar positive value around 300 K, indicating that the high-temperature normal state is dominated by hole-channel transport. FeTe exhibits a sign reversal from positive to negative across the transition to the low-temperature antiferromagnetic state, indicating the occurrence of drastic reconstruction in the band structure. The mobility analysis using the carrier density theoretically calculated reveals that the mobility of holes is strongly suppressed to zero, and hence the electric transport looks to be dominated by electrons. The Se substitution to Te suppresses the antiferromagnetic long-range order and induces superconductivity instead. The similar mobility analysis for Fe(Se0.4Te0.6) and Fe(Se0.5Te0.5) thin films shows that the mobility of electrons increases with decreasing temperature even in the paramagnetic state, and keeps sufficiently high values down to the superconducting transition temperature. From the comparison between FeTe and Fe(Se1-xTex), it is suggested that the coexistence of itinerant carriers both in electron and hole channels is indispensable for the occurrence of superconductivity.
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