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Register a new userSingle-pass, second harmonic generation of ultrafast, higher order vector vortex beams at blue
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We report a novel experimental scheme for single-pass second harmonic generation (SHG) of vector vortex beam in the blue. Using an ultrafast Ti:Sapphire laser of pulse width ~17 fs and a set of spiral phase plates in polarization based Mach-Zehnder interferometer (MZI) we have generated vector vortex beams of order as high as lp = 12 at an average power of 860 mW. Given the space-variant polarization of the vector vortex beam, and the dependence of nonlinear frequency conversion processes on the polarization of the interacting beams, using two contiguous bismuth borate crystals with optic axis orthogonal to each other, we have frequency-doubled the near-IR vector vortex beam into visible vector vortex beams with order as high as lsh=24. The maximum output power of the vector vortex beam of order, lsh =2 is measured be as high as 20.5 mW at a single-pass SHG efficiency of 2.4 %. Controlling the temporal delay in the MZI, we have preserved the vector vortex nature of the beams at both pump and frequency-doubled beams at ultrafast timescales. The measurement on mode purity confirms the generation of high quality vector vortex beams at pump and SHG wavelengths. The generic experimental scheme can be used to generate vector vortex beams across the electromagnetic spectrum.
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Harnessing the spontaneous emission of incoherent quantum emitters is one of the hallmarks of nano-optics. Yet, an enduring challenge remains-making them emit vector beams, which are complex forms of light associated with fruitful developments in fluorescence imaging, optical trapping and high-speed telecommunications. Vector beams are characterized by spatially varying polarization states whose construction requires coherence properties that are typically possessed by lasers-but not by photons produced by spontaneous emission. Here, we show a route to weave the spontaneous emission of an ensemble of colloidal quantum dots into vector beams. To this end, we use holographic nanostructures that impart the necessary spatial coherence, polarization and topological properties to the light originating from the emitters. We focus our demonstration on vector vortex beams, which are chiral vector beams carrying non-zero orbital angular momentum, and argue that our approach can be extended to other forms of vectorial light.
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