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Spontaneous Emission of Vector Vortex Beams

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 Added by Aloyse Degiron
 Publication date 2021
  fields Physics
and research's language is English




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Harnessing the spontaneous emission of incoherent quantum emitters is one of the hallmarks of nano-optics. Yet, an enduring challenge remains-making them emit vector beams, which are complex forms of light associated with fruitful developments in fluorescence imaging, optical trapping and high-speed telecommunications. Vector beams are characterized by spatially varying polarization states whose construction requires coherence properties that are typically possessed by lasers-but not by photons produced by spontaneous emission. Here, we show a route to weave the spontaneous emission of an ensemble of colloidal quantum dots into vector beams. To this end, we use holographic nanostructures that impart the necessary spatial coherence, polarization and topological properties to the light originating from the emitters. We focus our demonstration on vector vortex beams, which are chiral vector beams carrying non-zero orbital angular momentum, and argue that our approach can be extended to other forms of vectorial light.



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The spontaneous emergence of vector vortex beams with non-uniform polarization distribution is reported in a vertical-cavity surface-emitting laser (VCSEL) with frequency-selective feedback. Antivortices with a hyperbolic polarization structure and radially polarized vortices are demonstrated. They exist close to and partially coexist with vortices with uniform and non-uniform polarization distributions characterized by four domains of pairwise orthogonal polarization. The spontaneous formation of these nontrivial structures in a simple, nearly isotropic VCSEL system is remarkable and the vector vortices are argued to have soliton-like properties.
Vector vortex beams have played a fundamental role in the better understanding of coherence and polarization. They are described by spatially inhomogeneous polarization states, which present a rich optical mode structure that has attracted much attention for applications in optical communications, imaging, spectroscopy and metrology. However, this complex mode structure can be quite detrimental when propagation effects such as turbulence and birefringence perturb the beam. Optical phase conjugation has been proposed as a method to recover an optical beam from perturbations. Here we demonstrate full phase conjugation of vector vortex beams using three-wave mixing. Our scheme exploits a fast non-linear process that can be conveniently controlled via the pump beam. Our results pave the way for sophisticated, practical applications of vector beams.
Creating high-quality vector vortex (VV) beams is possible with a myriad of techniques at low power, and while a few studies have produced such beams at high-power, none have considered the impact of amplification on the vector purity. Here we employ novel tools to study the amplification of VV beams, and in particular the purity of such modes. We outline a general toolbox for such investigations and demonstrate its use in the general case of VV beams through a birefringent gain medium. Intriguingly, we show that it is possible to enhance the purity of such beams during amplification, paving the way for high-brightness VV beams, a requirement for their use in high-power applications such as laser materials processing.
Optical singularities manifesting at the center of vector vortex beams are unstable, since their topological charge is higher than the lowest value permitted by Maxwells equations. Inspired by conceptually similar phenomena occurring in the polarization pattern characterizing the skylight, we show how perturbations that break the symmetry of radially symmetric vector beams lead to the formation of a pair of fundamental and stable singularities, i.e. points of circular polarization. We prepare a superposition of a radial (or azimuthal) vector beam and a uniformly linearly polarized Gaussian beam; by varying the amplitudes of the two fields, we control the formation of pairs of these singular points and their spatial separation. We complete this study by applying the same analysis to vector vortex beams with higher topological charges, and by investigating the features that arise when increasing the intensity of the Gaussian term. Our results can find application in the context of singularimetry, where weak fields are measured by considering them as perturbation of unstable optical beams.
Perfect vortex beams are the orbital angular momentum (OAM)-carrying beams with fixed annular intensities, which provide a better source of OAM than traditional Laguerre- Gaussian beams. However, ordinary schemes to obtain the perfect vortex beams are usually bulky and unstable. We demonstrate here a novel generation scheme by designing planar Pancharatnam-Berry (PB) phase elements to replace all the elements required. Different from the conventional approaches based on reflective or refractive elements, PB phase elements can dramatically reduce the occupying volume of system. Moreover, the PB phase element scheme is easily developed to produce the perfect vector beams. Therefore, our scheme may provide prominent vortex and vector sources for integrated optical communication and micromanipulation systems.
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