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Register a new user17,000 %/W Second Harmonic Conversion Efficiency in Single Crystalline Aluminum Nitride Microresonators
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High quality factor optical microcavities have been employed in a variety of material systems to enhance nonlinear optical interactions. While single-crystalline aluminum nitride microresonators have recently emerged as a low loss platform for integrated nonlinear optics such as four wave mixing and Raman lasing, few studies have investigated this material for second-harmonic generation. In this Letter, we demonstrate an optimized fabrication of dually-resonant phase-matched ring resonators from epitaxial aluminum nitride thin films. An unprecendented second-harmonic generation efficiency of 17,000%/W is obtained in the low power regime and pump depletion is observed at a relatively low input power of 3.5 mW. This poses epitaxial aluminum nitride as the highest efficiency second-harmonic generator among current integrated platforms.
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The second-harmonic generation process of a focused laser beam inside a nonlinear crystal is described by the Boyd-Kleinman theory. Calculating the actual conversion efficiency and upconverted power requires the solution of a double integral that is analytically intractable. We provide an expression that predicts the exact gain coefficient within an error margin of less than 2% over several orders of magnitude of the confocal parameter and as a function of the walk-off parameter. Our result allows for readily tuning the beam parameters to optimize the performance of the upconversion process and improve optical system designs.
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