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Light Yield of Perovskite Nanocrystal-Doped Liquid Scintillator

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 Added by Lindley Winslow
 Publication date 2018
  fields Physics
and research's language is English




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Liquid scintillators doped with metals are needed for a variety of measurements in nuclear and particle physics. Nanoparticles provide a mechanism to dope the scintillator and their unique optical properties could be used to enhance detection capabilities. We present here the first study of lead-based perovskite nanoparticles for this application. Perovskites are an attractive choice due to the versatility of their crystal structure and their ease of synthesis.



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Liquid scintillator detectors are widely used in modern neutrino studies. The unique optical properties of semiconducting nanocrystals, known as quantum dots, offer intriguing possibilities for improving standard liquid scintillator, especially when combined with new photodetection technology. Quantum dots also provide a means to dope scintillator with candidate isotopes for neutrinoless double beta decay searches. In this work, the first studies of the scintillation properties of quantum-dot-doped liquid scintillator using both UV light and radioactive sources are presented.
359 - D.E. Fields , R. Gibbons , M. Gold 2020
Scintillation from noble gases is an important technique in particle physics including neutrino beam experiments, neutrino-less double beta-decay and dark matter searches. In liquid argon, the possibility of enhancing the light yield by the addition of a small quantity of xenon (doping at 10-1000 ppm) has been of particular interest. While the pathway for energy transfer between argon and xenon excimers is well known, the time-dependence of the process has not been fully studied in the context of a physics-based model. In this paper we present a model of the energy transfer process together with a fit to xenon-doped argon data. We have measured the diffusion limited rate constant as a function of xenon dopant. We find that the time dependence of the energy transfer is consistent with diffusion-limited reactions. Additionally, we find that commercially obtained argon can have a small xenon component (4 ppm). Our result will facilitate the use of xenon-doped liquid argon in future experiments.
The experimental efforts characterizing the era of precision neutrino physics revolve around collecting high-statistics neutrino samples and attaining an excellent energy and position resolution. Next generation liquid-based neutrino detectors, such as JUNO, HyperKamiokande, etc, share the use of a large target mass, and the need of pushing light collection to the edge for maximal calorimetric information. Achieving high light collection implies considerable costs, especially when considering detector masses of several kt. A traditional strategy to maximize the effective photo-coverage with the minimum number of PMTs relies on Light Concentrators (LC), such as Winston Cones. In this paper, the authors introduce a novel concept called Occulting Light Concentrators (OLC), whereby a traditional LC gets tailored to a conventional PMT, by taking into account its single-photoelectron collection efficiency profile and thus occulting the worst performing portion of the photocathode. Thus, the OLC shape optimization takes into account not only the optical interface of the PMT, but also the maximization of the PMT detection performances. The light collection uniformity across the detector is another advantage of the OLC system. By considering the case of JUNO, we will show OLC capabilities in terms of light collection and energy resolution.
This paper presents studies of the performance of water-based liquid scintillator in both 1-kt and 50-kt detectors. Performance is evaluated in comparison to both pure water Cherenkov detectors and a nominal model for pure scintillator detectors. Performance metrics include energy, vertex, and angular resolution, along with a metric for ability to separate the Cherenkov from the scintillation signal, as being representative of various particle identification capabilities that depend on the Cherenkov / scintillation ratio. We also modify the time profile of scintillation light to study the same performance metrics as a function of rise and decay time. We go on to interpret these results in terms of their impact on certain physics goals, such as solar neutrinos and the search for Majorana neutrinos. This work supports and validates previous results, and the assumptions made therein, by using a more complete detector model and full reconstruction. We confirm that a high-coverage, 50-kt detector would be capable of better than 10 (1)% precision on the CNO neutrino flux with a WbLS (pure LS) target in 5 years of data taking. A 1-kt LS detector, with a conservative 50% fiducial volume of 500~t, can achieve a better than 5% detection. Using the liquid scintillator model, we find a sensitivity into the normal hierarchy region for Majorana neutrinos, with half life sensitivity of $T^{0 ubetabeta}_{1/2} > 1.4 times 10^{28}$ years at 90% CL for 10 years of data taking with a Te-loaded target.
257 - Lindley Winslow 2013
Liquid-scintillator-based detectors are a robust technology that scales well to large volumes. For this reason, they are attractive for experiments searching for neutrinoless double-beta decay. A combination of improved photo-detection technology and novel liquid scintillators may allow for the extraction of particle direction in addition to the total energy of the particle. Such an advance would find applications beyond searches for neutrinoless double-beta decay.
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