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A Kinetic Model for Xenon-Doped Liquid Argon Scintillation Light

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 Added by Michael Gold
 Publication date 2020
  fields Physics
and research's language is English




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Scintillation from noble gases is an important technique in particle physics including neutrino beam experiments, neutrino-less double beta-decay and dark matter searches. In liquid argon, the possibility of enhancing the light yield by the addition of a small quantity of xenon (doping at 10-1000 ppm) has been of particular interest. While the pathway for energy transfer between argon and xenon excimers is well known, the time-dependence of the process has not been fully studied in the context of a physics-based model. In this paper we present a model of the energy transfer process together with a fit to xenon-doped argon data. We have measured the diffusion limited rate constant as a function of xenon dopant. We find that the time dependence of the energy transfer is consistent with diffusion-limited reactions. Additionally, we find that commercially obtained argon can have a small xenon component (4 ppm). Our result will facilitate the use of xenon-doped liquid argon in future experiments.

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Xenon-doped liquid argon has been proposed as a good alternative to pure liquid argon in scintillation detectors. In this study, we report on the measurement of the time profile of scintillation light emitted from xenon-doped liquid argon with molar concentrations up to 1600 ppm. A compact setup has been developed for this study, with silicon photomultiplier (SiPM) as the photosensor and $^{210}mathrm{Po}$ and $^{90}mathrm{Sr}$ as scintillation sources. An effective model based on the de-excitation processes has been developed to describe the data. The results show that xenon-doped liquid argon is a good fast scintillator and can be used in lieu of tetraphenyl butadiene (TPB) in a way that preserves its capability for particle identification via pulse shape discrimination (PSD).
The use of xenon-doped liquid argon is a promising alternative for large pure liquid-argon TPCs. Not only xenon-doped liquid argon enhances the light production, mitigating the possible suppression due to impurities, but also it increases the wavelength of the scintillation light, enlarging the effective Rayleigh scattering length and improving the detection uniformity. ProtoDUNE Dual-Phase is a 300-ton active volume LAr TPC, a prototype for the Deep Underground Neutrino Experiment (DUNE), a dual-site experiment for long-baseline neutrino oscillation studies, neutrino astrophysics and nucleon decay searches. ProtoDUNE Dual-Phase took cosmic muon data at CERN with pure liquid argon and with xenon-doped liquid argon for over a year. The impact of the presence of xenon in the scintillation light and its comparison with the pure liquid argon data will be presented. These results are of interest to any future large LAr TPCs.
130 - Ettore Segreto 2020
Liquid argon is used as active medium in a variety of neutrino and Dark Matter experiments thanks to its excellent properties of charge yield and transport and as a scintillator. Liquid argon scintillation photons are emitted in a narrow band of 10~nm centered around 127 nm and with a characteristic time profile made by two components originated by the decay of the lowest lying singlet and triplet state of the excimer Ar$_2^*$ to the dissociative ground state. A model is proposed which takes into account the quenching of the long lived triplet states through the self-interaction with other triplet states or through the interaction with molecular Ar$_2^+$ ions. The model predicts the time profile of the scintillation signals and its dependence on the intensity of an external electric field and on the density of deposited energy, if the relative abundance of the unquenched fast and slow components is know. The model successfully explains the experimentally observed dependence of the characteristic time of the slow component on the intensity of the applied electric field and the increase of photon yield of liquid argon when doped with small quantities of xenon (at the ppm level). The model also predicts the dependence of the pulse shape parameter, F$_{prompt}$, for electron and nuclear recoils on the recoil energy and the behavior of the relative light yield of nuclear recoils in liquid argon, $mathcal{L}_{eff}$
117 - E. Aprile 2005
We have studied the feasibility of a silicon photomultiplier (SiPM) to detect liquid xenon (LXe) scintillation light. The SiPM was operated inside a small volume of pure LXe, at -95 degree Celsius, irradiated with an internal Am-241 alpha source. The gain of the SiPM at this temperature was estimated to be 1.8 x 10^6 with bias voltage at 52 V. Based on the geometry of the setup, the quantum efficiency of the SiPM was estimated to be 22% at the Xe wavelength of 178 nm. The low excess noise factor, high single photoelectron detection efficiency, and low bias voltage of SiPMs make them attractive alternative UV photon detection devices to photomultiplier tubes (PMTs) for liquid xenon detectors, especially for experiments requiring a very low energy detection threshold, such as neutralino dark matter searches.
110 - K. Ni , E. Aprile , K.L. Giboni 2006
Scintillation light from gamma ray irradiation in liquid xenon is detected by two Hamamatsu R9288 photomultiplier tubes (PMTs) immersed in the liquid. UV light reflector material, PTFE, is used to optimize the light collection efficiency. The detector gives a high light yield of 6 photoelectron per keV (pe/keV), which allows efficient detection of the 122 keV gamma-ray line from Co-57, with a measured energy resolution of (8.8+/-0.6)% (sigma). The best achievable energy resolution, by removing the instrumental fluctuations, from liquid xenon scintillation light is estimated to be around 6-8% (sigma) for gamma-ray with energy between 662 keV and 122 keV.
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