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Register a new userEffect of Cr spacer on structural and magnetic properties of Fe/Gd multilayers
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In this work we analyse the role of a thin Cr spacer between Fe and Gd layers on structure and magnetic properties of a [Fe(35A)/Cr(tCr)/Gd(50A)/Cr(tCr)]x12 superlattice. Samples without the Cr spacer (tCr=0) and with a thin tCr=4A are investigated using X-ray diffraction, polarized neutron and resonance X-ray magnetic reflectometry, SQUID magnetometery, magneto-optical Kerr effect and ferromagnetic resonance techniques. Magnetic properties are studied experimentally in a wide temperature range 4-300K and analysed theoretically using numerical simulation on the basis of the mean-field model. We show that a reasonable agreement with the experimental data can be obtained considering temperature dependence of the effective field parameter in gadolinium layers. The analysis of the experimental data shows that besides a strong reduction of the antiferromagnetic coupling between Fe and Gd, the introduction of Cr spacers into Fe/Gd superlattice leads to modification of both structural and magnetic characteristics of the ferromagnetic layers.
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The dynamic response of dipole skyrmions in Fe/Gd multilayer films is investigated by ferromagnetic resonance measurements and compared to micromagnetic simulations. We detail thickness and temperature dependent studies of the observed modes as well as the effects of magnetic field history on the resonant spectra. Correlation between the modes and the magnetic phase maps constructed from real-space imaging and scattering patterns allows us to conclude the resonant modes arise from local topological features such as dipole skyrmions but does not depend on the collective response of a closed packed lattice of these chiral textures. Using, micromagnetic modeling, we are able to quantitatively reproduce our experimental observations which suggests the existence of localized spin-wave modes that are dependent on the helicity of the dipole skyrmion. We identify four localized spin wave excitations for the skyrmions that are excited under either in-plane or out-of-plane r.f. fields. Lastly we show that dipole skyrmions and non-chiral bubble domains exhibit qualitatively different localized spin wave modes.
Results of magnetization, magnetotransport and Mossbauer spectroscopy measurements of sequentially evaporated Fe-Ag granular composites are presented. The strong magnetic scattering of the conduction electrons is reflected in the sublinear temperature dependence of the resistance and in the large negative magnetoresistance. The simultaneous analysis of the magnetic properties and the transport behavior suggests a bimodal grain size distribution. A detailed quantitative description of the unusual features observed in the transport properties is given.
[Co/Ni] multilayers with perpendicular magnetic anisotropy (PMA) have been researched and applied in various spintronic applications. Typically the seed layer material is studied to provide the desired face-centered cubic (textit{fcc}) texture to the [Co/Ni] to obtain PMA. The integration of [Co/Ni] in back-end-of-line (BEOL) processes also requires the PMA to survive post-annealing. In this paper, the impact of NiCr, Pt, Ru, and Ta seed layers on the structural and magnetic properties of [Co(0.3 nm)/Ni(0.6 nm)] multilayers is investigated before and after annealing. The multilayers were deposited textit{in-situ} on different seeds via physical vapor deposition at room temperature. The as-deposited [Co/Ni] films show the required textit{fcc}(111) texture on all seeds, but PMA is only observed on Pt and Ru. In-plane magnetic anisotropy (IMA) is obtained on NiCr and Ta seeds, which is attributed to strain-induced PMA loss. PMA is maintained on all seeds after post-annealing up to 400$^{circ}$C. The largest effective perpendicular anisotropy energy ($K_U^{mathrm{eff}}approx 2times10^5$J/m$^3$) after annealing is achieved on NiCr seed. The evolution of PMA upon annealing cannot be explained by further crystallization during annealing or strain-induced PMA, nor can the observed magnetization loss and the increased damping after annealing. Here we identify the diffusion of the non-magnetic materials from the seed into [Co/Ni] as the major driver of the changes in the magnetic properties. By selecting the seed and post-annealing temperature, the [Co/Ni] can be tuned in a broad range for both PMA and damping.
In recent years, there has been an intense interest in understanding the microscopic mechanism of thermally induced magnetization switching driven by a femtosecond laser pulse. Most of the effort has been dedicated to periodic crystalline structures while the amorphous counterparts have been less studied. By using a multiscale approach, i.e. first-principles density functional theory combined with atomistic spin dynamics, we report here on the very intricate structural and magnetic nature of amorphous Gd-Fe alloys for a wide range of Gd and Fe atomic concentrations at the nanoscale level. Both structural and dynamical properties of Gd-Fe alloys reported in this work are in good agreement with previous experiments. We calculated the dynamic behavior of homogeneous and inhomogeneous amorphous Gd-Fe alloys and their response under the influence of a femtosecond laser pulse. In the homogeneous sample, the Fe sublattice switches its magnetization before the Gd one. However, the temporal sequence of the switching of the two sublattices is reversed in the inhomogeneous sample. We propose a possible explanation based on a mechanism driven by a combination of the Dzyaloshiskii-Moriya interaction and exchange frustration, modeled by an antiferromagnetic second-neighbour exchange interaction between Gd atoms in the Gd-rich region. We also report on the influence of laser fluence and damping effects in the all-thermal switching.
The effect of substituting iron and zinc for cobalt in CaBaCo$_4$O$_7$ has been investigated using neutron diffraction and x-ray absorption spectroscopy. The orthorhombic distortion present in the parent compound CaBaCo$_4$O$_7$ decreases with increasing the content of either Fe or Zn. The samples CaBaCo$_3$ZnO$_7$ and CaBaCo$_{4-x}$Fe$_x$O$_7$ with $x leq 1.5$ are metrically hexagonal but much better refinements in the neutron diffraction patterns are obtained using an orthorhombic unit cell. The two types of substitution have opposite effects on the structural and magnetic properties. Fe atoms preferentially occupy the sites at the triangular layer. Thus, the replacement of Co by Fe supresses the ferrimagnetic ordering and CaBaCo$_{4-x}$Fe$_x$O$_7$ samples are antiferromagnetically ordered with a new propagation vector k=(1/3,0,0). However, the Zn atoms prefer occupying the Kagome layer, which is very detrimental for the long range magnetic interactions giving rise to a magnetic glass. The oxidation state of iron and zinc is found to be 3+ and 2+, respectively, independently of the content. Therefore, the average Co oxidation state changes accordingly with the Fe$^{3+}$ or Zn$^{2+}$ doping. Also, x-ray absorption spectroscopy data confirms the different preferential occupation for both Fe and Zn cations. The combined information obtained by neutron diffraction and x-ray absorption spectroscopy indicates that cobalt atoms can be either in a fluctuating Co$^{2+}$/Co$^{3+}$ valence state or, alternatively, Co$^{2+}$ and Co$^{3+}$ ions being randomly distributed in the lattice. These results explain the occurrence of local disorder in the CoO$_4$ tetrahedra obtained by EXAFS. An anomaly in the lattice parameters and an increase in the local disorder is observed only at the ferrimagnetic transition for CaBaCo$_4$O$_7$ revealing the occurrence of local magneto-elastic coupling.
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