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Register a new userMollow triplet: pump probe single photon spectroscopy of artificial atoms
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We analyze a photon transport through an 1D open waveguide side coupled to the $N$-photon microwave cavity with embedded artificial two- level atom (qubit). The qubit state is probed by a weak signal at the fundamental frequency of the waveguide. Within the formalism of projection operators and non-Hermitian Hamiltonian approach we develop a one-photon approximation scheme to obtain the photon wavefunction which allows for the calculation of the probability amplitudes of the spontaneous transitions between the levels of two Rabi doublets in $N$- photon cavity. We obtain analytic expressions for the transmission and reflection factors of the microwave signal through a waveguide, which contain the information of the qubit parameters. We show that for small number of cavity photons the Mollow spectrum consists of four spectral lines which is a direct manifestation of quantum nature of light. The results obtained in the paper are of general nature and can be applied to any type of qubits. The specific properties of the qubit are only encoded in the two parameters: the energy $Omega$ of the qubit and its coupling $lambda$ to the cavity photons.
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We study the dressed states of 3He atoms and experimentally observe the Mollow triplet (MT) induced with an ultra-low-frequency (ULF) oscillating magnetic field as low as 4 Hz. The ULF MT signatures from the ground states of 3He atoms are transferred to the metastable states by metastability-exchange collisions (MECs) and measured optically, which demonstrates 2 s coherence time in the dressed ground states. The result shows the possibility of ULF magnetic field amplitude measurement and a new scheme for optical frequency modulation.
A theoretical frame for pump-probe photoemission is presented. The approach is based on a general formulation using the Keldysh formalism for the lesser Greens function to describe the real-time evolution of the electronic degrees of freedom in the initial state after a strong pump pulse that drives the system out of equilibrium. The final state is represented by a time-reversed low-energy electron diffraction state. Our one-step description is related to Pendrys original formulation of the photoemission process as close as possible. The formalism allows for a quantitative calculation of time-dependent photocurrent for simple metals where a picture of effectively independent electrons is assumed as reliable. The theory is worked out for valence- and core-electron excitations. It comprises the study of different relativistic effects as a function of the pump-probe delay.
We present magnetization measurements on the single molecule magnet Fe8 in the presence of pulsed microwave radiation. A pump-probe technique is used with two microwave pulses with frequencies of 107 GHz and 118 GHz and pulse lengths of several nanoseconds to study the spin dynamics via time-resolved magnetization measurements using a Hall probe magnetometer. We find evidence for short spin-phonon relaxation times of the order of one microsecond. The temperature dependence of the spin-phonon relaxation time in our experiments is in good agreement with previously published theoretical results. We also established the presence of very short energy diffusion times, that act on a timescale of about 70 ns.
In high-resolution core-valence-valence (CVV) Auger electron spectroscopy from the surface of a solid at thermal equilibrium, the main correlation satellite, visible in the case of strong valence-electron correlations, corresponds to a bound state of the two holes in the final state of the CVV Auger process. We discuss the physical significance of this satellite in nonequilibrium pump-probe Auger spectroscopy by numerical analysis of a single-band Hubbard-type model system including core states and a continuum of high-energy scattering states. It turns out that the spectrum of the photo-doped system, due to the increased double occupancy, shares features with the equilibrium spectrum at higher fillings. The pumping of doublons can be watched when working with overlapping pulses at short $Delta t$. For larger pump-probe delays $Delta t$ and on the typical femtosecond time scale for electronic relaxation processes, spectra are hardly $Delta t$-dependent, reflecting the high stability of bound two-hole states for strong Hubbard-$U$. We argue that taking into account the spatial expansion of single-particle orbitals when these are doubly occupied, as described by the dynamical Hubbard model, produces an oscillation of the barycenter of the satellite as a function of $Delta t$. Pump-probe Auger-electron spectroscopy is thus highly sensitive to dynamical screening of the Coulomb interaction.
Robust engineering of phonon squeezed states in optically excited solids has emerged as a promising tool to control and manipulate their properties. However, in contrast to quantum optical systems, detection of phonon squeezing is subtle and elusive, and an important question is what constitutes an unambiguous signature of it. The state of the art involves observing oscillations at twice the phonon frequency in time resolved measurements of the out of equilibrium phonon fluctuation. Using Keldysh formalism we show that such a signal is a necessary but not a sufficient signature of a squeezed phonon, since we identify several mechanisms that do not involve squeezing and yet which produce similar oscillations. We show that a reliable detection requires a time and frequency resolved measurement of the phonon spectral function.
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