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Mesoscopic superconductivity and high spin polarization coexisting at metallic point contacts on the Weyl semimetal TaAs

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 Publication date 2016
  fields Physics
and research's language is English




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A Weyl semimetal is a topologically non-trivial phase of matter that hosts mass-less Weyl fermions, the particles that remained elusive for more than 80 years since their theoretical discovery. The Weyl semimetals exhibit unique transport and magneto-transport properties and remarkably high surface spin polarization. Here we show that a unique mesoscopic superconducting phase with a critical temperature up to 7 K can be realized by forming metallic point contacts with silver (Ag) on single crystals of TaAs, while neither Ag nor TaAs are superconductors. The Andreev reflection spectra obtained from such point contacts are fitted well within a modified Blonder-Tinkham-Klapwijk (BTK) model with a superconducting energy gap up to 1.2 meV. The analysis within this model also reveals high transport spin polarization up to 60% indicating a spin polarized supercurrent flowing through the point contacts on TaAs. Such point contacts also show a large anisotropic magnetoresistance (AMR) originating from the spin polarized current. Therefore, apart from the discovery of a novel mesoscopic superconducting phase and its coexistence with a large spin polarization, our results also show that the point contacts on Weyl semimetals are potentially important for applications in spintronics.



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Recently, Wang $et$ $al.$ have reported the observation of unconventional superconductivity in the Weyl semimetal TaAs [arXiv:1607.00513]. The authors have written textit{A conductance plateau and sharp double dips are observed in the point contact spectra, indicating p-wave like unconventional superconductivity. Furthermore, the zero bias conductance peak in low temperature regime is detected, suggesting potentially the existence of Majorana zero modes. The experimentally observed tunneling spectra can be interpreted with a novel mirror-symmetry protected topological superconductor induced in TaAs, which can exhibit zero bias and double finite bias peaks, and double conductance dips in the measurements}. In this comment we show that for a superconducting point contact, the features like a zero-bias conductance peak, a plateau and single or multiple conductance dips might arise due to simple contact-heating related effects. Such features are routinely observed in point contacts involving a wide variety of superconductors when the experiments are not performed in the right regime of mesoscopic transport. We also show that the data presented by Wang $et$ $al.$ in a single transport regime of point contact do not confirm tip induced superconductivity (TISC). Even if it is assumed that Wang $et$ $al.$ achieved TISC on TaAs, all the spectra that they have reported show striking similarities with the type of spectra expected in thermal regime of transport. Such data cannot be used for extracting any spectroscopic information and based on such data any discussion on p-wave superconductivity or the emergence of Majorana modes should be considered invalid. This version (v2) also includes a brief discussion on the response of Wang $et$ $al.$ to the first version (v1) of this comment. Correct ballistic regime data on TaAs point contacts can be found in arXiv:1607.05131 (2016).
The motivation to search for signatures of superconductivity in Weyl semi-metals and other topological phases lies in their potential for hosting exotic phenomena such as nonzero-momentum pairing or the Majorana fermion, a viable candidate for the ultimate realization of a scalable quantum computer. Until now, however, all known reports of superconductivity in Weyl semimetals have arisen through surface contact with a sharp tip, focused ion-beam surface treatment or the application of high pressures. Here, we demonstrate the observation of superconductivity in single crystals, even an as-grown crystal, of the Weyl semi-metal tantalum phosphide (TaP), at ambient pressure. A superconducting transition temperature, $Tc$, varying between 1.7 and 5.3 K, is observed in different samples, both as-grown and microscopic samples processed with focused ion beam (FIB) etching. Our data show that the superconductivity present in the as-grown crystal is inhomogeneous yet exists in the bulk. For samples fabricated with FIB, we observe, in addition to the bulk superconductivity, a second superconducting state that resides on the sample surface. Through measurements of the characteristic fields as a function of temperature and angle, we are able to confirm the dimensionality of the two distinct superconducting phases.
247 - B. Q. Lv , H. M. Weng , B. B. Fu 2015
Weyl semimetals are a class of materials that can be regarded as three-dimensional analogs of graphene breaking time reversal or inversion symmetry. Electrons in a Weyl semimetal behave as Weyl fermions, which have many exotic properties, such as chiral anomaly and magnetic monopoles in the crystal momentum space. The surface state of a Weyl semimetal displays pairs of entangled Fermi arcs at two opposite surfaces. However, the existence of Weyl semimetals has not yet been proved experimentally. Here we report the experimental realization of a Weyl semimetal in TaAs by observing Fermi arcs formed by its surface states using angle-resolved photoemission spectroscopy. Our first-principles calculations, matching remarkably well with the experimental results, further confirm that TaAs is a Weyl semimetal.
We present a study of the Andreev reflections in superconductor/ferromagnet nanostructured point contacts. The experimental data are analyzed in the frame of a model with two spin-dependent transmission coefficients for the majority and minority charge carriers in the ferromagnet. This model consistently describes the whole set of conductance measurements as a function of voltage, temperature, and magnetic field. The ensemble of our results shows that the degree of spin polarization of the current can be unambiguously determined using Andreev physics.
Since the three dimensional (3D) Dirac semi-metal Cd$_3$As$_2$ exists close to topological phase boundaries, in principle it should be possible to drive it into exotic new phases, like topological superconductors, by breaking certain symmetries. Here we show that the mesoscopic point-contacts between silver (Ag) and Cd$_3$As$_2$ exhibit superconductivity up to a critical temperature (onset) of 6 K while neither Cd$_3$As$_2$ nor Ag are superconductors. A gap amplitude of 6.5 meV is measured spectroscopically in this phase that varies weakly with temperature and survives up to a remarkably high temperature of 13 K indicating the presence of a robust normal-state pseudogap. The observations indicate the emergence of a new unconventional superconducting phase that exists only in a quantum mechanically confined region under a point-contact between a Dirac semi-metal and a normal metal.
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