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Late Time Emission of Prompt Fission Gamma Rays

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 Added by Patrick Talou
 Publication date 2016
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and research's language is English




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The emission of prompt fission $gamma$ rays within a few nanoseconds to a few microseconds following the scission point is studied in the Hauser-Feshbach formalism applied to the deexcitation of primary excited fission fragments. Neutron and $gamma$-ray evaporations from fully accelerated fission fragments are calculated in competition at each stage of the decay, and the role of isomers in the fission products, before $beta$-decay, is analyzed. The time evolution of the average total $gamma$-ray energy, average total $gamma$-ray multiplicity, and fragment-specific $gamma$-ray spectra, is presented in the case of neutron-induced fission reactions of $^{235}$U and $^{239}$Pu, as well as spontaneous fission of $^{252}$Cf. The production of specific isomeric states is calculated and compared to available experimental data. About 7% of all prompt fission $gamma$ rays are predicted to be emitted between 10 nsec and 5 $mu$sec following fission, in the case of $^{235}$U and $^{239}$Pu $(n_{rm th},f)$ reactions, and up to 3% in the case of $^{252}$Cf spontaneous fission. The cumulative average total $gamma$-ray energy increases by 2 to 5% in the same time interval. Finally, those results are shown to be robust against significant changes in the model input parameters.



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175 - A.E. Lovell , I. Stetcu , P. Talou 2019
We propose a novel method to extract the prompt neutron multiplicity distribution, $P( u)$, in fission reactions based on correlations between prompt neutrons, $gamma$ rays, and fragment kinetic energy arising from energy conservation. In this approach, only event-by-event measurements of the total $gamma$-ray energy released as a function of the total kinetic energy (TKE) of the fission fragments are performed, and no neutron detection is required. Using the $texttt{CGMF}$ fission event generator, we illustrate the method and explore the accuracy of extracting the neutron multiplicity distribution when taking into account the energy resolution and calibration of the energy measurements. We find that a TKE resolution of under 2 MeV produces reasonably accurate results, independent of typical $gamma$-ray energy measurement resolution.
589 - P. Talou , R. Vogt , J. Randrup 2017
Detailed information on the fission process can be inferred from the observation, modeling and theoretical understanding of prompt fission neutron and $gamma$-ray~observables. Beyond simple average quantities, the study of distributions and correlations in prompt data, e.g., multiplicity-dependent neutron and gray~spectra, angular distributions of the emitted particles, $n$-$n$, $n$-$gamma$, and $gamma$-$gamma$~correlations, can place stringent constraints on fission models and parameters that would otherwise be free to be tuned separately to represent individual fission observables. The FREYA~and CGMF~codes have been developed to follow the sequential emissions of prompt neutrons and $gamma$-rays~from the initial excited fission fragments produced right after scission. Both codes implement Monte Carlo techniques to sample initial fission fragment configurations in mass, charge and kinetic energy and sample probabilities of neutron and $gamma$~emission at each stage of the decay. This approach naturally leads to using simple but powerful statistical techniques to infer distributions and correlations among many observables and model parameters. The comparison of model calculations with experimental data provides a rich arena for testing various nuclear physics models such as those related to the nuclear structure and level densities of neutron-rich nuclei, the $gamma$-ray~strength functions of dipole and quadrupole transitions, the mechanism for dividing the excitation energy between the two nascent fragments near scission, and the mechanisms behind the production of angular momentum in the fragments, etc. Beyond the obvious interest from a fundamental physics point of view, such studies are also important for addressing data needs in various nuclear applications. (See text for full abstract.)
213 - D. B. Ion 2011
In this paper we presented a short review of radioactive halos as from the perspective of their interpretation as integral record in time of different kind of known or unknown radioactivities. A special attention is paid for the unified interpretation of the supergiant halos (SGH), discovered by Grady, Walker and Laemlein, as integral record of pion emission during fission.
252 - I. Stetcu , A.E. Lovell , P. Talou 2021
We investigate the angular momentum removal from fission fragments (FFs) through neutron and $gamma$-ray emission, where we find that about half the neutrons are emitted with angular momenta $ge 1.5hbar$ and that the change in angular momentum after the emission of neutrons and statistical $gamma$ rays is significant, contradicting usual assumptions. Per fission event, in our simulations, the neutron and statistical $gamma$-ray emissions change the spin of the fragment by 3.5 -- 5~$hbar$, with a large standard deviation comparable to the average value. Such wide angular momentum removal distributions can hide any underlying correlations in the fission fragment initial spin values. Within our model, we reproduce data on spin measurements from discrete transitions after neutron emissions, especially in the case of light FFs. The agreement further improves for the heavy fragments if one removes from the analysis the events that would produce isomeric states. Finally, we show that while in our model the initial FF spins do not follow a saw-tooth like behavior observed in recent measurements, the average FF spin computed after neutron and statistical $gamma$ emissions exhibits a shape that resembles a saw tooth. This suggests that the average FF spin measured after statistical emissions is not necessarily connected with the scission mechanism as previously implied.
While Josephson-like junctions, transiently established in heavy ion collisions ($tau_{coll}approx10^{-21}$ s) between superfluid nuclei --through which Cooper pair tunneling ($Q$-value $Q_{2n}$) proceeds mainly in terms of successive transfer of entangled nucleons-- is deprived from the macroscopic aspects of a supercurrent, it displays many of the special effects associated with spontaneous symmetry breaking in gauge space (BCS condensation), which can be studied in terms of individual quantum states and of tunneling of single Cooper pairs. From the results of studies of one- and two- neutron transfer reactions carried out at energies below the Coulomb barrier we estimate the value of the mean square radius (correlation length) of the nuclear Cooper pair. A quantity related to the largest distance of closest approach for which the absolute two-nucleon tunneling cross section is of the order of the single-particle one. Furthermore, emission of $gamma$-rays of (Josephson) frequency $ u_J=Q_{2n}/h$ distributed over an energy range $hbar/tau_{coll}$ is predicted.
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