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Correlated Prompt Fission Data in Transport Simulations

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 Added by Ramona Vogt
 Publication date 2017
  fields
and research's language is English




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Detailed information on the fission process can be inferred from the observation, modeling and theoretical understanding of prompt fission neutron and $gamma$-ray~observables. Beyond simple average quantities, the study of distributions and correlations in prompt data, e.g., multiplicity-dependent neutron and gray~spectra, angular distributions of the emitted particles, $n$-$n$, $n$-$gamma$, and $gamma$-$gamma$~correlations, can place stringent constraints on fission models and parameters that would otherwise be free to be tuned separately to represent individual fission observables. The FREYA~and CGMF~codes have been developed to follow the sequential emissions of prompt neutrons and $gamma$-rays~from the initial excited fission fragments produced right after scission. Both codes implement Monte Carlo techniques to sample initial fission fragment configurations in mass, charge and kinetic energy and sample probabilities of neutron and $gamma$~emission at each stage of the decay. This approach naturally leads to using simple but powerful statistical techniques to infer distributions and correlations among many observables and model parameters. The comparison of model calculations with experimental data provides a rich arena for testing various nuclear physics models such as those related to the nuclear structure and level densities of neutron-rich nuclei, the $gamma$-ray~strength functions of dipole and quadrupole transitions, the mechanism for dividing the excitation energy between the two nascent fragments near scission, and the mechanisms behind the production of angular momentum in the fragments, etc. Beyond the obvious interest from a fundamental physics point of view, such studies are also important for addressing data needs in various nuclear applications. (See text for full abstract.)

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447 - P. Talou , T. Kawano , I. Stetcu 2016
The emission of prompt fission $gamma$ rays within a few nanoseconds to a few microseconds following the scission point is studied in the Hauser-Feshbach formalism applied to the deexcitation of primary excited fission fragments. Neutron and $gamma$-ray evaporations from fully accelerated fission fragments are calculated in competition at each stage of the decay, and the role of isomers in the fission products, before $beta$-decay, is analyzed. The time evolution of the average total $gamma$-ray energy, average total $gamma$-ray multiplicity, and fragment-specific $gamma$-ray spectra, is presented in the case of neutron-induced fission reactions of $^{235}$U and $^{239}$Pu, as well as spontaneous fission of $^{252}$Cf. The production of specific isomeric states is calculated and compared to available experimental data. About 7% of all prompt fission $gamma$ rays are predicted to be emitted between 10 nsec and 5 $mu$sec following fission, in the case of $^{235}$U and $^{239}$Pu $(n_{rm th},f)$ reactions, and up to 3% in the case of $^{252}$Cf spontaneous fission. The cumulative average total $gamma$-ray energy increases by 2 to 5% in the same time interval. Finally, those results are shown to be robust against significant changes in the model input parameters.
175 - A.E. Lovell , I. Stetcu , P. Talou 2019
We propose a novel method to extract the prompt neutron multiplicity distribution, $P( u)$, in fission reactions based on correlations between prompt neutrons, $gamma$ rays, and fragment kinetic energy arising from energy conservation. In this approach, only event-by-event measurements of the total $gamma$-ray energy released as a function of the total kinetic energy (TKE) of the fission fragments are performed, and no neutron detection is required. Using the $texttt{CGMF}$ fission event generator, we illustrate the method and explore the accuracy of extracting the neutron multiplicity distribution when taking into account the energy resolution and calibration of the energy measurements. We find that a TKE resolution of under 2 MeV produces reasonably accurate results, independent of typical $gamma$-ray energy measurement resolution.
314 - A.E. Lovell , P. Talou , I. Stetcu 2020
Several sources of angular anisotropy for fission fragments and prompt neutrons have been studied in neutron-induced fission reactions. These include kinematic recoils of the target from the incident neutron beam and the fragments from the emission of the prompt neutrons, preferential directions of the emission of the fission fragments with respect to the beam axis due to the population of particular transition states at the fission barrier, and forward-peaked angular distributions of pre-equilibrium neutrons which are emitted before the formation of a compound nucleus. In addition, there are several potential sources of angular anisotropies that are more difficult to disentangle: the angular distributions of prompt neutrons from fully accelerated fragments or from scission neutrons, and the emission of neutrons from fission fragments that are not fully accelerated. In this work, we study the effects of the first group of anisotropy sources, particularly exploring the correlations between the fission fragment anisotropy and the resulting neutron anisotropy. While kinematic effects were already accounted for in our Hauser-Feshbach Monte Carlo code, $mathtt{CGMF}$, anisotropic angular distributions for the fission fragments and pre-equilibrium neutrons resulting from neutron-induced fission on $^{233,234,235,238}$U, $^{239,241}$Pu, and $^{237}$Np have been introduced for the first time. The effects of these sources of anisotropy are examined over a range of incident neutron energies, from thermal to 20 MeV, and compared to experimental data from the Chi-Nu liquid scintillator array. The anisotropy of the fission fragments is reflected in the anisotropy of the prompt neutrons, especially as the outgoing energy of the prompt neutrons increases, allowing for an extraction of the fission fragment anisotropy to be made from a measurement of the neutrons.
Simulations by transport codes are indispensable to extract valuable physics information from heavy ion collisions. In order to understand the origins of discrepancies between different widely used transport codes, we compare 15 such codes under controlled conditions of a system confined to a box with periodic boundary, initialized with Fermi-Dirac distributions at saturation density and temperatures of either 0 or 5 MeV. In such calculations, one is able to check separately the different ingredients of a transport code. In this second publication of the code evaluation project, we only consider the two-body collision term, i.e. we perform cascade calculations. When the Pauli blocking is artificially suppressed, the collision rates are found to be consistent for most codes (to within $1%$ or better) with analytical results, or completely controlled results of a basic cascade code after eliminating the correlations within the same pair of colliding particles. In calculations with active Pauli blocking, the blocking probability was found to deviate from the expected reference values. The reason is found in substantial phase-space fluctuations and smearing tied to numerical algorithms and model assumptions in the representation of phase space. This results in the reduction of the blocking probability in most transport codes, so that the simulated system gradually evolves away from the Fermi-Dirac towards a Boltzmann distribution. As a result of this investigation, we are able to make judgements about the most effective strategies in transport simulations for determining the collision probabilities and the Pauli blocking. Investigation in a similar vein of other ingredients in transport calculations, like the mean field propagation or the production of nucleon resonances and mesons, will be discussed in the future publications.
We suggest a small set of fission observables to be used as test cases for validation of theoretical calculations. The purpose is to provide common data to facilitate the comparison of different fission theories and models. The proposed observables are chosen from fission barriers, spontaneous fission lifetimes, fission yield characteristics, and fission isomer excitation energies.
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