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Register a new userEnhancement of interfacial thermal conductance of SiC by overlapped carbon nanotubes and intertube atoms
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We proposed a new way, adding intertube atoms, to enhance interfacial thermal conductance (ITC) between SiC-carbon nanotube (CNT) array structure. Non-equilibrium molecular dynamics method was used to study the ITC. The results show that the intertube atoms can significantly enhance the ITC. The dependence of ITC on both the temperature and the number of intertube atoms are shown. The mechanism is analyzed by calculating probability distributions of atomic forces and vibrational density of states. Our study may provide some guidance on enhancing the ITC of CNT-based composites.
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Exploring the mechanism of interfacial thermal transport and reducing the interfacial thermal resistance is of great importance for thermal management and modulation. Herein, the interfacial thermal resistance between overlapped graphene nanoribbons is largely reduced by adding bonded carbon chains by performing molecular dynamics simulations. And the analytical model (cross-interface model, CIM) is utilized to analyze and explain the two-dimensional thermal transport mechanism at cross-interface. An order of magnitude reduction in interfacial thermal resistance is found as the graphene nanoribbons are bonded by just one carbon chain. Interestingly, the decreasing rate of interfacial thermal resistance slows down gradually with the increasing of the number of carbon chains, which can be explained by the proposed theoretical relationship based on CIM. Moreover, by the comparison of CIM and traditional simplified model, the accuracy of CIM is verified and demonstrated in overlapped graphene nanoribbons. This work provides a new way to improve the interfacial thermal transport and reveal the essential mechanism for low-dimensional materials applied in thermal management.
We have calculated the effects of structural distortions of armchair carbon nanotubes on their electrical transport properties. We found that the bending of the nanotubes decreases their transmission function in certain energy ranges and leads to an increased electrical resistance. Electronic structure calculations show that these energy ranges contain localized states with significant $sigma$-$pi$ hybridization resulting from the increased curvature produced by bending. Our calculations of the contact resistance show that the large contact resistances observed for SWNTs are likely due to the weak coupling of the NT to the metal in side bonded NT-metal configurations.
We use DFT to study the effect of molecular adsorbates on the conductance of metallic carbon nanotubes. The five molecules considered (NO2, NH2, H, COOH, OH) lead to similar scattering of the electrons. The adsorption of a single molecule suppresses one of the two available channels of the CNT at low bias conductance. If more molecules are adsorbed on the same sublattice, the remaining open channel can be blocked or not, depending on the relative position of the adsorbates. If a simple geometric condition is fulfilled this channel is still open, even after adsorbing an arbitrary number of molecules.
The quest for non-Abelian quasiparticles has inspired decades of experimental and theoretical efforts, where the scarcity of direct probes poses a key challenge. Among their clearest signatures is a thermal Hall conductance with quantized half-integer value in natural units $ pi^2 k_B^2 T /3 h$ ($T$ is temperature, $h$ the Planck constant, $k_B$ the Boltzmann constant). Such a value was indeed recently observed in a quantum-Hall system and a magnetic insulator. We show that a non-topological thermal metal phase that forms due to quenched disorder may disguise as a non-Abelian phase by well approximating the trademark quantized thermal Hall response. Remarkably, the quantization here improves with temperature, in contrast to fully gapped systems. We provide numerical evidence for this effect and discuss its possible implications for the aforementioned experiments.
We have prepared solutions of multiwalled carbon nanotubes in Aroclor 1254, a mixture of polychlorinated biphenyls. The solutions are stable at room temperature. Transport measurements were performed using a scanning--tunneling probe on a sample prepared by spin--coating of the solution on gold substrates. Conductance steps were clearly seen. An histogram of a high number of traces shows maximum peaks at integer values of the conductance quantum $G_0 = 2e^2/h$, demonstrating ballistic transport at room temperature along the carbon nanotube over distances longer than $1.4mu m$.
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