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Terahertz emission from multiple-microcavity exciton-polariton lasers

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 Added by Simon Huppert
 Publication date 2014
  fields Physics
and research's language is English




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Terahertz emission between exciton-polariton branches in semiconductor microcavities is expected to be strongly stimulated in the polariton laser regime, due to the high density of particles in the lower state (final state stimulation effect). However, non-radiative scattering processes depopulate the upper state and greatly hinder the efficiency of such terahertz sources. In this work, we suggest a new scheme using multiple microcavities and exploiting the transition between two interband polariton branches located below the exciton level. We compare the non-radiative processes loss rates in single and double cavity devices and we show that a dramatic reduction can be achieved in the latter, enhancing the efficiency of the terahertz emission.



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Interactions of few-cycle terahertz pulses with the induced optical polarization in a quantum-well microcavity reveal that the lower and higher exciton-polariton modes together with the optically forbidden 2p-exciton state form a unique {Lambda}-type three-level system. Pronounced nonlinearities are observed via time-resolved strong-terahertz and weak-optical excitation spectroscopy and explained with a fully microscopic theory. The results show that the terahertz pulses strongly couple the exciton-polariton states to the 2p-exciton state while no resonant transition between the two polariton levels is observed.
We study a system of microcavity pillars arranged into a kagome lattice. We show that polarization-dependent tunnel coupling of microcavity pillars leads to the emergence of the effective spin-orbit interaction consisting of the Dresselhaus and Rashba terms, similar to the case of polaritonic graphene studied earlier. Appearance of the effective spin-orbit interaction combined with the time-reversal symmetry-breaking resulting from the application of the magnetic field leads to the nontrivial topological properties of the Bloch bundles of polaritonic wavefunction. These are manifested in opening of the gap in the band structure and topological edge states localized on the boundary. Such states are analogs of the edge states arising in topological insulators. Our study of polarization properties of the edge states clearly demonstrate that opening of the gap is associated with the band inversion in the region of the Dirac points of the Brillouin zone where the two bands corresponding to polaritons of opposite polarizations meet. For one particular type of boundary we observe a highly nonlinear energy dispersion of the edge state which makes polaritonic kagome lattice a promising system for observation of edge state solitons.
We have performed real and momentum space spin-dependent spectroscopy of spontaneously formed exciton polariton condensates for a non-resonant pumping scheme. Under linearly polarized pump, our results can be understood in terms of spin-dependent Boltzmann equations in a two-state model. This suggests that relaxation into the ground state occurs after multiple phonon scattering events and only one polariton-polariton scattering. For the circular pumping case, in which only excitons of one spin are injected, a bottleneck effect is observed, implying inefficient relaxation.
Topological insulators (TIs) are a striking example of materials in which topological invariants are manifested in robustness against perturbations. Their most prominent feature is the emergence of topological edge states with reduced dimension at the boundary between areas with distinct topological invariants. The observable physical effect is unidirectional robust transport, unaffected by defects or disorder. TIs were originally observed in the integer quantum Hall effect for fermionic systems of correlated electrons. However, during the past decade the concepts of topological physics have been introduced into numerous fields beyond condensed matter, ranging from microwaves and photonic systems to cold atoms, acoustics and even mechanics. Recently, TIs were proposed in exciton-polariton systems organized as honeycomb lattices, under the influence of a magnetic field. Topological phenomena in polaritons are fundamentally different from all topological effects demonstrated experimentally thus far: exciton-polaritons are part-light part-matter quasiparticles emerging from the strong coupling of quantum well excitons and cavity photons. Here, we demonstrate experimentally the first exciton-polariton TI. This constitutes the first symbiotic light-matter TIs. Our polariton lattice is excited non-resonantly, and the chiral topological polariton edge mode is populated by a polariton condensation mechanism. We image real- and Fourier-space to measure photoluminescence, and demonstrate that the topological edge mode avoids defects, and that the propagation direction of the mode can be reversed by inverting the applied magnetic field. Our exciton-polariton TI paves the way for a variety of new topological phenomena, as they involve light-matter interaction, gain, and perhaps most importantly - exciton-polaritons interact with one another as a nonlinear many-body system.
We studied the intensity of resonant Raman scattering due to optical phonons in a planar II-VI-type semiconductor microcavity in the regime of strong coupling between light and matter. Two different sets of independent experiments were performed at near outgoing resonance with the middle polariton (MP)branch of the cavity. In the first, the Stokes-shifted photons were kept at exact resonance with the MP, varying the photonic or excitonic character of the polariton. In the second, only the incoming light wavelength was varied, and the resonant profile of the inelastic scattered intensity was studied when the system was tuned out of the resonant condition. Taking some matrix elements as free parameters, both independent experiments are quantitatively described by a model which incorporates lifetime effects in both excitons and photons, and the coupling of the cavity photons to the electron-hole continuum. The model is solved using a Greens function approach which treats the exciton-photon coupling nonperturbatively.
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