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Register a new userQuasiparticle-continuum level repulsion in a quantum magnet
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When the energy eigenvalues of two coupled quantum states approach each other in a certain parameter space, their energy levels repel each other and level crossing is avoided. Such level repulsion, or avoided level crossing, is commonly used to describe the dispersion relation of quasiparticles in solids. However, little is known about the level repulsion when more than two quasiparticles are present; for example, in an open quantum system where a quasiparticle can spontaneously decay into many particle continuum. Here we show that even in this case level repulsion exists between a long-lived quasiparticle state and a continuum. In our fine resolution neutron spectroscopy study of magnetic quasiparticles in a frustrated quantum magnet BiCu2PO6, we observe a renormalization of quasiparticle dispersion relation due to the presence of the continuum of multi-quasiparticle states. Our results have a broadimplication for understanding open quantum systems described by non-hermitian Hamiltonian.
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Magnetic systems composed of weakly coupled spin-1/2 chains are fertile ground for hosting the fractional magnetic excitations that are intrinsic to interacting fermions in one-dimension (1D). However, the exotic physics arising from the quantum many-body interactions beyond 1D are poorly understood in materials of this class. Spinons and psinons are two mutually exclusive low-energy magnetic quasiparticles; the excitation seen depends on the ground state of the spin chain. Here, we present inelastic neutron scattering and neutron diffraction evidence for their coexistence in SrCo$_{2}$V$_{2}$O$_{8}$ at milli-Kelvin temperatures in part of the Neel phase (2.4 T $leq$ $mu_mathrm{{0}}$H $<$ 3.9 T) and possibly also the field-induced spin density wave phase up to the highest field probed ($mu_mathrm{{0}}$H $geq$ 3.9 T, $mu_mathrm{{0}}$H$_mathbf{mathrm{{max}}}$ = 5.5 T). These results unveil a novel spatial phase inhomogeneity for the weakly coupled spin chains in this compound. This quantum dynamical phase separation is a new phenomenon in quasi-1D quantum magnets, highlighting the non-trivial consequences of inter-chain coupling.
Conventional crystalline magnets are characterized by symmetry breaking and normal modes of excitation called magnons with quantized angular momentum $hbar$. Neutron scattering correspondingly features extra magnetic Bragg diffraction at low temperatures and dispersive inelastic scattering associated with single magnon creation and annihilation. Exceptions are anticipated in so-called quantum spin liquids as exemplified by the one-dimensional spin-1/2 chain which has no magnetic order and where magnons accordingly fractionalize into spinons with angular momentum $hbar/2$. This is spectacularly revealed by a continuum of inelastic neutron scattering associated with two-spinon processes and the absence of magnetic Bragg diffraction. Here, we report evidence for these same key features of a quantum spin liquid in the three-dimensional Heisenberg antiferromagnet NaCaNi$_2$F$_7$. Through specific heat and neutron scattering measurements, Monte Carlo simulations, and analytic approximations to the equal time correlations, we show that NaCaNi$_2$F$_7$ is an almost ideal realization of the spin-1 antiferromagnetic Heisenberg model on a pyrochlore lattice with weak connectivity and frustrated interactions. Magnetic Bragg diffraction is absent and 90% of the spectral weight forms a continuum of magnetic scattering not dissimilar to that of the spin-1/2 chain but with low energy pinch points indicating NaCaNi$_2$F$_7$ is in a Coulomb phase. The residual entropy and diffuse elastic scattering points to an exotic state of matter driven by frustration, quantum fluctuations and weak exchange disorder.
A family of spin-orbit coupled honeycomb Mott insulators offers a playground to search for quantum spin liquids (QSLs) via bond-dependent interactions. In candidate materials, a symmetric off-diagonal $Gamma$ term, close cousin of Kitaev interaction, has emerged as another source of frustration that is essential for complete understanding of these systems. However, the ground state of honeycomb $Gamma$ model remains elusive, with a suggested zigzag magnetic order. Here we attempt to resolve the puzzle by perturbing the $Gamma$ region with a staggered Heisenberg interaction which favours the zigzag ordering. Despite such favour, we find a wide disordered region inclusive of the $Gamma$ limit in the phase diagram. Further, this phase exhibits a vanishing energy gap, a collapse of excitation spectrum, and a logarithmic entanglement entropy scaling on long cylinders, indicating a gapless QSL. Other quantities such as plaquette-plaquette correlation are also discussed.
We identify a large family of ground states of a topological Skyrmion magnet whose classical degeneracy persists to all orders in a semiclassical expansion. This goes along with an exceptional robustness of the concomitant ground state configurations, which are not at all dressed by quantum fluctuations. We trace these twin observations back to a common root: this class of topological ground states saturates a Bogomolny inequality. A similar phenomenology occurs in high-energy physics for some field theories exhibiting supersymmetry. We propose quantum Hall ferromagnets, where these Skyrmions configurations arise naturally as ground states away from integer filling, as the best available laboratory realisations.
The discovery of massless Dirac electrons in graphene and topological Dirac-Weyl materials has prompted a broad search for bosonic analogues of such Dirac particles. Recent experiments have found evidence for Dirac magnons above an Ising-like ferromagnetic ground state in a two-dimensional (2D) kagome lattice magnet and in the van der Waals layered honeycomb crystal CrI$_3$, and in a 3D Heisenberg magnet Cu$_3$TeO$_6$. Here we report on our inelastic neutron scattering investigation on large single crystals of a stacked honeycomb lattice magnet CoTiO$_3$, which is part of a broad family of ilmenite materials. The magnetically ordered ground state of CoTiO$_3$ features ferromagnetic layers of Co$^{2+}$, stacked antiferromagnetically along the $c$-axis. We discover that the magnon dispersion relation exhibits strong easy-plane exchange anisotropy and hosts a clear gapless Dirac cone along the edge of the 3D Brillouin zone. Our results establish CoTiO$_3$ as a model pseudospin-$1/2$ material to study interacting Dirac bosons in a 3D quantum XY magnet.
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