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Register a new userDirac magnons in a honeycomb lattice quantum XY magnet CoTiO3
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The discovery of massless Dirac electrons in graphene and topological Dirac-Weyl materials has prompted a broad search for bosonic analogues of such Dirac particles. Recent experiments have found evidence for Dirac magnons above an Ising-like ferromagnetic ground state in a two-dimensional (2D) kagome lattice magnet and in the van der Waals layered honeycomb crystal CrI$_3$, and in a 3D Heisenberg magnet Cu$_3$TeO$_6$. Here we report on our inelastic neutron scattering investigation on large single crystals of a stacked honeycomb lattice magnet CoTiO$_3$, which is part of a broad family of ilmenite materials. The magnetically ordered ground state of CoTiO$_3$ features ferromagnetic layers of Co$^{2+}$, stacked antiferromagnetically along the $c$-axis. We discover that the magnon dispersion relation exhibits strong easy-plane exchange anisotropy and hosts a clear gapless Dirac cone along the edge of the 3D Brillouin zone. Our results establish CoTiO$_3$ as a model pseudospin-$1/2$ material to study interacting Dirac bosons in a 3D quantum XY magnet.
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We examine the presence and evolution of magnetic Dirac nodes in the Heisenberg honeycomb lattice. Using linear spin theory, we evaluate the collinear phase diagram as well as the change in the spin dynamics with various exchange interactions. We show that the ferromagnetic structure produces bosonic Dirac and Weyl points due to the competition between superexchange interactions. Furthermore, it is shown that the criteria for magnetic Dirac nodes are coupled to the magnetic structure and not the overall crystal symmetry, where the breaking of inversion symmetry greatly affects the antiferromagnetic configurations. The tunability of the nodal points through variation of the exchange parameters leads to the possibility of controlling Dirac symmetries through an external manipulation of the orbital interactions.
A family of spin-orbit coupled honeycomb Mott insulators offers a playground to search for quantum spin liquids (QSLs) via bond-dependent interactions. In candidate materials, a symmetric off-diagonal $Gamma$ term, close cousin of Kitaev interaction, has emerged as another source of frustration that is essential for complete understanding of these systems. However, the ground state of honeycomb $Gamma$ model remains elusive, with a suggested zigzag magnetic order. Here we attempt to resolve the puzzle by perturbing the $Gamma$ region with a staggered Heisenberg interaction which favours the zigzag ordering. Despite such favour, we find a wide disordered region inclusive of the $Gamma$ limit in the phase diagram. Further, this phase exhibits a vanishing energy gap, a collapse of excitation spectrum, and a logarithmic entanglement entropy scaling on long cylinders, indicating a gapless QSL. Other quantities such as plaquette-plaquette correlation are also discussed.
The study of magnonic thermal Hall effect has recently attracted attention because this effect can be associated with topological phases activated by Dzyaloshinskii-Moriya interaction, which acts similar to a spin-orbital coupling in an electronic system. A topological phase transition may arise when there exist two or more distinct topological phases, and this transition is often revealed by a gap closing. In this work, we consider a ferromagnetic honeycomb lattice described by a Hamiltonian that contains Heisenberg exchange interaction, Dzyaloshinskii-Moriya interaction, and an applied Zeeman field. When expanding the spin operators in the Hamiltonian using Holstein-Primakoff (HP) transformation to the order of $S^{1/2}$, where $S$ is the magnitude of spin, the thermal Hall conductivity stays negative for all values of parameters such as the strength of Zeeman interaction and temperature. However, we demonstrate in this work that by including the next order, $S^{-1/2}$, in HP transformation to take into account magnon-magnon interaction, the Hartree type of interaction gives rise to topological phase transitions driven by temperature. When the temperature increases, we find that the gap of the magnonic energy spectrum closes at Dirac points at a critical temperature, $T_c$, and the gap-closing is indeed the signature for a topological phase transition as confirmed by showing that the Chern numbers are distinct above and below $T_c$. Finally, our analysis points out that thermal Hall conductivity exhibits sign reversal at the same temperature. This phenomenon can be used in experiments to verify the topological nature of magnons in honeycomb magnets.
We study the spin-1 honeycomb lattice magnets with frustrated exchange interactions. The proposed microscopic spin model contains first and second neighbor Heisenberg interactions as well as the single-ion anisotropy. We establish a rich phase diagram that includes a featureless quantum paramagnet and various spin spiral states induced by the mechanism of order by quantum disorder. Although the quantum paramagnet is dubbed featureless, it is shown that, the magnetic excitations develop a contour degeneracy in the reciprocal space at the band minima. These contour degenerate excitations are responsible for the frustrated criticality from the quantum paramagnet to the ordered phases. This work illustrates the effects of magnetic frustration on both magnetic orderings and the magnetic excitations. We discuss the experimental relevance to various Ni-based honeycomb lattice magnets.
We have investigated spin-wave excitations in a four-sublattice (4SL) magnetic ground state of a frustrated magnet CuFeO2, in which `electromagnon (electric-field-active magnon) excitation has been discovered by recent terahertz time-domain spectroscopy [Seki et al. Phys. Rev. Lett. 105 097207 (2010)]. In previous study, we have identified two spin-wave branches in the 4SL phase by means of inelastic neutron scattering measurements under applied uniaxial pressure. [T. Nakajima et al. J. Phys. Soc. Jpn. 80 014714 (2011) ] In the present study, we have performed high-energy-resolution inelastic neutron scattering measurements in the 4SL phase, resolving fine structures of the lower-energy spin-wave branch near the zone center. Taking account of the spin-driven lattice distortions in the 4SL phase, we have developed a model Hamiltonian to describe the spin-wave excitations. The determined Hamiltonian parameters have successfully reproduced the spin-wave dispersion relations and intensity maps obtained in the inelastic neutron scattering measurements. The results of the spin-wave analysis have also revealed physical pictures of the magnon and electromagnon modes in the 4SL phase, suggesting that collinear and noncollinear characters of the two spin-wave modes are the keys to understand the dynamical coupling between the spins and electric dipole moments in this system.
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