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Register a new userLarge gap, a pseudogap and proximity effect in the Bi2Te3/Fe1+yTe interfacial superconductor
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We report directional point-contact spectroscopy data on the novel Bi2Te3/Fe1+yTe interfacial superconductor for a Bi2Te3 thickness of 9 quintuple layers, bonded by van der Waals epitaxy to a Fe1+yTe film at an atomically sharp interface. Our data show a very large superconducting twin-gap structure with an energy scale exceeding that of bulk FeSe or FeSe1-xTex by a factor of 4. While the larger gap is isotropic and attributed to a thin FeTe layer in proximity of the interface, the smaller gap has a pronounced anisotropy and is associated with proximity-induced superconductivity in the topological insulator Bi2Te3. Zero resistance is lost above 8 K, but superconducting fluctuations are visible up to at least 12 K and the large gap is replaced by a pseudogap that persists up to 40 K. The spectra show a pronounced zero-bias conductance peak in the superconducting state, which may be a signature of an unconventional pairing mechanism.
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We investigate the hydrostatic pressure dependence of interfacial superconductivity occurring at the atomically sharp interface between two non-superconducting materials: the topological insulator (TI) Bi2Te3 and the parent compound Fe1+yTe of the chalcogenide iron based superconductors. Under pressure, a significant increase in the superconducting transition temperature Tc is observed. We trace the pressure dependence of a superconducting twin gap structure by Andreev reflection point contact spectroscopy (PCARS), which shows that a large superconducting gap associated with the interfacial superconductivity increases along with Tc. A second smaller gap, which is attributed to proximity-induced superconductivity in the TI layer, increases first, but then reaches a maximum and appears to be gradually suppressed at higher pressure. We interpret our data in the context of a pressure-induced doping effect of the interface, in which charge is transferred from the TI layer to the interface and the interfacial superconductivity is enhanced. This demonstrates the important role of the TI in the interfacial superconductivity mechanism.
The recent discovery of the interfacial superconductivity (SC) of the Bi2Te3/Fe1+yTe heterostructure has attracted extensive studies due to its potential as a novel platform for trapping and controlling Majorana fermions. Here we present studies of another topological insulator (TI)/Fe1+yTe heterostructure, Sb2Te3/Fe1+yTe, which also enjoys an interfacial two-dimensional SC. The results of transport measurements support that the reduction of excess Fe concentration of the Fe1+yTe layer not only increases the fluctuation of its antiferromagnetic (AFM) order but also enhances the quality of the SC of this heterostructure system. On the other hand, the interfacial SC of this heterostructure was found to have a wider-ranging TI-layer thickness dependence than that of the Bi2Te3/Fe1+yTe heterostructure, which is believed to be attributed to the much higher bulk conductivity of Sb2Te3 that enhances indirect coupling between its top and bottom topological surface states (TSSs). Our results provide the evidence of the interplay among the AFM order, itinerant carries from the TSSs and the induced interfacial SC of the TI/Fe1+yTe heterostructure system.
We report on temperature-dependent soft X-ray absorption spectroscopy (XAS) measurements utilizing linearly polarized synchrotron radiation to probe magnetic phase transitions in iron-rich Fe1+yTe. X-ray magnetic linear dichroism (XMLD) signals, which sense magnetic ordering processes at surfaces, start to increase monotonically below the Neel temperature TN = 57 K. This increase is due to a progressive bicollinear antiferromagnetic (AFM) alignment of Fe spins of the monoclinic Fe1+yTe parent phase. This AFM alignment was achieved by a [100]-oriented biasing field favoring a single-domain state during cooling across TN. Our specific heat and magnetization measurements confirm the bulk character of this AFM phase transition. On longer time scales, however, we observe that the field-biased AFM state is highly unstable even at the lowest temperature of T = 3 K. After switching off the biasing field, the XMLD signal decays exponentially with a time constant {tau} = 1506 s. The initial XMLD signal is restored only upon repeating a cycle consisting of heating and field-cooling through TN. We explain the time effect by a gradual formation of a multi-domain state with 90 deg rotated AFM domains, promoted by structural disorder, facilitating the motion of twin-domains. Significant disorder in our Fe1+yTe sample is evident from our X-ray diffraction and specific heat data. The stability of magnetic phases in Fe-chalcogenides is an important material property, since the Fe(Te1-xSex) phase diagram shows magnetism intimately connected with superconductivity.
The magnetization in a superconductor induced due to the inverse proximity effect is investigated in hybrid bilayers containing a superconductor and a ferromagnetic insulator or a strongly spin-polarized ferromagnetic metal. The study is performed within a quasiclassical Green function framework, wherein Usadel equations are solved with boundary conditions appropriate for strongly spin-polarized ferromagnetic materials. A comparison with recent experimental data is presented. The singlet to triplet conversion of the superconducting correlations as a result of the proximity effect with a ferromagnet is studied.
Measurements of the polar Kerr effect using a zero-area-loop Sagnac magnetometer on Pb/Ni and Al/(Co-Pd) proximity-effect bilayers show unambiguous evidence for the inverse proximity effect, in which the ferromagnet (F) induces a finite magnetization in the superconducting (S) layer. To avoid probing the magnetic effects in the ferromagnet, the superconducting layer was prepared much thicker than the lights optical penetration depth. The sign and size of the effect, as well as its temperature dependence agree with recent predictions by Bergeret et al..
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