Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userDisorder-induced time effect in the antiferromagnetic domain state of Fe1+yTe
156
0
0.0
(
0
)
Added by
Jan Fik\\'a\\v{c}ek
Publication date
2021
fields
Physics
and research's language is
English
Ask ChatGPT about the research
No Arabic abstract
We report on temperature-dependent soft X-ray absorption spectroscopy (XAS) measurements utilizing linearly polarized synchrotron radiation to probe magnetic phase transitions in iron-rich Fe1+yTe. X-ray magnetic linear dichroism (XMLD) signals, which sense magnetic ordering processes at surfaces, start to increase monotonically below the Neel temperature TN = 57 K. This increase is due to a progressive bicollinear antiferromagnetic (AFM) alignment of Fe spins of the monoclinic Fe1+yTe parent phase. This AFM alignment was achieved by a [100]-oriented biasing field favoring a single-domain state during cooling across TN. Our specific heat and magnetization measurements confirm the bulk character of this AFM phase transition. On longer time scales, however, we observe that the field-biased AFM state is highly unstable even at the lowest temperature of T = 3 K. After switching off the biasing field, the XMLD signal decays exponentially with a time constant {tau} = 1506 s. The initial XMLD signal is restored only upon repeating a cycle consisting of heating and field-cooling through TN. We explain the time effect by a gradual formation of a multi-domain state with 90 deg rotated AFM domains, promoted by structural disorder, facilitating the motion of twin-domains. Significant disorder in our Fe1+yTe sample is evident from our X-ray diffraction and specific heat data. The stability of magnetic phases in Fe-chalcogenides is an important material property, since the Fe(Te1-xSex) phase diagram shows magnetism intimately connected with superconductivity.
rate research
Read More
We report directional point-contact spectroscopy data on the novel Bi2Te3/Fe1+yTe interfacial superconductor for a Bi2Te3 thickness of 9 quintuple layers, bonded by van der Waals epitaxy to a Fe1+yTe film at an atomically sharp interface. Our data show a very large superconducting twin-gap structure with an energy scale exceeding that of bulk FeSe or FeSe1-xTex by a factor of 4. While the larger gap is isotropic and attributed to a thin FeTe layer in proximity of the interface, the smaller gap has a pronounced anisotropy and is associated with proximity-induced superconductivity in the topological insulator Bi2Te3. Zero resistance is lost above 8 K, but superconducting fluctuations are visible up to at least 12 K and the large gap is replaced by a pseudogap that persists up to 40 K. The spectra show a pronounced zero-bias conductance peak in the superconducting state, which may be a signature of an unconventional pairing mechanism.
CeAu2Si2 is a newly discovered pressure-induced heavy fermion superconductor which shows very unusual interplay between superconductivity and magnetism under pressure. Here we compare the results of high-pressure measurements on single crystalline CeAu2Si2 samples with different levels of disorder. It is found that while the magnetic properties are essentially sample independent, superconductivity is rapidly suppressed when the residual resistivity of the sample increases. We show that the depression of bulk Tc can be well understood in terms of pair breaking by nonmagnetic disorder, which strongly suggests an unconventional pairing state in pressurized CeAu2Si2. Furthermore, increasing the level of disorder leads to the emergence of another phase transition at T* within the magnetic phase, which might be in competition with superconductivity.
The recent discovery of the interfacial superconductivity (SC) of the Bi2Te3/Fe1+yTe heterostructure has attracted extensive studies due to its potential as a novel platform for trapping and controlling Majorana fermions. Here we present studies of another topological insulator (TI)/Fe1+yTe heterostructure, Sb2Te3/Fe1+yTe, which also enjoys an interfacial two-dimensional SC. The results of transport measurements support that the reduction of excess Fe concentration of the Fe1+yTe layer not only increases the fluctuation of its antiferromagnetic (AFM) order but also enhances the quality of the SC of this heterostructure system. On the other hand, the interfacial SC of this heterostructure was found to have a wider-ranging TI-layer thickness dependence than that of the Bi2Te3/Fe1+yTe heterostructure, which is believed to be attributed to the much higher bulk conductivity of Sb2Te3 that enhances indirect coupling between its top and bottom topological surface states (TSSs). Our results provide the evidence of the interplay among the AFM order, itinerant carries from the TSSs and the induced interfacial SC of the TI/Fe1+yTe heterostructure system.
We investigate the hydrostatic pressure dependence of interfacial superconductivity occurring at the atomically sharp interface between two non-superconducting materials: the topological insulator (TI) Bi2Te3 and the parent compound Fe1+yTe of the chalcogenide iron based superconductors. Under pressure, a significant increase in the superconducting transition temperature Tc is observed. We trace the pressure dependence of a superconducting twin gap structure by Andreev reflection point contact spectroscopy (PCARS), which shows that a large superconducting gap associated with the interfacial superconductivity increases along with Tc. A second smaller gap, which is attributed to proximity-induced superconductivity in the TI layer, increases first, but then reaches a maximum and appears to be gradually suppressed at higher pressure. We interpret our data in the context of a pressure-induced doping effect of the interface, in which charge is transferred from the TI layer to the interface and the interfacial superconductivity is enhanced. This demonstrates the important role of the TI in the interfacial superconductivity mechanism.
The quest to understand correlated electronic systems has pushed the frontiers of experimental measurements toward the development of new experimental techniques and methodologies. Here we use a novel home-built uniaxial-strain device integrated into our variable temperature scanning tunneling microscope that enables us to controllably manipulate in-plane uniaxial strain in samples and probe their electronic response at the atomic scale. Using scanning tunneling microscopy with spin-polarization techniques, we visualize antiferromagnetic domains and their atomic structure in Fe1+yTe samples, the parent compound of iron-based superconductors, and demonstrate how these domains respond to applied uniaxial strain. We observe the bidirectional antiferromagnetic domains in the unstrained sample, with an average domain size of 50 to 150 nm, to transition into a single unidirectional domain under applied uniaxial strain. The findings presented here open a new direction to utilize a valuable tuning parameter in scanning tunneling microscopy, as well as other spectroscopic techniques, both for tuning the electronic properties as for inducing symmetry breaking in quantum material systems.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
