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Register a new userObservation and control of shock waves in individual nanoplasmas
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In a novel experiment that images the momentum distribution of individual, isolated 100-nm-scale plasmas, we make the first experimental observation of shock waves in nanoplasmas. We demonstrate that the introduction of a heating pulse prior to the main laser pulse increases the intensity of the shock wave, producing a strong burst of quasi-monochromatic ions with an energy spread of less than 15%. Numerical hydrodynamic calculations confirm the appearance of accelerating shock waves, and provide a mechanism for the generation and control of these shock waves. This observation of distinct shock waves in dense plasmas enables the control, study, and exploitation of nanoscale shock phenomena with tabletop-scale lasers.
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The expansion of laser-irradiated clusters or nanodroplets depends strongly on the amount of energy delivered to the electrons and can be controlled by using appropriately shaped laser pulses. In this paper, a self-consistent kinetic model is used to analyze the transition from quasineutral, hydrodinamic-like expansion regimes to the Coulomb explosion (CE) regime when increasing the ratio between the thermal energy of the electrons and the electrostatic energy stored in the cluster. It is shown that a suitable double-pump irradiation scheme can produce hybrid expansion regimes, wherein a slow hydrodynamic expansion is followed by a fast CE, leading to ion overtaking and producing multiple ion flows expanding with different velocities. This can be exploited to obtain intracluster fusion reactions in both homonuclear deuterium clusters and heteronuclear deuterium-tritium clusters, as also proved by three-dimensional molecular-dynamics simulations.
We report a study of high harmonic generation from noble gas clusters of xenon atoms in a gas jet. Harmonic spectra were investigated as a function of backing pressure, showing spectral shifts due to the nanoplasma electrons in the clusters. At certain value of laser intensity this process may oppose the effect of the well-known ionization-induced blueshift. In addition, these cluster-induced harmonic redshifts may give the possibility to estimate cluster density and cluster size in the laser-gas jet interaction range.
The reversible control of a single spin of an atom or a molecule is of great interest in Kondo physics and a potential application in spin based electronics.Here we demonstrate that the Kondo resonance of manganese phthalocyanine molecules on an Au(111) substrate have been reversibly switched off and on via a robust route through attachment and detachment of single hydrogen atom to the magnetic core of the molecule. As further revealed by density functional theory calculations, even though the total number of electrons of the Mn ion remains almost the same in the process, gaining one single hydrogen atom leads to redistribution of charges within 3d orbitals with a reduction of the molecular spin state from S = 3/2 to S = 1 that directly contributes to the Kondo resonance disappearance. This process is reversed by a local voltage pulse or thermal annealing to desorb the hydrogen atom.
Supersonic beams are a prevalent source of cold molecules utilized in the study of chemical reactions, atom interferometry, gas-surface interactions, precision spectroscopy, molecular cooling and more. The triumph of this method emanates from the high densities produced in relation to other methods, however beam density remains fundamentally limited by interference with shock waves reflected from collimating surfaces. Here we show experimentally that this shock interaction can be reduced or even eliminated by cryo-cooling the interacting surface. An increase in beam density of nearly an order of magnitude was measured at the lowest surface temperature, with no further fundamental limitation reached. Visualization of the shock waves by plasma discharge and reproduction with direct simulation Monte Carlo calculations both indicate that the suppression of the shock structure is partially caused by lowering the momentum flux of reflected particles, and significantly enhanced by the adsorption of particles to the surface. We observe that the scaling of beam density with source pressure is recovered, paving the way to order of magnitude brighter cold molecular beams.
A peculiar ion behavior is found in a Si cluster, moving with a speed of ~0.22c (c: speed of light) in a solid Al plasma: the Si ion, moving behind the forward moving Si ion closely in a several angstrom distance in the cluster, feels the wake field generated by the forward Si. The interaction potential on the rear Si may balance the deceleration backward force by itself with the acceleration forward force by the forward Si in the longitudinal moving direction. The forward Si would be decelerated normally. However, the deceleration of the rear Si, moving behind closely, would be reduced significantly, and the rear Si may catch up and overtake the forward moving Si in the cluster during the Si cluster interaction with the high-density Al plasma.
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