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Beta-decay of Mn-65 to Fe-65

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 Added by Bruno Olaizola
 Publication date 2013
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and research's language is English




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The low energy structure of Fe-65 has been studied by means of gamma- and fast-timing spectroscopy. A level scheme of Fe-65 populated following the beta-decay of Mn-65 was established for the first time. It includes 41 levels and 85 transitions. The excitation energy of the beta-decaying isomer in Fe-65 has been precisely determined at 393.7(2) keV. The beta delayed neutron emission branch was measured as Pn = 7.9(12)%, which cannot be reconciled with the previously reported value of 21.0(5)%. Four gamma-rays and four excited states in Fe-64 were identified as being populated following the beta-n decay. Four lifetimes and five lifetime limits in the subnanosecond range have been measured using the Advanced Time-Delayed Method. The level scheme is compared with shell-model calculations. Tentative spin and parity assignments are proposed based on the observed transition rates, the calculations and the systematics of the region.

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Background: Shell evolution can impact the structure of the nuclei and lead to effects such as shape coexistence. The nuclei around $^{68}$Ni represent an excellent study case, however, spectroscopic information of the neutron-rich, $Z<28$ nuclei is limited. Purpose: The goal is to measure $gamma$-ray transitions in $^{66}$Fe, $^{66}$Co and $^{66}$Ni populated in the $beta^-$ decay of $^{66}$Mn, to determine absolute $beta$-feedings and relative $gamma$-decay probabilities and to compare the results with Monte Carlo Shell Model calculations in order to study the influence of the relevant single neutron and proton orbitals occupancies around $Z=28$ and $N=40$. Method: The low-energy structures of $^{65,66}$Fe, $^{66}$Co and $^{66}$Ni were studied in the $beta^-$ decay of $^{66}$Mn produced at ISOLDE, CERN. The beam was purified by means of laser resonance ionization and mass separation. The $beta$ and $gamma$ events detected by three plastic scintillators and two MiniBall cluster germanium detectors, respectively, were correlated in time to build the low-energy excitation schemes and to determine the $beta$-decay half-lives of the nuclei. Results: The relative small $beta$-decay ground state feeding of $^{66}$Fe obtained in this work is at variant to the earlier studies. Spin and parity $1^+$ was assigned to the $^{66}$Co ground state based on the strong ground state feeding in the decay of $^{66}$Fe as well as in the decay of $^{66}$Co. Experimental log(ft) values, $gamma$-ray deexcitation patterns and energies of excited states were compared to Monte Carlo Shell Model calculations. Based on this comparison, spin and parity assignments for the selected number of low-lying states in the $^{66}$Mn to $^{66}$Ni chain were proposed. Conclusions: The $beta$-decay chain starting $^{66}$Mn towards $^{66}$Ni, crossing $N=40$, evolves from deformed nuclei to sphericity...
The use of chemically selective laser ionization combined with beta-delayed neutron counting at CERN/ISOLDE has permitted identification and half-life measurements for 623-ms Mn-61 up through 14-ms Mn-69. The measured half-lives are found to be significantly longer near N=40 than the values calculated with a QRPA shell model using ground-state deformations from the FRDM and ETFSI models. Gamma-ray singles and coincidence spectroscopy has been performed for Mn-64 and Mn-66 decays to levels of Fe-64 and Fe-66, revealing a significant drop in the energy of the first 2+ state in these nuclides that suggests an unanticipated increase in collectivity near N=40.
Sub-barrier Coulomb-excitation was performed on a mixed beam of $^{62}$Mn and $^{62}$Fe, following in-trap $beta^{-}$ decay of $^{62}$Mn at REX-ISOLDE, CERN. The trapping and charge breeding times were varied in order to alter the composition of the beam, which was measured by means of an ionisation chamber at the zero-angle position of the Miniball array. A new transition was observed at 418~keV, which has been tentatively associated to a $(2^{+},3^{+})rightarrow1^{+}_{g.s.}$ transition. This fixes the relative positions of the $beta$-decaying $4^{+}$ and $1^{+}$ states in $^{62}$Mn for the first time. Population of the $2^{+}_{1}$ state was observed in $^{62}$Fe and the cross-section determined by normalisation to the $^{109}$Ag target excitation, confirming the $B(E2)$ value measured in recoil-distance lifetime experiments.
Elastic scattering of photons from 12C has been investigated using quasi-monoenergetic tagged photons with energies in the range 65 - 115 MeV at laboratory angles of 60 deg, 120 deg, and 150 deg at the Tagged-Photon Facility at the MAX IV Laboratory in Lund, Sweden. A phenomenological model was employed to provide an estimate of the sensitivity of the 12C(g,g)12C cross section to the bound-nucleon polarizabilities.
The results of a study of the beta decays of three proton-rich nuclei with $T_z=text{-}2$, namely $^{48}$Fe, $^{52}$Ni and $^{56}$Zn, produced in an experiment carried out at GANIL, are reported. In all three cases we have extracted the half-lives and the total $beta$-delayed proton emission branching ratios. We have measured the individual $beta$-delayed protons and $beta$-delayed $gamma$ rays and the branching ratios of the corresponding levels. Decay schemes have been determined for the three nuclei, and new energy levels are identified in the daughter nuclei. Competition between $beta$-delayed protons and $gamma$ rays is observed in the de-excitation of the $T=2$ Isobaric Analogue States in all three cases. Absolute Fermi and Gamow-Teller transition strengths have been determined. The mass excesses of the nuclei under study have been deduced. In addition, we discuss in detail the data analysis taking as a test case $^{56}$Zn, where the exotic $beta$-delayed $gamma$-proton decay has been observed.
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