In this work we report the modification of the normal Auger line shape under the action of an intense x-ray radiation. Under strong Rabi-type coupling of the core, the Auger line profile develops into a doublet structure with an energy separation mainly determined by the relative strength of the Rabi coupling. In addition, we find that the charge resolved ion yields can be controlled by judicious choice of the x-ray frequency.
We review the main aspects of multiple photoionization processes in atoms exposed to intense, short wavelength radiation. The main focus is the theoretical framework for the description of such processes as well as the conditions under which direct multiphoton multiple ionization processes can dominate over the sequential ones. We discuss in detail the mechanisms available in different wavelength ranges from the infrared to the hard X-rays. The effect of field fluctuations, present at this stage in all SASE free-electron-laser (FEL) facilities, as well as the effect of the interaction volume integration, are also discussed.
We report the observation of a novel nonlinear effect in the hard x-ray range. Upon illuminating Fe and Cu metal foils with intense x-ray pulses tuned near their respective K edges, photons at nearly twice the incoming photon energy are emitted. The signal rises quadratically with the incoming intensity, consistent with two-photon excitation. The spectrum of emitted high-energy photons comprises multiple Raman lines that disperse with the incident photon energy. Upon reaching the double K-shell ionization threshold, the signal strength undergoes a marked rise. Above this threshold, the lines cease dispersing, turning into orescence lines with energies much greater than obtainable by single electron transitions, and additional Raman lines appear. We attribute these processes to electron-correlation mediated multielectron transitions involving double-core hole excitation and various two-electron de-excitation processes to a final state involving one or more L and M core-holes.
We investigate the effects of static electric and magnetic fields on the differential ac Stark shifts for microwave transitions in ultracold bosonic $^{87}$Rb$^{133}$Cs molecules, for light of wavelength $lambda = 1064~mathrm{nm}$. Near this wavelength we observe unexpected two-photon transitions that may cause trap loss. We measure the ac Stark effect in external magnetic and electric fields, using microwave spectroscopy of the first rotational transition. We quantify the isotropic and anisotropic parts of the molecular polarizability at this wavelength. We demonstrate that a modest electric field can decouple the nuclear spins from the rotational angular momentum, greatly simplifying the ac Stark effect. We use this simplification to control the ac Stark shift using the polarization angle of the trapping laser.
We present a rather elaborate theoretical model describing the dynamics of Neon under radiation of photon energies $sim 93$ eV and pulse duration in the range of 15 fs, within the framework of Lowest non-vanishing Order of Perturbation Theory (LOPT), cast in terms of rate equations. Our model includes sequential as well as direct multiple ionization channels from the 2s and 2p atomic shells, including aspects of fine structure, whereas the stochastic nature of SASE-FEL light pulses is also taken into account. Our predictions for the ionization yields of the different ionic species are in excellent agreement with the related experimental observations at FLASH.
High-precision magnetic field measurement is an ubiquitous issue in physics and a critical task in metrology. Generally, magnetic field has DC and AC components and it is hard to extract both DC and AC components simultaneously. The conventional Ramsey interferometry can easily measure DC magnetic fields, while it becomes invalid for AC magnetic fields since the accumulated phases may average to zero. Here, we propose a scheme for simultaneous measurement of DC and AC magnetic fields by combining Ramsey interferometry and rapid periodic pulses. In our scheme, the interrogation stage is divided into two signal accumulation processes linked by a unitary operation. In the first process, only DC component contributes to the accumulated phase. In the second process, by applying multiple rapid periodic $pi$ pulses, only the AC component gives rise to the accumulated phase. By selecting suitable input state and the unitary operations in interrogation and readout stages, and the DC and AC components can be extracted by population measurements. In particular, if the input state is a GHZ state and two interaction-based operations are applied during the interferometry, the measurement precisions of DC and AC magnetic fields can approach the Heisenberg limit simultaneously. Our scheme provides a feasible way to achieve Heisenberg-limited simultaneous measurement of DC and AC fields.
L. A. A. Nikolopoulos
,T. J. Kelly
,J. T. Costello
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(2011)
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"Theory of ac-Stark splitting in core-resonant Auger decay under strong x-ray fields"
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Lampros Nikolopoulos aa
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